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Data for: The branching ratio of intercombination $A^1Sigma^+sim b^3Pito a^3Sigma^+/X^1Sigma^+$ transitions in the RbCs molecule: measurements and calculations 数据:红细胞分子中相互结合的分支比$A^1Sigma^+sim b^3Pito a^3Sigma^+/X^1Sigma^+$跃迁:测量和计算
arXiv: Atomic Physics Pub Date : 2020-07-09 DOI: 10.17632/M256T3PV3R.1
R. Ferber, A. Stolyarov
{"title":"Data for: The branching ratio of intercombination $A^1Sigma^+sim b^3Pito a^3Sigma^+/X^1Sigma^+$ transitions in the RbCs molecule: measurements and calculations","authors":"R. Ferber, A. Stolyarov","doi":"10.17632/M256T3PV3R.1","DOIUrl":"https://doi.org/10.17632/M256T3PV3R.1","url":null,"abstract":"We observed the $A^1Sigma^+sim b^3Pito a^3Sigma^+/X^1Sigma^+$ laser-induced fluorescence (LIF) spectra of the RbCs molecule excited from the ground $X^1Sigma^+$ state by the Ti:Sapphire laser. The LIF radiation from the common perturbed levels of the singlet-triplet $Asim b$ complex was recorded by the Fourier-transform (FT) spectrometer with the instrumental resolution of 0.03~cm$^{-1}$. The relative intensity distribution in the rotationally resolved $Asim bto a^3Sigma^+(v_a)/X^1Sigma^+(v_X)$ progressions was measured, and their branching ratio was found to be about of 1$÷$5$ times$10$^{-4}$ in the bound region of the $a^3Sigma^+$ and $X^1Sigma^+$ states. The experiment was complemented with the scalar and full relativistic calculations of the $A/b - X/a$ transition dipole moments (TDMs) as functions of internuclear distance. The relative systematic error in the resulting emph{ab initio} TDM functions evaluated for the strong $A - X$ transition was estimated as few percent in the energy region, where the experimental LIF intensities are relevant. The relative spectral sensitivity of the FT registration system, operated with the InGaAs diode detector and CaF beam-splitter, was calibrated in the range $[6~500,12~000]$~cm$^{-1}$ by a comparison of experimental intensities in the long $Asim bto X(v_X)$ LIF progressions of the K$_2$ and KCs molecules with their theoretical counterparts evaluated using the emph{ab initio} $A - X$ TDMs. Both experimental and theoretical transition probabilities can be employed to improve the stimulated Raman adiabatic passage process, $ato Asim b to X$, which is exploited for a laser assembling of ultracold RbCs molecules.","PeriodicalId":8441,"journal":{"name":"arXiv: Atomic Physics","volume":"64 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2020-07-09","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"80831677","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Sequential single-photon and direct two-photon absorption processes for Xe interacting with attosecond XUV pulses Xe与阿秒XUV脉冲相互作用的顺序单光子和直接双光子吸收过程
arXiv: Atomic Physics Pub Date : 2020-07-03 DOI: 10.1103/physreva.102.043108
A. Hadjipittas, H. Banks, B. Bergues, A. Emmanouilidou
{"title":"Sequential single-photon and direct two-photon absorption processes for Xe interacting with attosecond XUV pulses","authors":"A. Hadjipittas, H. Banks, B. Bergues, A. Emmanouilidou","doi":"10.1103/physreva.102.043108","DOIUrl":"https://doi.org/10.1103/physreva.102.043108","url":null,"abstract":"We investigate the interaction of Xe with isolated attosecond XUV pulses. Specifically, we calculate the ion yields and determine the pathways leading to the formation of ionic charged states up to Xe$^{5+}$. To do so, in our formulation we account for single-photon absorption, sequential multi-photon absorption, direct two-photon absorption, single and double Auger decays, and shake-off. We compare our results for the ion yields and for ion yield ratios with recent experimental results obtained for 93 eV and 115 eV attosecond XUV pulses. In particular, we investigate the role that a sequence of two single-photon ionization processes plays in the formation of Xe$^{4+}$. We find that each one of these two processes ionizes a core electron and thus leads to the formation of a double core-hole state. Remarkably, we find that the formation of Xe$^{5+}$ involves a direct two-photon absorption process and the absorption of a total of three photons.","PeriodicalId":8441,"journal":{"name":"arXiv: Atomic Physics","volume":"61 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2020-07-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"82580471","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 2
Theoretical determination of polarizability and magnetic susceptibility of neon 氖的极化率和磁化率的理论测定
arXiv: Atomic Physics Pub Date : 2020-06-27 DOI: 10.1103/physreva.102.052816
M. Lesiuk, M. Przybytek, B. Jeziorski
{"title":"Theoretical determination of polarizability and magnetic susceptibility of neon","authors":"M. Lesiuk, M. Przybytek, B. Jeziorski","doi":"10.1103/physreva.102.052816","DOIUrl":"https://doi.org/10.1103/physreva.102.052816","url":null,"abstract":"We report theoretical determination of the dipole polarizability of the neon atom, including its frequency dependence. Corrections for the relativistic, quantum electrodynamics, finite nuclear mass, and finite nuclear size effects are taken into account. We obtain the value $alpha_0=2.66080(36)$ for the static polarizability, and $alpha_2=2.850(7)$ and $alpha_4=4.932(14)$ for the first two polarizability dispersion coefficients (Cauchy moments); all values are in atomic units (a.u.). In the case of static polarizability, our result agrees with the best experimental determination [C. Gaiser and B. Fellmuth, Phys. Rev. Lett. 120, 123203 (2018)], but our estimated uncertainty is significantly larger. For the dispersion coefficients, the results obtained in this work appear to be the most accurate to date overall compared to published theoretical and experimental data. We also calculated the static magnetic susceptibility of the neon atom, needed to obtain the refractive index of gaseous neon. Our result, $chi_0 = -8.484(19) cdot 10^{-5}$ a.u., is about 9% larger in absolute value than the recommended experimental value [CRC Handbook of Chemistry and Physics, CRC Press, 2019, p. 4-145].","PeriodicalId":8441,"journal":{"name":"arXiv: Atomic Physics","volume":"189 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2020-06-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"77359741","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 8
Magnetometry using sodium fluorescence with synchronous modulation of two-photon resonant light fields 同步调制双光子共振光场的钠荧光磁强计
arXiv: Atomic Physics Pub Date : 2020-06-25 DOI: 10.1063/5.0030696
R. Grewal, Mauricio Pulido, G. Pati, R. Tripathi
{"title":"Magnetometry using sodium fluorescence with synchronous modulation of two-photon resonant light fields","authors":"R. Grewal, Mauricio Pulido, G. Pati, R. Tripathi","doi":"10.1063/5.0030696","DOIUrl":"https://doi.org/10.1063/5.0030696","url":null,"abstract":"We report a new technique for generating magnetic resonance with synchronous modulation of two-photon resonant light fields. Magnetic resonances in fluorescence from a sodium cell are measured to demonstrate suitability of this technique for remote magnetometry. A strong magnetic resonance with its dip corresponding to the Larmor frequency is produced in the presence of a transverse magnetic field. An additional resonance at 3{Omega_L} is observed, which can be used to determine the magnetic field orientation. We have developed a theoretical model based on the density matrix equations to verify our experimental observations. An average magnetic field sensitivity of 41 mathbf{pT}/sqrt{mathbf{Hz}} is measured using light duty cycles ranging from 35% to 10%. We have discussed possible changes that can be made to improve the sensitivity of this scheme further.","PeriodicalId":8441,"journal":{"name":"arXiv: Atomic Physics","volume":"1 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2020-06-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"80993676","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 5
Ellipticity-dependent sequential over-barrier ionization of cold rubidium 依赖椭圆度的冷铷序贯过势垒电离
arXiv: Atomic Physics Pub Date : 2020-06-16 DOI: 10.1103/physreva.102.043112
J. Yuan, Shiwei Liu, Xincheng Wang, Z. Shen, Yixuan Ma, Huanyu Ma, Qiuxiang Meng, T. Yan, Yizhu Zhang, A. Dorn, M. Weidemüller, D. Ye, Yuhai Jiang
{"title":"Ellipticity-dependent sequential over-barrier ionization of cold rubidium","authors":"J. Yuan, Shiwei Liu, Xincheng Wang, Z. Shen, Yixuan Ma, Huanyu Ma, Qiuxiang Meng, T. Yan, Yizhu Zhang, A. Dorn, M. Weidemüller, D. Ye, Yuhai Jiang","doi":"10.1103/physreva.102.043112","DOIUrl":"https://doi.org/10.1103/physreva.102.043112","url":null,"abstract":"We perform high-resolution measurements of momentum distribution on Rb$^{n+}$ recoil ions up to charge state $n=4$, where laser-cooled rubidium atoms are ionized by femtosecond elliptically polarized lasers with the pulse duration of 35 fs and the intensity of 3.3$times$10$^{15}$ W/cm$^2$ in the over-barrier ionization (OBI) regime. The momentum distributions of the recoil ions are found to exhibit multi-band structures as the ellipticity varies from the linear to circular polarizations. The origin of these band structures can be explained quantitatively by the classical OBI model and dedicated classical trajectory Monte Carlo simulations with Heisenberg potential. Specifically, with back analysis of the classical trajectories, we reveal the ionization time and the OBI geometry of the sequentially released electrons, disentangling the mechanisms behind the tilted angle of the band structures. These results indicate that the classical treatment can describe the strong-field multiple ionization processes of alkali atoms.","PeriodicalId":8441,"journal":{"name":"arXiv: Atomic Physics","volume":"11 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2020-06-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"78223197","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 3
Cavity probe for real-time detection of atom dynamics in an optical lattice 用于光学晶格中原子动力学实时探测的腔探针
arXiv: Atomic Physics Pub Date : 2020-06-08 DOI: 10.1103/physreva.102.051301
R. Niederriter, Chandler Schlupf, P. Hamilton
{"title":"Cavity probe for real-time detection of atom dynamics in an optical lattice","authors":"R. Niederriter, Chandler Schlupf, P. Hamilton","doi":"10.1103/physreva.102.051301","DOIUrl":"https://doi.org/10.1103/physreva.102.051301","url":null,"abstract":"We propose and demonstrate real-time sub-wavelength cavity QED measurements of the spatial distribution of atoms in an optical lattice. Atoms initially confined in one \"trap\" standing wave of an optical cavity mode are probed with a second \"probe\" standing wave. With frequencies offset by one free spectral range, the nodes of the trap fall on the anti-nodes of the probe in the ${approx}$10$^4$ lattice sites around the center of the cavity. This lattice site independent atom-cavity coupling enables high sensitivity detection of atom dynamics even with atoms spread over many lattice sites. To demonstrate, we measure the temperature of 20-70 $mu$K atom ensembles in ${<}$10 $mu$s by monitoring their expansion of ${approx}$100 nm after sudden release from the trap lattice. Atom-cavity coupling imprints the atom dynamics on the probe transmission. The new technique will enable improved non-destructive detection of Bloch oscillations and other atom dynamics in optical lattices.","PeriodicalId":8441,"journal":{"name":"arXiv: Atomic Physics","volume":"97 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2020-06-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"81631844","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 6
Perturbative theory of statistically averaged atomic dynamics in fluctuating laser fields 波动激光场中统计平均原子动力学的微扰理论
arXiv: Atomic Physics Pub Date : 2020-06-03 DOI: 10.1103/physreva.102.053111
Tejaswi Katravulapally, L. A. A. Nikolopoulos
{"title":"Perturbative theory of statistically averaged atomic dynamics in fluctuating laser fields","authors":"Tejaswi Katravulapally, L. A. A. Nikolopoulos","doi":"10.1103/physreva.102.053111","DOIUrl":"https://doi.org/10.1103/physreva.102.053111","url":null,"abstract":"We have developed a perturbative method to model the resonant ionization of atomic systems in fluctuating laser fields. The perturbative method is based on an expansion in terms of the multitime cumulants, a suitable combination of moments (field's coherence functions), used to represent the field's statistical properties. The second-order truncated expansion is expressed in terms of the radiation's power spectrum and the intensity autocorrelation function. We investigate the range of validity of the model in terms of the field's coherence temporal length and peak intensity and have compared the results with conventional Monte-Carlo calculations. We apply the theory in the case of a near-resonant ionization of the Helium 2s2p autoionizing state with a SASE FEL pulse with square-exponentially dependent 1st-order coherence function. The ionization lineshape profile acquires a Voight profile; the degree of the Gaussian or Lorentzian character of which to depend crucially on the field's coherence time.","PeriodicalId":8441,"journal":{"name":"arXiv: Atomic Physics","volume":"28 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2020-06-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"82728040","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Establishing a nearly closed cycling transition in a polyatomic molecule 在多原子分子中建立近乎封闭的循环跃迁
arXiv: Atomic Physics Pub Date : 2020-06-02 DOI: 10.1103/PhysRevA.103.043111
L. Baum, N. Vilas, Christian Hallas, B. Augenbraun, S. Raval, D. Mitra, J. Doyle
{"title":"Establishing a nearly closed cycling transition in a polyatomic molecule","authors":"L. Baum, N. Vilas, Christian Hallas, B. Augenbraun, S. Raval, D. Mitra, J. Doyle","doi":"10.1103/PhysRevA.103.043111","DOIUrl":"https://doi.org/10.1103/PhysRevA.103.043111","url":null,"abstract":"We study optical cycling in the polar free radical calcium monohydroxide (CaOH) and establish an experimental path towards scattering >$10^4$ photons. We report vibrational branching ratio measurements with accuracy at the $sim$$5 times 10^{-4}$ level and observe weak symmetry-forbidden decays to bending modes with non-zero vibrational angular momentum. Quantitative theory is developed to explain these observations and predict additional decay pathways. Additionally, we perform high-resolution spectroscopy of the $widetilde{text{X}},^2Sigma^+(12^00)$ and $widetilde{text{X}},^2Sigma^+(12^20)$ hybrid vibrational states of CaOH. These advances establish a path towards radiative slowing, 3D magneto-optical trapping, and sub-Doppler cooling of CaOH.","PeriodicalId":8441,"journal":{"name":"arXiv: Atomic Physics","volume":"23 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2020-06-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"83078843","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 17
Role of rotational coherence in femtosecond-pulse-driven nitrogen ion lasing 旋转相干性在飞秒脉冲驱动氮离子激光中的作用
arXiv: Atomic Physics Pub Date : 2020-05-22 DOI: 10.1103/PHYSREVRESEARCH.2.023329
Hongqiang Xie, H. Lei, Guihua Li, Qian Zhang, Xiaowei Wang, Jing Zhao, Zhiming Chen, J. Yao, Ya Cheng, Zengxiu Zhao
{"title":"Role of rotational coherence in femtosecond-pulse-driven nitrogen ion lasing","authors":"Hongqiang Xie, H. Lei, Guihua Li, Qian Zhang, Xiaowei Wang, Jing Zhao, Zhiming Chen, J. Yao, Ya Cheng, Zengxiu Zhao","doi":"10.1103/PHYSREVRESEARCH.2.023329","DOIUrl":"https://doi.org/10.1103/PHYSREVRESEARCH.2.023329","url":null,"abstract":"We experimentally investigated the rotationally resolved polarization characteristics of N$_2^+$ lasing at 391 and 428 nm using a pump-seed scheme. By varying the relative angle between the linear polarizations of the pump and seed, it is found that the polarizations of the P and R branches of 391-nm lasing are counter-rotated. By contrast, both branches of 428-nm lasing remain polarized along the pump. The origin of the puzzled abnormal polarization characteristics is found based on a complete physical model that simultaneously includes the transient photoionization and the subsequent coupling among the electronic, vibrational and rotational quantum states of this http URL suggests that the cascaded resonant Raman processes following ionization create negative coherence between the rotational states of $J$ and $J$+2 in the ionic ground state X$^2Sigma_g^+(nu=0)$, which leads to mirror-symmetrical polarization for the P and R branches of 391-nm lasing. Both the experiment and theory indicate that the demonstrated rotational coherence plays an extremely pivotal role in clarifying the gain mechanism of N$_2^+$ lasing and opens up the route toward quantum optics under ultrafast strong fields.","PeriodicalId":8441,"journal":{"name":"arXiv: Atomic Physics","volume":"121 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2020-05-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"76199097","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 13
Magneto-Optical Trap with Millimeter Ball Lenses 毫米球透镜磁光阱
arXiv: Atomic Physics Pub Date : 2020-05-20 DOI: 10.1103/PHYSREVAPPLIED.14.044013
C. S. Nichols, L. Nofs, M. Viray, Lu Ma, E. Paradis, G. Raithel
{"title":"Magneto-Optical Trap with Millimeter Ball Lenses","authors":"C. S. Nichols, L. Nofs, M. Viray, Lu Ma, E. Paradis, G. Raithel","doi":"10.1103/PHYSREVAPPLIED.14.044013","DOIUrl":"https://doi.org/10.1103/PHYSREVAPPLIED.14.044013","url":null,"abstract":"We present a magneto-optical trap (MOT) design based on millimeter ball lenses, contained within a metal cube of 0.75$^{prime prime}$ side length. We present evidence of trapping approximately $4.2times 10^5$ of $^{85}$Rb atoms with a number density of $3.2times 10^9$ atoms/cm$^{3}$ and a loading time of 1.3 s. Measurement and a kinetic laser-cooling model are used to characterize the atom trap design. The design provides several advantages over other types of MOTs: the laser power requirement is low, the small lens and cube sizes allow for miniaturization of MOT applications, and the lack of large-diameter optical beam pathways prevents external blackbody radiation from entering the trapping region.","PeriodicalId":8441,"journal":{"name":"arXiv: Atomic Physics","volume":"26 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2020-05-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"84611807","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 3
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