Transactions of the Materials Research Society of Japan最新文献

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Preparation and performance study of intrinsic self-healing epoxy composite based on phase separation 基于相分离的本征自愈环氧复合材料的制备及性能研究
Transactions of the Materials Research Society of Japan Pub Date : 2025-08-01 DOI: 10.1016/j.tramat.2025.100159
Xiaochen Xue, Wenqi Xie, Shengrong Zhao, Kaiyun Fu, Yinmin Zhang, Yongfeng Zhang, Yace Mi
{"title":"Preparation and performance study of intrinsic self-healing epoxy composite based on phase separation","authors":"Xiaochen Xue, Wenqi Xie, Shengrong Zhao, Kaiyun Fu, Yinmin Zhang, Yongfeng Zhang, Yace Mi","doi":"10.1016/j.tramat.2025.100159","DOIUrl":"https://doi.org/10.1016/j.tramat.2025.100159","url":null,"abstract":"Intrinsic self-healing epoxy composites were successfully prepared through reaction-induced phase separation, utilizing diglycidyl ether of bisphenol A (DGEBA) and 4,4'-diaminodicyclohexyl methane (DDCM) as the continuous phase, linseed oil (Lo) as the healing phase and silica as the regulatory and reinforcing phase, resulting in the formation of uniformly sized and controllably distributed micron-scale healing units. Notably, the incorporation of silica particles compensates for the strength loss caused by Lo, while also enabling a breakthrough in overall performance through multiphase synergy. The composite containing 1.5 wt% hydrophobically modified fumed silica (MFS) exhibited optimal properties, with a flexural strength of 144.66 MPa and an impact strength of 31.91 kJ/m 2 , both surpassing those of pure epoxy. Additionally, it had a low friction coefficient of 0.042 and minimal wear loss of 0.024 g/0.5 h. Furthermore, electrochemical impedance spectroscopy confirmed its superior long-term anticorrosion performance, with higher values of R f (1.1×107 Ω·cm 2 ) and R ct (7.2×106 Ω·cm 2 ) compared to the pure epoxy system, representing approximately 3.9 times and 3.8 times the corresponding values of the pure epoxy coating, respectively. This work successfully overcomes the traditional compromise between mechanical properties and self-healing functionality, establishing a practical materials design strategy for advanced protective coatings and structural composites requiring multifunctional performance.","PeriodicalId":237990,"journal":{"name":"Transactions of the Materials Research Society of Japan","volume":"1 8","pages":"100159-100159"},"PeriodicalIF":0.0,"publicationDate":"2025-08-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147917200","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Low-dimensional structure and strong anharmonicity render Sn2S3 low thermal conductivity in the Sn-S system Sn2S3在Sn-S体系中的低维结构和强非调和性使得Sn2S3的导热系数较低
Transactions of the Materials Research Society of Japan Pub Date : 2025-06-01 DOI: 10.1016/j.tramat.2025.100103
Yumo Zhu, Shaoping Zhan, Shulin Bai, Yi Wen, Hongyao Xie, Haonan Shi, Lizhong Su, Lei Wang, Shibo Liu, Dongrui Liu, Li‐Dong Zhao
{"title":"Low-dimensional structure and strong anharmonicity render Sn2S3 low thermal conductivity in the Sn-S system","authors":"Yumo Zhu, Shaoping Zhan, Shulin Bai, Yi Wen, Hongyao Xie, Haonan Shi, Lizhong Su, Lei Wang, Shibo Liu, Dongrui Liu, Li‐Dong Zhao","doi":"10.1016/j.tramat.2025.100103","DOIUrl":"https://doi.org/10.1016/j.tramat.2025.100103","url":null,"abstract":"Recent research on Sn-S-based semiconductor materials has revealed their significant potential as thermoelectric materials, owing to their inherently wide bandgap structure and electrical characteristics featuring multiband transport at elevated temperatures. However, their relatively high phonon frequencies and sound velocities, stemming from the lighter atomic masses and the strong covalent Sn-S bonds, limit their performance. Consequently, developing novel Sn-S-based thermoelectric materials with intrinsically low thermal conductivity is crucial. Herein, we constructed a composition with a stoichiometric Sn to S ratio of 2:3. Using a low-temperature powder fusion synthesis method, we successfully obtained an intrinsically p-type semiconductor material with low thermal conductivity. Sn 2 S 3 , synthesized from SnS and SnS 2 , exhibits ultralow lattice thermal conductivity κ lat (∼1.16 W/m·K at 300 K) due to the strong anharmonicity induced by weak bonding, low symmetry, and lone pairs. Furthermore, detailed structural/elastic analyses link large Grüneisen parameters to the low κ lat , advancing low- κ lat thermoelectric design.","PeriodicalId":237990,"journal":{"name":"Transactions of the Materials Research Society of Japan","volume":"1 6","pages":"100103-100103"},"PeriodicalIF":0.0,"publicationDate":"2025-06-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147893844","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Smart thermal-shutdown separators with fast response for safe Li-metal batteries 智能热关闭分离器,具有快速响应的安全锂金属电池
Transactions of the Materials Research Society of Japan Pub Date : 2025-05-01 DOI: 10.1016/j.tramat.2025.100096
Ruifeng Song, Nuo Li, Tianyi Hou, Yue Zhang, Jie Zhao, Zhenyu Huang, Yihan Wu, Hongbin Wang, Cong Wang, Guangyu Bian, Min Wang, Yunhui Huang, Henghui Xu
{"title":"Smart thermal-shutdown separators with fast response for safe Li-metal batteries","authors":"Ruifeng Song, Nuo Li, Tianyi Hou, Yue Zhang, Jie Zhao, Zhenyu Huang, Yihan Wu, Hongbin Wang, Cong Wang, Guangyu Bian, Min Wang, Yunhui Huang, Henghui Xu","doi":"10.1016/j.tramat.2025.100096","DOIUrl":"https://doi.org/10.1016/j.tramat.2025.100096","url":null,"abstract":"Rapid and efficient thermal shutdown separators are essential to enhance Li-metal battery safety by swiftly blocking ionic conduction pathways before thermal runaway. Existing thermal-responsive separators, however, face significant limitations, including high shutdown temperatures, sluggish response times, and inadequate thermal stability, severely restricting their practical deployment. This work proposed a tri-layer smart separator featuring a polybutylene succinate (PBS) thermal-responsive interlayer sandwiched by two robust boron nitride (BN)-enhanced polyvinylidene fluoride (PVDF) outer layers. At approximately 115 ​°C, the PBS interlayer quickly melts to form a pore-free barrier, effectively blocking lithium-ion transport within minutes. Simultaneously, the thermally conductive PVDF-BN layers retain structural integrity and facilitate efficient heat dissipation, ensuring rapid and stable thermal shutdown. This synergistic multi-layer approach achieves significant improvements in battery safety, demonstrated by: (1) an 11-fold reduction in discharge current compared to conventional polyolefin separators after overheated, (2) a delay of thermal-induced internal short circuit onset by up to 293 ​min, and (3) enhanced suppression of lithium dendrite growth, resulting in exceptional cycling stability with 95 ​% capacity retention over 3000 ​h. Additionally, the increased thermal conductivity (1.51 ​W/mK) ensures uniform internal heat distribution, minimizing localized hotspots. Our findings present a practical route for developing advanced separators with integrated thermal management capability.","PeriodicalId":237990,"journal":{"name":"Transactions of the Materials Research Society of Japan","volume":"1 5","pages":"100096-100096"},"PeriodicalIF":0.0,"publicationDate":"2025-05-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147332027","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 2
Synergistic effect of boron and nitrogen co-doping on anthracite-based hard carbon anode toward enhanced sodium storage 硼氮共掺杂对无烟煤基硬碳阳极增强钠储存的协同效应
Transactions of the Materials Research Society of Japan Pub Date : 2025-04-01 DOI: 10.1016/j.tramat.2025.100069
Yanhong Zhao, Zhuang Hu, Jingtong Chen, Peng Gao, Zhixiao Liu, Yan Duan, Aiping Hu, Changling Fan, Jilei Liu
{"title":"Synergistic effect of boron and nitrogen co-doping on anthracite-based hard carbon anode toward enhanced sodium storage","authors":"Yanhong Zhao, Zhuang Hu, Jingtong Chen, Peng Gao, Zhixiao Liu, Yan Duan, Aiping Hu, Changling Fan, Jilei Liu","doi":"10.1016/j.tramat.2025.100069","DOIUrl":"https://doi.org/10.1016/j.tramat.2025.100069","url":null,"abstract":"Anthracite-based carbon materials are widely regarded as practical anode materials for sodium-ion batteries due to their abundant resources, cost-effectiveness, high carbon yield, and excellent chemical stability. However, their widespread applications are hindered by issues such as poor cycling performance, limited storage capacity, and low coulombic efficiency. Herein, we propose an innovative “construction-release-repair” design strategy that leverages the synergistic effect of B/N co-doping to address these challenges. By constructing B–N bonds, releasing unstable heteroatoms, and repairing defect sites on carbon layers, this strategy significantly enhances the microstructure and surface engineering of anthracite-based hard carbon. The optimized hard carbon anode delivers high specific capacity of 344.2 mAh g -1 at 0.03 A g -1 with an initial coulombic efficiency of 85.3%, and excellent cycle retention of 88.2% after 500 cycles at 0.2 A g -1 . In-situ Raman spectroscopy and density functional theory calculations reveal that the B/N synergistic effect enhances the sodium-ion adsorption, reduces the diffusion barrier, and enhances reaction activity, facilitating more efficient intercalation and nanopore filling in the low-voltage plateau region. This work offers valuable insights into microstructure regulation and the design of high-performance anode for sodium-ion materials. This work proposes a \"construction-release-repair\" design strategy, utilizing the synergistic effect of B/N co-doping to enhance the microstructure and surface engineering of anthracite, resulting in coal-based hard carbon with high initial coulombic efficiency and capacity. DFT calculations demonstrate that the synergistic effect improves sodium ion adsorption, reduces diffusion barriers, and significantly enhances anode reaction activity.","PeriodicalId":237990,"journal":{"name":"Transactions of the Materials Research Society of Japan","volume":"1 4","pages":"100069-100069"},"PeriodicalIF":0.0,"publicationDate":"2025-04-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147880861","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 6
Thermally conductive bidirectional carbon structure enhanced heat-dissipative aluminum framework composites 导热双向碳结构增强散热铝骨架复合材料
Transactions of the Materials Research Society of Japan Pub Date : 2025-03-01 DOI: 10.1016/j.tramat.2025.100038
Yaotian Yan, Bin Wang, Peixin Li, Bin Qin, Zhenyu Ye, Yong Xia, Zilong Zhang, Zeyu Wang, Yanmei Li, Xiaohang Zheng, Hassaan Ahmad Butt, Dmitry V. Krasnikov, Albert G. Nasibulin, Jian Cao, Junlei Qi
{"title":"Thermally conductive bidirectional carbon structure enhanced heat-dissipative aluminum framework composites","authors":"Yaotian Yan, Bin Wang, Peixin Li, Bin Qin, Zhenyu Ye, Yong Xia, Zilong Zhang, Zeyu Wang, Yanmei Li, Xiaohang Zheng, Hassaan Ahmad Butt, Dmitry V. Krasnikov, Albert G. Nasibulin, Jian Cao, Junlei Qi","doi":"10.1016/j.tramat.2025.100038","DOIUrl":"https://doi.org/10.1016/j.tramat.2025.100038","url":null,"abstract":"Lightweight, highly integrated and miniaturized modern high-power electronic devices put forward higher requirements on the heat removal efficiency of heat sinks. Herein, the bidirectional carbon hierarchical structure consisting of high crystalline carbon (HCC) layer and carbon nanotubes (CNTs) reinforced aluminum foam (AF) composites were prepared by the combination process of dopamine annealing and plasma enhanced in-situ growth. The hybrid carbon reinforcements establish two high-speed thermal conduction paths on the surface of the aluminum skeleton, enhancing the skeleton axial transport efficiency. The calculation results of non-equilibrium molecular dynamics (NEMD) reveal that the utilization of an optimal thickness of HCC layers can effectively strengthen the axial thermal conduction flux of the skeletons while minimizing the detrimental impact on radial heat flow from aluminum substrate to CNTs caused by thermal resistance. The composites exhibit the effective thermal conductivity of 43.17 W·m -1 ·K -1 , which is 5.6 times higher than that of the pristine AF. The instantaneous cooling rate of 16.1 K·s -1 and the cooling efficiency of 34.6% demonstrate the superior heat dissipation performance of the composites compared to other similar carbon phase reinforcing heat sinks. Therefore, the composites prepared in this work holds promising potential for heat removal applications.","PeriodicalId":237990,"journal":{"name":"Transactions of the Materials Research Society of Japan","volume":"1 3","pages":"100038-100038"},"PeriodicalIF":0.0,"publicationDate":"2025-03-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147886043","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 4
Highly stretchable strain sensors using conductive MoS2 composited PVA-PAA-Li+ hydrogels for information interaction 使用导电二硫化钼复合PVA-PAA-Li+水凝胶进行信息交互的高拉伸应变传感器
Transactions of the Materials Research Society of Japan Pub Date : 2025-03-01 DOI: 10.1016/j.tramat.2025.100041
Zhixiang Zhang, Jianhua Zhou, Xiaoling Ke, Lili Zhao, Xiaojiang Mu, Yulian Chen, Lida Jia, Fengmei He, Jie Gao, Jing Liu, Junliang Chen, Xiaoyang Wang, Lei Miao, Libo Yuan
{"title":"Highly stretchable strain sensors using conductive MoS2 composited PVA-PAA-Li+ hydrogels for information interaction","authors":"Zhixiang Zhang, Jianhua Zhou, Xiaoling Ke, Lili Zhao, Xiaojiang Mu, Yulian Chen, Lida Jia, Fengmei He, Jie Gao, Jing Liu, Junliang Chen, Xiaoyang Wang, Lei Miao, Libo Yuan","doi":"10.1016/j.tramat.2025.100041","DOIUrl":"https://doi.org/10.1016/j.tramat.2025.100041","url":null,"abstract":"Wearable sensors using conductive hydrogels have been widely used in advanced technologies such as artificial intelligence, information interaction, and medical monitoring. However, it remains a major challenge to strike a balance between mechanical properties and electrical conductivity. In this work, we propose and demonstrate a conductivity-enhanced strain sensor with molybdenum disulfide (MoS 2 ) compounded as a conductive filler in the hydrogel matrix. MoS 2 not only facilitates the molding of the dual-networked poly(vinyl alcohol) and poly(acrylic acid) but also provides a physical cross-linking point for the hydrogel matrix, which improves the mechanical properties of the hydrogel with tensile strains up to 780%. Upon further immersion in lithium chloride (LiCl) solution, the conductivity of the hydrogel sensors was significantly improved up to 3.88 S m -1 because the intercalation of Li + into MoS 2 induces the synergistic effect of ionic and electronic conductivity. The inherent -OH and -COOH groups in the network made the hydrogels also self-adhesive. This study provides a new approach for the development of advanced information-interaction devices, with potential applications extending to next-generation wearable electronics and responsive sensor technologies.","PeriodicalId":237990,"journal":{"name":"Transactions of the Materials Research Society of Japan","volume":"1 3","pages":"100041-100041"},"PeriodicalIF":0.0,"publicationDate":"2025-03-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147884232","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 1
Co pre-intercalated Layered K0.27MnO2·0.54H2O as high capacity cathode for aqueous zinc ion batteries Co预插层状K0.27MnO2·0.54H2O作为高容量锌离子电池正极
Transactions of the Materials Research Society of Japan Pub Date : 2025-02-01 DOI: 10.1016/j.tramat.2025.100031
Congfen Zhang, Wenjie Ma, Weitang Yao
{"title":"Co pre-intercalated Layered K0.27MnO2·0.54H2O as high capacity cathode for aqueous zinc ion batteries","authors":"Congfen Zhang, Wenjie Ma, Weitang Yao","doi":"10.1016/j.tramat.2025.100031","DOIUrl":"https://doi.org/10.1016/j.tramat.2025.100031","url":null,"abstract":"Aqueous zinc ion batteries (ZIBs) have attracted many scholars' attention due to its environmental benignity and high safety. Manganese dioxide, as one of the cathode materials of high-performance ZIBs, has high theoretical capacity and safety. However, due to the disproportionation reaction of Mn 3+ , the structure collapse caused by the dissolution of Mn 2+ has become the main problem of manganese-based materials. We dope Co 2+ into K 0.27 MnO 2 ⋅0.54H 2 O (Co-KMnO). The doped Co introduces more crystal water, which supports the layered structure of materials and makes it have excellent long cycle performance. It can reach a specific capacity of 192.5 mAh g −1 at 1 ​A ​g −1 and good stability with 158.3 mAh g −1 even after 800 cycles.","PeriodicalId":237990,"journal":{"name":"Transactions of the Materials Research Society of Japan","volume":"1 2","pages":"100031-100031"},"PeriodicalIF":0.0,"publicationDate":"2025-02-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147891923","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 2
Nickel carrier transfer bridge for improved photocatalytic water splitting of Zn2GeO4 改进Zn2GeO4光催化水裂解的镍载体转移桥
Transactions of the Materials Research Society of Japan Pub Date : 2025-01-01 DOI: 10.1016/j.tramat.2025.100006
Ruiqing Zou, Sibi Liu, Jie Su, Wei Ding, Y. Wang, Fei Yan, Peng Guo, Junchao Zhou, Youzi Zhang, Xuanhua Li
{"title":"Nickel carrier transfer bridge for improved photocatalytic water splitting of Zn2GeO4","authors":"Ruiqing Zou, Sibi Liu, Jie Su, Wei Ding, Y. Wang, Fei Yan, Peng Guo, Junchao Zhou, Youzi Zhang, Xuanhua Li","doi":"10.1016/j.tramat.2025.100006","DOIUrl":"https://doi.org/10.1016/j.tramat.2025.100006","url":null,"abstract":"Photocatalytic water splitting can convert solar energy into hydrogen, which has important implications for reducing dependence on fossil fuels. Constructing heterojunctions is a universal method for facilitating charge transfer, but the poor interface matching limits its charge separation and photocatalytic activity. Here, a metal-nickel bridging (nickel interlayer) NiO-Ni-Zn 2 GeO 4 photocatalyst with well interface matching is designed through a partial oxidation strategy. Structure and in situ Raman characterization demonstrate that the nickel interlayer substantially optimizes interface matching and causes the first-order phonon mode transfer from the first-order longitudinal wave to the first-order transverse wave, which implies that NiO acts as the site for hydrogen production and violent surface reaction. Therefore, the nickel interlayer provides a charge transfer channel for carrier separation. Meanwhile, density functional theory calculations prove an optimal hydrogen-oxygen bond-breaking process with 36 ​% barriers decrease obtained via the effect of nickel interlayer. As a result, NiO-Ni-Zn 2 GeO 4 shows the photocatalytic hydrogen production rate of 206.6 ​μmol ​g −1 ​h −1 , which is over 8 times greater than that of Zn 2 GeO 4 . This study offers a new approach for designing heterojunctions with well-matched interface and efficient charge separation.","PeriodicalId":237990,"journal":{"name":"Transactions of the Materials Research Society of Japan","volume":"1 1","pages":"100006-100006"},"PeriodicalIF":0.0,"publicationDate":"2025-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147333605","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Developing graphene oxide@In-Bi alloy composite via layer-by-layer strategy achieving efficient heat dissipation towards thermal interfacial applications 通过逐层策略开发石墨烯oxide@In-Bi合金复合材料,实现热界面应用的高效散热
Transactions of the Materials Research Society of Japan Pub Date : 2025-01-01 DOI: 10.1016/j.tramat.2025.100010
Yifan Li, Junhui Fan, Changqing Liu, Dahai Zhu, Chen Jiang, Wei Yu
{"title":"Developing graphene oxide@In-Bi alloy composite via layer-by-layer strategy achieving efficient heat dissipation towards thermal interfacial applications","authors":"Yifan Li, Junhui Fan, Changqing Liu, Dahai Zhu, Chen Jiang, Wei Yu","doi":"10.1016/j.tramat.2025.100010","DOIUrl":"https://doi.org/10.1016/j.tramat.2025.100010","url":null,"abstract":"We develop a graphene oxide (GO)@In-Bi alloy composite that exhibits flexibility, leak-proof properties, and efficient interfacial heat transfer. This composite was fabricated using a layer-by-layer strategy for applications in thermal interface materials (TIMs). The incorporation of liquid metal with high thermal conductivity enhances the cross-plane thermal conductivity of the GO film to 1.35 ​W/(m · K) while reducing the thermal contact resistance to 0.47 ​°C ​cm 2 /W. Upon exposure to high-temperature conditions, the In-Bi phase transition occurs, filling the gaps between rough interfaces and facilitating interface wetting, thereby improving heat transfer efficiency. Additionally, due to surface tension effects, the liquid alloy evenly coats the GO surface, providing the composite film with robust mechanical properties and ensuring excellent leak resistance. Overall, this study presents a novel approach for fabricating flexible liquid alloy-based composites with high thermal conductivity and low thermal contact resistance, providing fresh perspectives on the synthesis of TIMs.","PeriodicalId":237990,"journal":{"name":"Transactions of the Materials Research Society of Japan","volume":"1 1","pages":"100010-100010"},"PeriodicalIF":0.0,"publicationDate":"2025-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147896204","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 2
Grain boundary segregation mediated highly stable and high performance nanostructured MgAgSb bulk thermoelectric materials 晶界偏析介导的高稳定高性能纳米MgAgSb块体热电材料
Transactions of the Materials Research Society of Japan Pub Date : 2025-01-01 DOI: 10.1016/j.tramat.2025.100016
Lei Jiao, Liangjun Xie, Yuke Zhu, Lankun Wang, Yuxin Sun, Yuan Yu, A.B. Ivanova, Vladimir Khovaylo, Fengkai Guo, Wei Cai, Jiehe Sui, Zihang Liu
{"title":"Grain boundary segregation mediated highly stable and high performance nanostructured MgAgSb bulk thermoelectric materials","authors":"Lei Jiao, Liangjun Xie, Yuke Zhu, Lankun Wang, Yuxin Sun, Yuan Yu, A.B. Ivanova, Vladimir Khovaylo, Fengkai Guo, Wei Cai, Jiehe Sui, Zihang Liu","doi":"10.1016/j.tramat.2025.100016","DOIUrl":"https://doi.org/10.1016/j.tramat.2025.100016","url":null,"abstract":"","PeriodicalId":237990,"journal":{"name":"Transactions of the Materials Research Society of Japan","volume":"1 1","pages":"100016-100016"},"PeriodicalIF":0.0,"publicationDate":"2025-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147920065","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 4
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