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Approach for the Low Carbon Footprint of Biodegradable Plastic PBAT: Complete Recovery of Its Every Monomer via High-Efficiency Hydrolysis and Separation 生物可降解塑料PBAT的低碳足迹途径:通过高效水解和分离完全回收其所有单体
ACS Sustainable Chemistry & Engineering Pub Date : 2023-01-24 DOI: 10.1021/acssuschemeng.2c07413
Chengfeng Shen, Xue Zhao, Yuwei Long, Wenli An, Xuelian Zhou, Xuehui Liu, Shimei Xu, Yu-zhong Wang
{"title":"Approach for the Low Carbon Footprint of Biodegradable Plastic PBAT: Complete Recovery of Its Every Monomer via High-Efficiency Hydrolysis and Separation","authors":"Chengfeng Shen, Xue Zhao, Yuwei Long, Wenli An, Xuelian Zhou, Xuehui Liu, Shimei Xu, Yu-zhong Wang","doi":"10.1021/acssuschemeng.2c07413","DOIUrl":"https://doi.org/10.1021/acssuschemeng.2c07413","url":null,"abstract":"","PeriodicalId":131518,"journal":{"name":"ACS Sustainable Chemistry & Engineering","volume":"98 ","pages":"0"},"PeriodicalIF":0.0,"publicationDate":"2023-01-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"117432929","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 3
High-Index Surface Structure Engineering of Au–Pd Concave Triple-Octahedrons for Boosting Electrocatalytic Nitrate Reduction to Ammonia Au-Pd凹三八面体促进电催化硝酸还原制氨的高指数表面结构工程
ACS Sustainable Chemistry & Engineering Pub Date : 2023-01-24 DOI: 10.1021/acssuschemeng.2c07101
Feng Liu, Cheng Chen, Xin Jiang, Jiabao Guo, Yongsheng Wei, Jianwei Li, Tian Sheng, Xinsheng Zhao, Lu Wei
{"title":"High-Index Surface Structure Engineering of Au–Pd Concave Triple-Octahedrons for Boosting Electrocatalytic Nitrate Reduction to Ammonia","authors":"Feng Liu, Cheng Chen, Xin Jiang, Jiabao Guo, Yongsheng Wei, Jianwei Li, Tian Sheng, Xinsheng Zhao, Lu Wei","doi":"10.1021/acssuschemeng.2c07101","DOIUrl":"https://doi.org/10.1021/acssuschemeng.2c07101","url":null,"abstract":"","PeriodicalId":131518,"journal":{"name":"ACS Sustainable Chemistry & Engineering","volume":"31 1","pages":"0"},"PeriodicalIF":0.0,"publicationDate":"2023-01-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"117972229","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 3
Solvent Fractionation and Depolymerization Provide Liquid Lignin Fractions Exploited as Bio-based Aromatic Building Blocks in Epoxies 溶剂分馏和解聚提供液态木质素馏分作为生物基芳香族环氧树脂的构建单元
ACS Sustainable Chemistry & Engineering Pub Date : 2023-01-19 DOI: 10.1021/acssuschemeng.2c06668
Harald Silau, A. Melas, K. Dam‐Johansen, Hao Wu, A. Daugaard, M. Høj
{"title":"Solvent Fractionation and Depolymerization Provide Liquid Lignin Fractions Exploited as Bio-based Aromatic Building Blocks in Epoxies","authors":"Harald Silau, A. Melas, K. Dam‐Johansen, Hao Wu, A. Daugaard, M. Høj","doi":"10.1021/acssuschemeng.2c06668","DOIUrl":"https://doi.org/10.1021/acssuschemeng.2c06668","url":null,"abstract":"","PeriodicalId":131518,"journal":{"name":"ACS Sustainable Chemistry & Engineering","volume":"177 39","pages":"0"},"PeriodicalIF":0.0,"publicationDate":"2023-01-19","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"117436510","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 1
Amphiphilic Co-Solvents Modulate the Structure of Membrane Domains 两亲性共溶剂调节膜结构域
ACS Sustainable Chemistry & Engineering Pub Date : 2023-01-18 DOI: 10.1021/acssuschemeng.2c06876
Luoxi Tan, H. L. Scott, M. Smith, S. Pingali, H. O’Neill, J. Morrell-Falvey, J. Katsaras, Jeremy C. Smith, B. Davison, J. Elkins, J. Nickels
{"title":"Amphiphilic Co-Solvents Modulate the Structure of Membrane Domains","authors":"Luoxi Tan, H. L. Scott, M. Smith, S. Pingali, H. O’Neill, J. Morrell-Falvey, J. Katsaras, Jeremy C. Smith, B. Davison, J. Elkins, J. Nickels","doi":"10.1021/acssuschemeng.2c06876","DOIUrl":"https://doi.org/10.1021/acssuschemeng.2c06876","url":null,"abstract":"","PeriodicalId":131518,"journal":{"name":"ACS Sustainable Chemistry & Engineering","volume":"70 1","pages":"0"},"PeriodicalIF":0.0,"publicationDate":"2023-01-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"117615476","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Multilayer Engineering of an Escherichia coli-Based Biotransformation System to Exclusively Produce Glycolic Acid from Formaldehyde 以大肠杆菌为基础的甲醛合成乙醇酸生物转化体系的多层工程研究
ACS Sustainable Chemistry & Engineering Pub Date : 2023-01-11 DOI: 10.1021/acssuschemeng.2c05936
H. Jo, Hanna Yu, Huijin Cheon, Jun-Hong Kim, G. Kim, Byoung Sik Kim, Jeong-Sun Kim, Jin‐Byung Park
{"title":"Multilayer Engineering of an Escherichia coli-Based Biotransformation System to Exclusively Produce Glycolic Acid from Formaldehyde","authors":"H. Jo, Hanna Yu, Huijin Cheon, Jun-Hong Kim, G. Kim, Byoung Sik Kim, Jeong-Sun Kim, Jin‐Byung Park","doi":"10.1021/acssuschemeng.2c05936","DOIUrl":"https://doi.org/10.1021/acssuschemeng.2c05936","url":null,"abstract":"","PeriodicalId":131518,"journal":{"name":"ACS Sustainable Chemistry & Engineering","volume":"164 1","pages":"0"},"PeriodicalIF":0.0,"publicationDate":"2023-01-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"119753894","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 4
Emergent Chemical Behavior in Mixed Food and Lignocellulosic Green Waste Hydrothermal Liquefaction 混合食品和木质纤维素绿色废弃物水热液化中的紧急化学行为
ACS Sustainable Chemistry & Engineering Pub Date : 2022-12-23 DOI: 10.1021/acssuschemeng.2c06266
Heather O. LeClerc, Jeffrey R. Page, G. Tompsett, Sydney F. Niles, A. McKenna, J. Valla, M. Timko, Andrew R. Teixeira
{"title":"Emergent Chemical Behavior in Mixed Food and Lignocellulosic Green Waste Hydrothermal Liquefaction","authors":"Heather O. LeClerc, Jeffrey R. Page, G. Tompsett, Sydney F. Niles, A. McKenna, J. Valla, M. Timko, Andrew R. Teixeira","doi":"10.1021/acssuschemeng.2c06266","DOIUrl":"https://doi.org/10.1021/acssuschemeng.2c06266","url":null,"abstract":"GC-MS Methodology. Gas chromatography mass spectrometry was performed using an Agilent 6890N gas chromatogram equipped with an Agilent 5973N mass spectrometer. Samples were diluted 1:100 in acetone before injection of 0.5µL at a 25:1 split ratio with constant flow of helium carrier gas. Inlet temperature was set to 270 °C. The oven was initially heated to 40 °C and utilized a ramp of 10 °C/min to a temperature of 170 °C before reducing the ramp rate to 3 °C until a final temperature of 270 °C was reached. The column utilized was an HP-5. (+) APPI FT-ICR MS Methodology. Biocrude (and aqueous) samples were diluted in (50/50, by volume) toluene/tetrahydrofuran (THF) to a concentration of 125 µg/mL for analysis by positive-ion (+) atmospheric pressure photoionization (APPI) Fourier transform ion cyclotron resonance mass spectrometry (FT-ICR MS) at 21 tesla. Toluene and THF increased the ionization efficiency of nonpolar aromatic compounds 1, 2 through charge exchange, 3, 4 and proton transfer 5 reactions between ionized toluene molecules and neutral analyte molecules. An atmospheric pressure photoionization (APPI) source (Thermo-Fisher Scientific, San Jose, CA) was coupled to the first stage","PeriodicalId":131518,"journal":{"name":"ACS Sustainable Chemistry & Engineering","volume":"237 1","pages":"0"},"PeriodicalIF":0.0,"publicationDate":"2022-12-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"118071361","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 1
Eco-Friendly Production of Hyper-Cross-Linked Polymers Using Mechanosynthesis and Bioresources: A Critical Review 利用机械合成和生物资源生产超交联聚合物的生态友好型研究进展
ACS Sustainable Chemistry & Engineering Pub Date : 2022-12-02 DOI: 10.1021/acssuschemeng.2c04954
A. M. Borrero-López, A. Celzard, V. Fierro
{"title":"Eco-Friendly Production of Hyper-Cross-Linked Polymers Using Mechanosynthesis and Bioresources: A Critical Review","authors":"A. M. Borrero-López, A. Celzard, V. Fierro","doi":"10.1021/acssuschemeng.2c04954","DOIUrl":"https://doi.org/10.1021/acssuschemeng.2c04954","url":null,"abstract":"","PeriodicalId":131518,"journal":{"name":"ACS Sustainable Chemistry & Engineering","volume":"54 1","pages":"0"},"PeriodicalIF":0.0,"publicationDate":"2022-12-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"119566966","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 2
A Simple, Low-Cost, and Green Method for Preparing Strong, Tough, and Ductile Poly(lactic acid) Materials with Good Transparency and Heat Resistance 一种简单、低成本、绿色的制备透明、耐热、强韧、延展性好的聚乳酸材料的方法
ACS Sustainable Chemistry & Engineering Pub Date : 2022-11-30 DOI: 10.1021/acssuschemeng.2c05613
Tairong Kuang, Jingbing Zhang, F. Chen, Yanpei Fei, Hongfu Zhou, Yunxuan Weng, Tong Liu, Jintao Yang, Mingqiang Zhong
{"title":"A Simple, Low-Cost, and Green Method for Preparing Strong, Tough, and Ductile Poly(lactic acid) Materials with Good Transparency and Heat Resistance","authors":"Tairong Kuang, Jingbing Zhang, F. Chen, Yanpei Fei, Hongfu Zhou, Yunxuan Weng, Tong Liu, Jintao Yang, Mingqiang Zhong","doi":"10.1021/acssuschemeng.2c05613","DOIUrl":"https://doi.org/10.1021/acssuschemeng.2c05613","url":null,"abstract":"","PeriodicalId":131518,"journal":{"name":"ACS Sustainable Chemistry & Engineering","volume":"64 2 1","pages":"0"},"PeriodicalIF":0.0,"publicationDate":"2022-11-30","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"119466849","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 7
Superhydrophobic Poplar Scrimber Via In Situ Synthesis of Cu7Cl4(OH)10·H2O Heterostructure Inspired by Pine Cone with Superultraviolet Resistance 受松果启发原位合成Cu7Cl4(OH)10·H2O异质结构的超疏水杨树纤维
ACS Sustainable Chemistry & Engineering Pub Date : 2022-11-29 DOI: 10.1021/acssuschemeng.2c04327
Haiqiu Jiang, Lingling Wang, Qian Liu, Q. Lu, R. Cheng, Keming Zhan, Hui Wan, Long Yang, G. Du, Wei Gao
{"title":"Superhydrophobic Poplar Scrimber Via In Situ Synthesis of Cu7Cl4(OH)10·H2O Heterostructure Inspired by Pine Cone with Superultraviolet Resistance","authors":"Haiqiu Jiang, Lingling Wang, Qian Liu, Q. Lu, R. Cheng, Keming Zhan, Hui Wan, Long Yang, G. Du, Wei Gao","doi":"10.1021/acssuschemeng.2c04327","DOIUrl":"https://doi.org/10.1021/acssuschemeng.2c04327","url":null,"abstract":"","PeriodicalId":131518,"journal":{"name":"ACS Sustainable Chemistry & Engineering","volume":"7 1","pages":"0"},"PeriodicalIF":0.0,"publicationDate":"2022-11-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"120631993","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 2
Bioinspired Enzymatic Mineralization Incorporates CaCO3 Mesocrystals in Wood for Surface Reinforcement and Flame-Retardancy 生物启发酶矿化结合CaCO3介晶在木材表面加固和阻燃
ACS Sustainable Chemistry & Engineering Pub Date : 2022-11-23 DOI: 10.1021/acssuschemeng.2c05094
Tian Fei, H. Yi, R. Zboray, Xiao-Qiang Yan, Si-Si Song, Lei Ren, Huizhang Guo, Yuanyan Jiang
{"title":"Bioinspired Enzymatic Mineralization Incorporates CaCO3 Mesocrystals in Wood for Surface Reinforcement and Flame-Retardancy","authors":"Tian Fei, H. Yi, R. Zboray, Xiao-Qiang Yan, Si-Si Song, Lei Ren, Huizhang Guo, Yuanyan Jiang","doi":"10.1021/acssuschemeng.2c05094","DOIUrl":"https://doi.org/10.1021/acssuschemeng.2c05094","url":null,"abstract":"","PeriodicalId":131518,"journal":{"name":"ACS Sustainable Chemistry & Engineering","volume":"17 1","pages":"0"},"PeriodicalIF":0.0,"publicationDate":"2022-11-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"119965551","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 5
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