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Eco-Friendly Bionic Flexible Multifunctional Sensors Based on Biomass–MXene Composites 基于生物质- mxene复合材料的环保仿生柔性多功能传感器
ACS Sustainable Chemistry & Engineering Pub Date : 2023-04-06 DOI: 10.1021/acssuschemeng.2c04712
Chi Zheng, D. Gao, Bin Lyu, Yingying Zhou, Ailin Zhang, Y. Gu, Jianzhong Ma, Davida Briana DuBois, Shaowei Chen
{"title":"Eco-Friendly Bionic Flexible Multifunctional Sensors Based on Biomass–MXene Composites","authors":"Chi Zheng, D. Gao, Bin Lyu, Yingying Zhou, Ailin Zhang, Y. Gu, Jianzhong Ma, Davida Briana DuBois, Shaowei Chen","doi":"10.1021/acssuschemeng.2c04712","DOIUrl":"https://doi.org/10.1021/acssuschemeng.2c04712","url":null,"abstract":": Flexible sensors with multifunctions have attracted great attention for their extensive application values. Most of the reported multifunctional flexible sensors lack the intuitive signal display function, have limitations of work environment, and are weakly resistant to electromagnetic waves, and the landfill and incineration of the sensor wastes could pose irreversible damage to the environment. Herein, a trilayer composite (referred to as TGM) is prepared by the layer-by-layer assembly of MXene, gelatin, and a water-based multiporous membrane (WMM), which exhibits a hierarchically ordered bionic heterostructure. The top layer is multilayers of MXene nanosheets, the middle layer consists of artificial neural cages and synapses from an MXene@gelatin structure, and the bottom layer is a brick-mortar mimic of MXene@WMM. The resulting TGM heterostructure displays excellent performance in pressure sensing both in air and under water due to the ready variation of the electrical conductivity with applied pressures. The TGM composite also shows an apparent actuation response under IR, moisture, and heating stimulations. These multifunctional characteristics can be integrated for visual sensing of environmental temperature and humidity. Additionally, the composite possesses efficient electromagnetic shielding and shows great degradation. Results from this study highlight the unique potential of MXene − biomass composites in the development of eco-friendly multifunctional sensors.","PeriodicalId":131518,"journal":{"name":"ACS Sustainable Chemistry & Engineering","volume":"47 1","pages":"0"},"PeriodicalIF":0.0,"publicationDate":"2023-04-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"119006022","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 1
Performance Enhancement of Asphalt Mixtures Enabled by Bamboo Fibers and Acrylated Epoxidized Soybean Oil 竹纤维与丙烯酸环氧大豆油对沥青混合料性能的增强研究
ACS Sustainable Chemistry & Engineering Pub Date : 2023-04-05 DOI: 10.1021/acssuschemeng.2c06764
{"title":"Performance Enhancement of Asphalt Mixtures Enabled by Bamboo Fibers and Acrylated Epoxidized Soybean Oil","authors":"","doi":"10.1021/acssuschemeng.2c06764","DOIUrl":"https://doi.org/10.1021/acssuschemeng.2c06764","url":null,"abstract":"","PeriodicalId":131518,"journal":{"name":"ACS Sustainable Chemistry & Engineering","volume":"38 1","pages":"0"},"PeriodicalIF":0.0,"publicationDate":"2023-04-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"118398933","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 2
At-Field and On-Demand Nitrogenous Fertilizer Synthesis 现场和按需氮肥合成
ACS Sustainable Chemistry & Engineering Pub Date : 2023-04-03 DOI: 10.1021/acssuschemeng.2c06551
C. Butler, Yingzheng Fan, Saachi Grewal, Lea R. Winter
{"title":"At-Field and On-Demand Nitrogenous Fertilizer Synthesis","authors":"C. Butler, Yingzheng Fan, Saachi Grewal, Lea R. Winter","doi":"10.1021/acssuschemeng.2c06551","DOIUrl":"https://doi.org/10.1021/acssuschemeng.2c06551","url":null,"abstract":"","PeriodicalId":131518,"journal":{"name":"ACS Sustainable Chemistry & Engineering","volume":"123 1","pages":"0"},"PeriodicalIF":0.0,"publicationDate":"2023-04-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"119463297","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 1
Upcycling of Titanium by Molten Salt Electrorefining 熔盐电精炼钛的升级回收
ACS Sustainable Chemistry & Engineering Pub Date : 2023-03-31 DOI: 10.1021/acssuschemeng.3c00645
Handong Jiao, Mengjun Liu, Zhe Wang, Manpeng Lin, Z. Qu, Jianxun Song, S. Jiao
{"title":"Upcycling of Titanium by Molten Salt Electrorefining","authors":"Handong Jiao, Mengjun Liu, Zhe Wang, Manpeng Lin, Z. Qu, Jianxun Song, S. Jiao","doi":"10.1021/acssuschemeng.3c00645","DOIUrl":"https://doi.org/10.1021/acssuschemeng.3c00645","url":null,"abstract":"","PeriodicalId":131518,"journal":{"name":"ACS Sustainable Chemistry & Engineering","volume":"271 1","pages":"0"},"PeriodicalIF":0.0,"publicationDate":"2023-03-31","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"119688344","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 2
Prospective Life Cycle Assessment Bridging Biochemical, Thermochemical, and Electrochemical CO2 Reduction toward Sustainable Ethanol Synthesis 生物化学，热化学和电化学二氧化碳还原，可持续乙醇合成的前瞻性生命周期评估
ACS Sustainable Chemistry & Engineering Pub Date : 2023-03-30 DOI: 10.1021/acssuschemeng.3c00842
Wuwei Mo, Xin-Quan Tan, Wee‐Jun Ong
{"title":"Prospective Life Cycle Assessment Bridging Biochemical, Thermochemical, and Electrochemical CO2 Reduction toward Sustainable Ethanol Synthesis","authors":"Wuwei Mo, Xin-Quan Tan, Wee‐Jun Ong","doi":"10.1021/acssuschemeng.3c00842","DOIUrl":"https://doi.org/10.1021/acssuschemeng.3c00842","url":null,"abstract":"","PeriodicalId":131518,"journal":{"name":"ACS Sustainable Chemistry & Engineering","volume":"9 1","pages":"0"},"PeriodicalIF":0.0,"publicationDate":"2023-03-30","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"120446299","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 4
Oxidative Degradation Mechanism and Antidegradation Strategy of Paper-Based Relics with Transition Metal Pigments: From the Cellobiose Model to Cellulose Paper 过渡金属颜料对纸基遗迹的氧化降解机理及抗降解策略:从纤维素二糖模型到纤维素纸
ACS Sustainable Chemistry & Engineering Pub Date : 2023-03-29 DOI: 10.1021/acssuschemeng.2c04248
Yueer Yan, Jingjing Yao, Wenjuan Xu, Shutong Jin, Yahong Zhang, Yi Tang
{"title":"Oxidative Degradation Mechanism and Antidegradation Strategy of Paper-Based Relics with Transition Metal Pigments: From the Cellobiose Model to Cellulose Paper","authors":"Yueer Yan, Jingjing Yao, Wenjuan Xu, Shutong Jin, Yahong Zhang, Yi Tang","doi":"10.1021/acssuschemeng.2c04248","DOIUrl":"https://doi.org/10.1021/acssuschemeng.2c04248","url":null,"abstract":"","PeriodicalId":131518,"journal":{"name":"ACS Sustainable Chemistry & Engineering","volume":"89 1","pages":"0"},"PeriodicalIF":0.0,"publicationDate":"2023-03-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"120763603","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Enhanced Interstitial Oxygen-Enabled Efficient CuAl(M)O2 Hole Extractors for Air-Stable All-Inorganic Perovskite Solar Cells 用于空气稳定型全无机钙钛矿太阳能电池的增强型间隙氧激活高效CuAl(M)O2孔提取器
ACS Sustainable Chemistry & Engineering Pub Date : 2023-03-27 DOI: 10.1021/acssuschemeng.3c00149
Fanliang Bao, Haojie Sui, Zekun Gong, Yujing Jiao, Haiyan Chen, Yanyan Duan, Peizhi Yang, Q. Tang, B. He
{"title":"Enhanced Interstitial Oxygen-Enabled Efficient CuAl(M)O2 Hole Extractors for Air-Stable All-Inorganic Perovskite Solar Cells","authors":"Fanliang Bao, Haojie Sui, Zekun Gong, Yujing Jiao, Haiyan Chen, Yanyan Duan, Peizhi Yang, Q. Tang, B. He","doi":"10.1021/acssuschemeng.3c00149","DOIUrl":"https://doi.org/10.1021/acssuschemeng.3c00149","url":null,"abstract":"","PeriodicalId":131518,"journal":{"name":"ACS Sustainable Chemistry & Engineering","volume":"12 1","pages":"0"},"PeriodicalIF":0.0,"publicationDate":"2023-03-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"119045161","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 3
Sphere-like PdNi Alloy: Unveiling the Twin Functional Properties toward Oxygen Reduction and Temperature-Dependent Methanol Oxidation for Alkaline Direct Methanol Fuel Cells 球形PdNi合金:揭示用于碱性直接甲醇燃料电池的氧还原和温度依赖甲醇氧化的双功能特性
ACS Sustainable Chemistry & Engineering Pub Date : 2023-03-27 DOI: 10.1021/acssuschemeng.2c05220
Arunprasath Sathyaseelan, Vijayakumar Elumalai, K. Krishnamoorthy, Aparna Sajeev, Sang‐Jae Kim
{"title":"Sphere-like PdNi Alloy: Unveiling the Twin Functional Properties toward Oxygen Reduction and Temperature-Dependent Methanol Oxidation for Alkaline Direct Methanol Fuel Cells","authors":"Arunprasath Sathyaseelan, Vijayakumar Elumalai, K. Krishnamoorthy, Aparna Sajeev, Sang‐Jae Kim","doi":"10.1021/acssuschemeng.2c05220","DOIUrl":"https://doi.org/10.1021/acssuschemeng.2c05220","url":null,"abstract":"","PeriodicalId":131518,"journal":{"name":"ACS Sustainable Chemistry & Engineering","volume":"17 1","pages":"0"},"PeriodicalIF":0.0,"publicationDate":"2023-03-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"120174426","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 2
Interface Engineering of Oxygen Vacancy-Enriched Ru/RuO2–Co3O4 Heterojunction for Efficient Oxygen Evolution Reaction in Acidic Media 富氧空位- Ru/ RuO2-Co3O4异质结在酸性介质中高效析氧反应的界面工程
ACS Sustainable Chemistry & Engineering Pub Date : 2023-03-24 DOI: 10.1021/acssuschemeng.2c07322
Tiantian Wang, Zijian Li, Haeseong Jang, M. Kim, Qing Qin, Xien Liu
{"title":"Interface Engineering of Oxygen Vacancy-Enriched Ru/RuO2–Co3O4 Heterojunction for Efficient Oxygen Evolution Reaction in Acidic Media","authors":"Tiantian Wang, Zijian Li, Haeseong Jang, M. Kim, Qing Qin, Xien Liu","doi":"10.1021/acssuschemeng.2c07322","DOIUrl":"https://doi.org/10.1021/acssuschemeng.2c07322","url":null,"abstract":"","PeriodicalId":131518,"journal":{"name":"ACS Sustainable Chemistry & Engineering","volume":"21 1","pages":"0"},"PeriodicalIF":0.0,"publicationDate":"2023-03-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"120606828","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 7
Highly Selective Photocatalytic Methane Oxidation to Methanol Using CO2 as a Soft Oxidant 以CO2为软氧化剂的高选择性光催化甲烷氧化制甲醇
ACS Sustainable Chemistry & Engineering Pub Date : 2023-03-24 DOI: 10.1021/acssuschemeng.2c07355
Y. Gan, Min Huang, Fei Yu, Xingming Yu, Zhanjun He, Jin Liu, Tiejun Lin, Yuanyuan Dai, Q. Niu, Liangshu Zhong
{"title":"Highly Selective Photocatalytic Methane Oxidation to Methanol Using CO2 as a Soft Oxidant","authors":"Y. Gan, Min Huang, Fei Yu, Xingming Yu, Zhanjun He, Jin Liu, Tiejun Lin, Yuanyuan Dai, Q. Niu, Liangshu Zhong","doi":"10.1021/acssuschemeng.2c07355","DOIUrl":"https://doi.org/10.1021/acssuschemeng.2c07355","url":null,"abstract":"","PeriodicalId":131518,"journal":{"name":"ACS Sustainable Chemistry & Engineering","volume":"97 1","pages":"0"},"PeriodicalIF":0.0,"publicationDate":"2023-03-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"120118095","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 2
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