Digest Journal of Nanomaterials and Biostructures最新文献

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Sustainable generation of electricity using carbonized lignin/thermoplastic polyurethane composite films in water 利用炭化木质素/热塑性聚氨酯复合薄膜在水中可持续发电
4区 材料科学
Digest Journal of Nanomaterials and Biostructures Pub Date : 2025-05-15 DOI: 10.15251/djnb.2025.202.507
Zhipeng Zhang, Shiqing Li, Yiheng Zhou, Yu Lei, Wěi Zhāng, Junwei Sha
{"title":"Sustainable generation of electricity using carbonized lignin/thermoplastic polyurethane composite films in water","authors":"Zhipeng Zhang, Shiqing Li, Yiheng Zhou, Yu Lei, Wěi Zhāng, Junwei Sha","doi":"10.15251/djnb.2025.202.507","DOIUrl":"https://doi.org/10.15251/djnb.2025.202.507","url":null,"abstract":"Harvesting energy from water/carbon interfaces represents an eco-friendly approach to addressing the global energy crisis. Unlike conventional nanogenerators utilizing carbon nanomaterials, which typically require integration into specific systems with external pumps for liquid flow, this study presents the fabrication of a novel water-driven energy generator (WEG) utilizing composite films that integrate carbonized lignin, with varying oxygencontaining groups, and thermoplastic polyurethane in an aqueous environment. Upon optimization, the WEG demonstrates remarkable performance, achieving stable output voltage and current of 210 mV and 1.04 μA, respectively. The WEG’s output voltage demonstrated remarkable stability and reproducibility during numerous cyclic bending tests. Furthermore, by simply connecting eight WEGs in series, an elevated voltage of 1.63 V can be achieved, and these scalable units have the capability to directly power commercial electronics, such as light-emitting diodes. This energy conversion technology may provide new insights into the design of WEGs capable of harvesting water energy.","PeriodicalId":11233,"journal":{"name":"Digest Journal of Nanomaterials and Biostructures","volume":"20 2","pages":"507-518"},"PeriodicalIF":0.0,"publicationDate":"2025-05-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://doi.org/10.15251/djnb.2025.202.507","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147334078","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Simultaneously reinforce and de-color nanocellulose/lignin composite films by tuning hydroxyl groups with sodium borohydride 用硼氢化钠调节羟基,同时增强和脱色纳米纤维素/木质素复合膜
4区 材料科学
Digest Journal of Nanomaterials and Biostructures Pub Date : 2025-01-15 DOI: 10.15251/djnb.2025.201.23
, X. G. Liu, S. Y. Zeng, , Q. F. Wang, , J. Li, , X. Tong, , J. B. Chen, , D. L. Guo, , H. F. Zhao, , X. H. Chen,
{"title":"Simultaneously reinforce and de-color nanocellulose/lignin composite films by tuning hydroxyl groups with sodium borohydride","authors":", X. G. Liu, S. Y. Zeng, , Q. F. Wang, , J. Li, , X. Tong, , J. B. Chen, , D. L. Guo, , H. F. Zhao, , X. H. Chen,","doi":"10.15251/djnb.2025.201.23","DOIUrl":"https://doi.org/10.15251/djnb.2025.201.23","url":null,"abstract":"","PeriodicalId":11233,"journal":{"name":"Digest Journal of Nanomaterials and Biostructures","volume":"20 1","pages":"23-36"},"PeriodicalIF":0.0,"publicationDate":"2025-01-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147333567","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Properties regulation of carbon paper through incorporating lignin-based carbon nanofibers 木质素基纳米碳纤维对碳纸性能的调控
4区 材料科学
Digest Journal of Nanomaterials and Biostructures Pub Date : 2025-01-15 DOI: 10.15251/djnb.2025.201.1
Jicui Dai, C. H. Shen, Qianqian Tian, Xuan Liu, Shanmin Gao, Jun Li, Xin Tong
{"title":"Properties regulation of carbon paper through incorporating lignin-based carbon nanofibers","authors":"Jicui Dai, C. H. Shen, Qianqian Tian, Xuan Liu, Shanmin Gao, Jun Li, Xin Tong","doi":"10.15251/djnb.2025.201.1","DOIUrl":"https://doi.org/10.15251/djnb.2025.201.1","url":null,"abstract":"Carbon paper is commonly used as one of the electrode materials in batteries, where its main function is to serve as a conductive material, providing a channel for electron transport, and also helping to improve the conductivity and stability of the battery. Therefore, it is necessary to study how to improve the performance of carbon paper. This study aims to enhance the performance of carbon paper used in proton exchange membrane fuel cells (PEMFCs) by incorporating lignin-based carbon nanofibers (CNFs). We investigated the effects of different process flows, papermaking methods, and the addition amount of ligninbased carbon fibers on the performance of carbon paper. The research indicates that using the wet papermaking method and the process of electrospinning, impregnation and hot pressing, addition of lignin nanofibers, pre-oxidation, impregnation and hot pressing, and carbonization can yield carbon paper with the best overall performance. The tensile strength is 9.4 mPa, the flexural strength is 390 mPa, the air permeability is 1320 L/m²/s, and the resistivity is 15 mΩ/cm. This significantly improves its mechanical strength, air permeability, and electrical conductivity, making it a promising material for PEMFCs.","PeriodicalId":11233,"journal":{"name":"Digest Journal of Nanomaterials and Biostructures","volume":"20 1","pages":"1-12"},"PeriodicalIF":0.0,"publicationDate":"2025-01-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://doi.org/10.15251/djnb.2025.201.1","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147334025","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Biomineralization of Bi2S3-Gd2O3 nanocomposites: a novel approach for enhanced photothermal and MRI applications Bi2S3-Gd2O3纳米复合材料的生物矿化:增强光热和MRI应用的新方法
4区 材料科学
Digest Journal of Nanomaterials and Biostructures Pub Date : 2024-12-15 DOI: 10.15251/djnb.2024.194.1903
Qiang Lu, B. H. Zhang, Ting‐Hua Yi, Lifeng Hao, Jay L. Xue, Wubiao Duan, Yuenan Wan, D. T. Chen, Jiacheng Wang, Xuefeng Guo, Liying Zhang
{"title":"Biomineralization of Bi2S3-Gd2O3 nanocomposites: a novel approach for enhanced photothermal and MRI applications","authors":"Qiang Lu, B. H. Zhang, Ting‐Hua Yi, Lifeng Hao, Jay L. Xue, Wubiao Duan, Yuenan Wan, D. T. Chen, Jiacheng Wang, Xuefeng Guo, Liying Zhang","doi":"10.15251/djnb.2024.194.1903","DOIUrl":"https://doi.org/10.15251/djnb.2024.194.1903","url":null,"abstract":"In this study, Bi2S3-Gd2O3 nanocomposites (Bi2S3-Gd2O3@BSA) were prepared via biomineralization using albumin as a template, and the nanomaterials were directed to the tumor site through surface folic acid modification. Among these materials, Bi2S3 serves as an effective photothermal conversion agent (PTA) for photothermal therapy at tumor sites, attributed to its impressive photothermal conversion efficiency. In contrast, Gd2O3, being a paramagnetic substance, can serve effectively as a contrast agent in the magnetic resonance imaging (MRI). According to in vitro and in vivo experiments, the nanomaterials exhibit low toxicity, favorable biocompatibility, and outstanding photothermal properties. Upon the exposure to 808 nm laser irradiation, the nanomaterials quickly reach the therapeutic temperature necessary for effective tumor treatment. With folic acid modification, these nanomaterials accumulate in the tumor region, enabling efficient treatment. This strategy provides a fresh outlook for the purposeful design of diagnostic agents aimed at tumor imaging and therapy.","PeriodicalId":11233,"journal":{"name":"Digest Journal of Nanomaterials and Biostructures","volume":"19 4","pages":"1903-1920"},"PeriodicalIF":0.0,"publicationDate":"2024-12-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://doi.org/10.15251/djnb.2024.194.1903","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147918989","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Study on the surface sizing of modified chitosan and its effect on the properties of dialysis paper 改性壳聚糖表面施胶及其对透析纸性能影响的研究
4区 材料科学
Digest Journal of Nanomaterials and Biostructures Pub Date : 2024-12-15 DOI: 10.15251/djnb.2024.194.1835
Baoqin Fu, Jing‐Lin Zuo, Hai-Ming Zhao, Lizheng Sha, Junjie Li, Jianbing Chen
{"title":"Study on the surface sizing of modified chitosan and its effect on the properties of dialysis paper","authors":"Baoqin Fu, Jing‐Lin Zuo, Hai-Ming Zhao, Lizheng Sha, Junjie Li, Jianbing Chen","doi":"10.15251/djnb.2024.194.1835","DOIUrl":"https://doi.org/10.15251/djnb.2024.194.1835","url":null,"abstract":"In order to improve the paper properties and enhance the utilization efficiency of functional chemical additives, surface sizing agents were prepared by combining water-soluble maleic anhydride acylated chitosan (MAAC), carboxymethylated chitosan (O-CMCS) and polyvinyl alcohol (PVA), and the effects of sizing process on the surface morphology, physical strength and antimicrobial properties of the dialysis paper were investigated. The results showed that when the coating weight was about 6.5 g/m2 and the dosage of the modified chitosan was about 1.5% of the paper weight, the dry tensile strength, wet tensile strength and burst strength of paper sized with MAAC/PVA sizing agent increased by 46.5%, 82.2% and 107%, respectively, compared to that of unsized paper, while the dry tensile strength, wet tensile strength and burst strength of paper sized with O-CMCS/PVA sizing agent increased by 41.4%, 53.6% and 107%, respectively. In addition, the paper sized with MAAC/PVA and O-CMCS/PVA sizing agent displayed excellent antibacterial effect, which had the antibacterial rate against E. coli of 94.8% and 92.9%, respectively. In a word, the physical strength and antimicrobial properties of paper could be greatly improved by adding a small amount of modified chitosan (CS) to the surface sizing agent, and the strength improvement and antibacterial effect of MAAC/PVA sizing agent were better than that of O-CMCS/PVA.","PeriodicalId":11233,"journal":{"name":"Digest Journal of Nanomaterials and Biostructures","volume":"19 4","pages":"1835-1845"},"PeriodicalIF":0.0,"publicationDate":"2024-12-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://doi.org/10.15251/djnb.2024.194.1835","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147887484","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Fabrication of superhydrophobic coating with enhanced stability and anti-icing performance 稳定性和防冰性能增强的超疏水涂层的制备
4区 材料科学
Digest Journal of Nanomaterials and Biostructures Pub Date : 2024-12-15 DOI: 10.15251/djnb.2024.194.1855
Xinyu Fang, Jiwen Shen, Zhaozhong Feng, Zhuoqi Tang
{"title":"Fabrication of superhydrophobic coating with enhanced stability and anti-icing performance","authors":"Xinyu Fang, Jiwen Shen, Zhaozhong Feng, Zhuoqi Tang","doi":"10.15251/djnb.2024.194.1855","DOIUrl":"https://doi.org/10.15251/djnb.2024.194.1855","url":null,"abstract":"Ice accretion on outdoor equipment detrimentally affect their performance and increase the maintenance cost. Significant advancements have been made in the development of superhydrophobic coatings for anti-icing, however, the intricate manufacturing procedures and limited stability remain primary challenges that hinder their widespread use in practical application. In this context, a durable superhydrophobic coating has been fabricated using a simple spraying technique, achieving a contact angle of 166.7±1.4° and a roll-off angle of 0.6±0.2°. The coating exhibits excellent stability with contact angle maintained above 160° after undergoing various examinations. Meantime, the superhydrophobic coating possesses an enhanced anti-icing property with the time to ice formation prolonged to 42.8 min. This stable superhydrophobic coating, suitable for various outdoor uses, is hoped to contribute to the development of eco-friendly anti-icing coatings.","PeriodicalId":11233,"journal":{"name":"Digest Journal of Nanomaterials and Biostructures","volume":"19 4","pages":"1855-1863"},"PeriodicalIF":0.0,"publicationDate":"2024-12-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://doi.org/10.15251/djnb.2024.194.1855","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147892404","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 1
The effect of Pr substitution on the spectrum and photocatalytic performance of MgAl2O4 nanoparticles Pr取代对MgAl2O4纳米粒子光谱和光催化性能的影响
4区 材料科学
Digest Journal of Nanomaterials and Biostructures Pub Date : 2024-11-15 DOI: 10.15251/djnb.2024.194.1719
Zou Yu, Jiabin Zhou, Min Xu, Ya Yang, Yongya Wang
{"title":"The effect of Pr substitution on the spectrum and photocatalytic performance of MgAl2O4 nanoparticles","authors":"Zou Yu, Jiabin Zhou, Min Xu, Ya Yang, Yongya Wang","doi":"10.15251/djnb.2024.194.1719","DOIUrl":"https://doi.org/10.15251/djnb.2024.194.1719","url":null,"abstract":"To study the spectral regulation of Pr on MgAl2O4 nanoparticles, different contents of Pr doped MgAlPr ternary hydrotalcite were synthesized by co-precipitation method, and Pr containing mixed metal oxides Pr-x-y was prepared by high-temperature calcination. The Pr had little effect on the morphology of hydrotalcite, but significantly improved the heat resistance. The Pr significantly reduced the Eg values of MgAl-L and its mixed oxide ( Eg=1.68–1.87 eV). After 100 min of irradiation with visible light, the degradation rate of MB reached 87.7%. In the reaction system of Pr-0.05-500/H2O2, h+ played a major role. There was a corresponding relationship between the photocatalytic performance and L* value of mixed oxide nanoparticles based on MgAl-L and Pr-0.05-L. The NIR of hydrotalcite or Pr containing nanoparticles was greatly affected by the calcination temperature and Pr containing, but the values of NIR were more than 50%.","PeriodicalId":11233,"journal":{"name":"Digest Journal of Nanomaterials and Biostructures","volume":"19 4","pages":"1719-1735"},"PeriodicalIF":0.0,"publicationDate":"2024-11-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://doi.org/10.15251/djnb.2024.194.1719","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147904722","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Research on PbTiO3 nanoparticles optimized mesoporous layer for perovskite solar cells 纳米PbTiO3优化钙钛矿太阳能电池介孔层的研究
4区 材料科学
Digest Journal of Nanomaterials and Biostructures Pub Date : 2024-11-01 DOI: 10.15251/djnb.2024.194.1561
Yihui Zhang, Jinyun Li, Junming Li, Haiyang Tao, C. X. Zhang
{"title":"Research on PbTiO3 nanoparticles optimized mesoporous layer for perovskite solar cells","authors":"Yihui Zhang, Jinyun Li, Junming Li, Haiyang Tao, C. X. Zhang","doi":"10.15251/djnb.2024.194.1561","DOIUrl":"https://doi.org/10.15251/djnb.2024.194.1561","url":null,"abstract":"Organic-inorganic hybrid perovskite solar cells have garnered significant attention due to their facile fabrication process and high photovoltaic conversion efficiency. The electron transport layer plays a crucial role in the carrier separation mechanism of perovskite solar cells, making it a focal point for enhancing cell performance. In this study, PbTiO3 was introduced into TiO2 mesoporous layers by modification and doping in order to optimize cell performance. Initially, the use of PbTiO3-modified mesoporous layers revealed issues such as non-uniform modification layers, low film coverage rates, and reduced light transmittance. These issues hindered the ability of PbTiO3 to facilitate carrier separation and resulting in suboptimal optimization effects. However, by utilizing PbTiO3-doped mesoporous layers for optimizing cell performance, we observed improved quality and higher light transmittance in the perovskite films. As a consequence of the improved carrier separation achieved by PbTiO3, the efficiency of the solar cell has been enhanced to 5.51%.","PeriodicalId":11233,"journal":{"name":"Digest Journal of Nanomaterials and Biostructures","volume":"19 4","pages":"1561-1575"},"PeriodicalIF":0.0,"publicationDate":"2024-11-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"http://dx.doi.org/10.15251/djnb.2024.194.1561","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147908677","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
CoFe bimetallic phosphide fabricated by topological transformation strategy for efficient electrooxidation of benzyl alcohol 用拓扑转化策略制备苯甲醇高效电氧化的咖啡双金属磷化物
4区 材料科学
Digest Journal of Nanomaterials and Biostructures Pub Date : 2024-08-19 DOI: 10.15251/djnb.2024.193.1159
Junyan Liu, Heng‐Jui Liu, Yuwei Xu, Hongwei Wang, L. J. Wang
{"title":"CoFe bimetallic phosphide fabricated by topological transformation strategy for efficient electrooxidation of benzyl alcohol","authors":"Junyan Liu, Heng‐Jui Liu, Yuwei Xu, Hongwei Wang, L. J. Wang","doi":"10.15251/djnb.2024.193.1159","DOIUrl":"https://doi.org/10.15251/djnb.2024.193.1159","url":null,"abstract":"Rational design of effective non-precious metallic electrocatalysts is crucial for electrooxidation of benzyl alcohol (BA) producing benzoic acid (BAC). Herein, CoFe bimetallic phosphide (CoFeP-m) with bimetallic synergy, fully exposed active sites, and fast charge transfer was fabricated by topological transformation of CoFe-LDH for the efficient electrooxidation of BA to BAC under mild condition. Under the optimal conditions of starting voltage of 0.7 V vs. Ag/AgCl at 25oC, CoFeP-300 achieved 97.71% transformation of BA and 97.84% BAC's selectivity for 8 h. In addition, CoFeP-300 showed excellent stability which maintained 95.89% transform into BA and 95.37% BAC's selectivity at the sixth cycle.","PeriodicalId":11233,"journal":{"name":"Digest Journal of Nanomaterials and Biostructures","volume":"19 3","pages":"1159-1171"},"PeriodicalIF":0.0,"publicationDate":"2024-08-19","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"http://dx.doi.org/10.15251/djnb.2024.193.1159","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147902922","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Direct ink writing of WC-Co composite with flexible green bodies 柔性绿体WC-Co复合材料的直墨书写
4区 材料科学
Digest Journal of Nanomaterials and Biostructures Pub Date : 2024-08-05 DOI: 10.15251/djnb.2024.193.1077
N. Zhang, Ting Luo, Xiaoling Yang
{"title":"Direct ink writing of WC-Co composite with flexible green bodies","authors":"N. Zhang, Ting Luo, Xiaoling Yang","doi":"10.15251/djnb.2024.193.1077","DOIUrl":"https://doi.org/10.15251/djnb.2024.193.1077","url":null,"abstract":"Direct ink writing of 3D WC-Co with conformable green bodies was achieved benefiting from the highly flexible WC-Co paste with high solid loading. Rheology properties of the paste, microstructure of the 3D structure was investigated. Organic-based paste of WC-8Co with a high solid content of 91 wt% were prepared, which exhibited shear thinning behavior and had a high storage modulus, two key parameters for ensuring the smooth printing. After secondary molding, 3D WC-Co green bodies with overhanging structure and no cracks were confirmed through secondary treatment of twisting or bending. Sound 3D structures with uniform and dense microstructure were obtained after debinding and sintering in vacuum. This work showed a facile route for the fabrication of 3D bone cemented carbides by direct ink writing with flexible green bodies.","PeriodicalId":11233,"journal":{"name":"Digest Journal of Nanomaterials and Biostructures","volume":"19 3","pages":"1077-1085"},"PeriodicalIF":0.0,"publicationDate":"2024-08-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"http://dx.doi.org/10.15251/djnb.2024.193.1077","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147907752","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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