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Tuneable EfficientnWhite Emission of Sb3+/Mn2+ Co-Doped Lead-FreenPerovskites for Single-ComponentnWhite Light-Emitting Diodes Sb3+/Mn2+</sup&gt；共掺杂无铅钙钛矿用于单组分白光发光二极管的可调谐高效白光发射

Figshare Pub Date : 2024-04-04 DOI: 10.1021/acsami.4c00745.s001

Yuanyuan Sheng (5156153), Ping Chen (89712), Yanpeng Gao (1862740), Yong He (115255), Junchun Li (12914422), Muhammad (9038204), Xiang Xie (317801), Chen Cheng (76970), Jingting Yang (380099), Yajing Chang (1504330), Guoqing Tong (4966054), Yang Jiang (46459)

{"title":"Tuneable EfficientnWhite Emission of Sb3+/Mn2+ Co-Doped Lead-FreenPerovskites for Single-ComponentnWhite Light-Emitting Diodes","authors":"Yuanyuan Sheng (5156153), Ping Chen (89712), Yanpeng Gao (1862740), Yong He (115255), Junchun Li (12914422), Muhammad (9038204), Xiang Xie (317801), Chen Cheng (76970), Jingting Yang (380099), Yajing Chang (1504330), Guoqing Tong (4966054), Yang Jiang (46459)","doi":"10.1021/acsami.4c00745.s001","DOIUrl":"https://doi.org/10.1021/acsami.4c00745.s001","url":null,"abstract":"Inorganic lead-free perovskite nanocrystals (NCs) withnbroadbandnself-trapped exciton (STEs) emission and low toxicity have shown enormousnapplication prospects in the field of display and lighting. However,nwhite light-emitting diodes (WLEDs) based on a single-component materialnwith high photoluminescence quantum yield (PLQY) remain challenging.nHere, we demonstrate a novel codoping strategy by introducing Sb3+/Mn2+ ions to achieve the tuneable dual emissionnin lead-free perovskite Cs3InCl6 NCs. The PLQYnincreases to 59.64% after doping with Sb3+. The codopednCs3InCl6 NCs exhibit efficient white light emissionndue to the energy transfer channel from STEs to Mn2+ ionsnwith PLQY of 51.38%. Density functional theory (DFT) calculationsnhave been used to verify deeply the effects of Sb3+/Mn2+ doping. WLEDs based on Sb3+/Mn2+-codopednCs3InCl6 NCs are explored with color renderingnindex of 85.5 and color coordinate of (0.398, 0.445), which have beennsuccessfully applied as photodetector lighting sources. This worknprovides a new perspective for designing novel lead-free perovskitesnto achieve single-component WLEDs.","PeriodicalId":521516,"journal":{"name":"Figshare","volume":"1 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2024-04-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147880719","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

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