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Single-shot single-beam coherent Raman scattering thermometry based on optically induced air lasing 基于光诱导空气激光的单光束相干拉曼散射测温技术
Light-Science & Applications Pub Date : 2024-11-25 DOI: 10.1038/s41377-024-01598-9
Xu Lu, Yewei Chen, Francesco Mazza, Siyi He, Zihan Li, Shunlin Huang, Quanjun Wang, Ning Zhang, Bo Shen, Yuzhu Wu, Jinping Yao, Ya Cheng
{"title":"Single-shot single-beam coherent Raman scattering thermometry based on optically induced air lasing","authors":"Xu Lu, Yewei Chen, Francesco Mazza, Siyi He, Zihan Li, Shunlin Huang, Quanjun Wang, Ning Zhang, Bo Shen, Yuzhu Wu, Jinping Yao, Ya Cheng","doi":"10.1038/s41377-024-01598-9","DOIUrl":"https://doi.org/10.1038/s41377-024-01598-9","url":null,"abstract":"<p>Thermometric techniques with high accuracy, fast response and ease of implementation are desirable for the study of dynamic combustion environments, transient reacting flows, and non-equilibrium plasmas. Herein, single-shot single-beam coherent Raman scattering (SS-CRS) thermometry is developed, for the first time to our knowledge, by using air lasing as a probe. We show that the air-lasing-assisted CRS signal has a high signal-to-noise ratio enabling single-shot measurements at a 1 kHz repetition rate. The SS-CRS thermometry consistently exhibits precision of &lt;2.3% at different temperatures, but the inaccuracy grows with the increase in temperature. The high measurement repeatability, 1 kHz acquisition rate and easy-to-implement single-beam scheme are achieved thanks to the unique temporal, spectral and spatial characteristics of air lasing. This work opens a novel avenue for high-speed CRS thermometry, holding tremendous potential for fast diagnostics of transient reacting flows and plasmas.</p>","PeriodicalId":18069,"journal":{"name":"Light-Science & Applications","volume":"13 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2024-11-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142696882","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Simultaneous biomethane and hydrochar recovery from washed elephant dung: The effects of inoculum source, substrate to inoculum ratio, and hydrothermal temperature 从洗象粪中同时回收生物甲烷和烃类:接种物来源、底物与接种物比和热液温度的影响
IF 6.4 3区 环境科学与生态学
Carbon Resources Conversion Pub Date : 2024-11-24 DOI: 10.1016/j.crcon.2024.100297
Chayanon Sawatdeenarunat , Boonya Charnnok , Rojapun Nirunsin , Sumate Chaiprapat , Chen-Yeon Chu
{"title":"Simultaneous biomethane and hydrochar recovery from washed elephant dung: The effects of inoculum source, substrate to inoculum ratio, and hydrothermal temperature","authors":"Chayanon Sawatdeenarunat ,&nbsp;Boonya Charnnok ,&nbsp;Rojapun Nirunsin ,&nbsp;Sumate Chaiprapat ,&nbsp;Chen-Yeon Chu","doi":"10.1016/j.crcon.2024.100297","DOIUrl":"10.1016/j.crcon.2024.100297","url":null,"abstract":"<div><div>This research aims to develop the appropriate biorefinery process integrating anaerobic digestion (AD) and hydrothermal carbonization (HTC) to recover the highest energy from the pretreated elephant dung. Initially, the raw elephant dung was physically processed by washing with water to generate the liquid waste, i.e., washing water (WW), and solid waste, i.e., washed fiber (WF). The appropriate substrate-to-inoculum ratio (SIR) and the inoculum source of the AD of WW were determined and the HTC temperature of WF was also examined. The results indicated that the AD of WW with the SIR of 1:2 and anaerobically digested swine manure as the inoculum presented the highest methane and energy yields of 412.3 ± 9.9 N mL/g VS <sub>added</sub> and 2,220.1 ± 53.03 MJ/ton dry wt., respectively. For HTC of WF, the optimum condition was the hydrothermal temperature of 170 °C at the residence time of 60 min. The highest hydrochar and energy yields were 76.8 % ± 1.9 % dry wt. and 12,067.0 ± 452.1 MJ/ton dry wt., respectively. Thus, this biorefinery process could simultaneously treat elephant camp-derived waste and produce clean energy.</div></div>","PeriodicalId":52958,"journal":{"name":"Carbon Resources Conversion","volume":"8 1","pages":"Article 100297"},"PeriodicalIF":6.4,"publicationDate":"2024-11-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142744302","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Catalytic gasification of a single coal char particle: An experimental and simulation study 单一煤炭颗粒的催化气化:实验和模拟研究
IF 6.4 3区 环境科学与生态学
Carbon Resources Conversion Pub Date : 2024-11-22 DOI: 10.1016/j.crcon.2024.100296
Zhuoran Liu , Xingjun Wang , Qian Chen , Hongxia Li , Qinghua Guo , Guangsuo Yu , Haifeng Liu , Fuchen Wang
{"title":"Catalytic gasification of a single coal char particle: An experimental and simulation study","authors":"Zhuoran Liu ,&nbsp;Xingjun Wang ,&nbsp;Qian Chen ,&nbsp;Hongxia Li ,&nbsp;Qinghua Guo ,&nbsp;Guangsuo Yu ,&nbsp;Haifeng Liu ,&nbsp;Fuchen Wang","doi":"10.1016/j.crcon.2024.100296","DOIUrl":"10.1016/j.crcon.2024.100296","url":null,"abstract":"<div><div>The catalytic coal gasification technology has been widely researched and developed under the background of “Carbon peaking and carbon neutrality goals”. Currently, most of catalytic gasification experiments on coal char particles are analyzed by thermogravimetric analyzer (TGA). However, the gasification agent will be subject to diffusion resistance during the reaction because of the sample stacking, making the inherent reaction kinetics unclear. In this study, we investigated the catalytic gasification behavior of single-particle coal char using high temperature stage microscope (HTSM). With the diffusion resistance ruled out, the reaction conditions when using a HTSM are more similar to those inside a real industrial gasifier. Numerical models of the gasification reaction of single-particle coal char were further developed using the kinetic parameters obtained under HTSM. Three models were investigated, including regular spherical structured, irregular spherical structured and porous spherical structured models, representing different morphologies of coal char particles in the gasifier. The gasification characteristics of coal char particles under different K<sub>2</sub>CO<sub>3</sub> catalyst loadings and gasification temperatures were also studied. Compared with the activation energies data of coal char particles without catalyst, the activation energies of coal char particles loaded with 2.2 %, 4.4 %, 6.6 %, and 10.0 % catalysts were reduced by 110 kJ/mol, 116 kJ/mol, 121 kJ/mol, and 126 kJ/mol, respectively. The reaction surface area affects the temperature distribution. The temperature near the irregular spherical particle is about 20 K higher than the temperature near the regular spherical particle.</div></div>","PeriodicalId":52958,"journal":{"name":"Carbon Resources Conversion","volume":"8 1","pages":"Article 100296"},"PeriodicalIF":6.4,"publicationDate":"2024-11-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142699380","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Topological protection of optical skyrmions through complex media 穿过复杂介质的光学天幕的拓扑保护
Light-Science & Applications Pub Date : 2024-11-22 DOI: 10.1038/s41377-024-01659-z
An Aloysius Wang, Zimo Zhao, Yifei Ma, Yuxi Cai, Runchen Zhang, Xiaoyi Shang, Yunqi Zhang, Ji Qin, Zhi-Kai Pong, Tádé Marozsák, Binguo Chen, Honghui He, Lin Luo, Martin J. Booth, Steve J. Elston, Stephen M. Morris, Chao He
{"title":"Topological protection of optical skyrmions through complex media","authors":"An Aloysius Wang, Zimo Zhao, Yifei Ma, Yuxi Cai, Runchen Zhang, Xiaoyi Shang, Yunqi Zhang, Ji Qin, Zhi-Kai Pong, Tádé Marozsák, Binguo Chen, Honghui He, Lin Luo, Martin J. Booth, Steve J. Elston, Stephen M. Morris, Chao He","doi":"10.1038/s41377-024-01659-z","DOIUrl":"https://doi.org/10.1038/s41377-024-01659-z","url":null,"abstract":"<p>Optical Skyrmions have many important properties that make them ideal units for high-density data applications, including the ability to carry digital information through a discrete topological number and the independence of spatially varying polarization to other dimensions. More importantly, the topological nature of the optical Skyrmion heuristically suggests a strong degree of robustness to perturbations, which is crucial for reliably carrying information in noisy environments. However, the study of the topological robustness of optical Skyrmions is still in its infancy. Here, we quantify this robustness precisely by proving that the topological nature of the Skyrmion arises from its structure on the boundary and, by duality, is resilient to spatially varying perturbations provided they respect the relevant boundary conditions of the unperturbed Skyrmion. We then present experimental evidence validating this robustness in the context of paraxial Skyrmion beams against complex polarization aberrations. Our work provides a framework for handling various perturbations of Skyrmion fields and offers guarantees of robustness in a general sense. This, in turn, has implications for applications of the Skyrmion where their topological nature is exploited explicitly, and, in particular, provides an underpinning for the use of optical Skyrmions in communications and computing.</p>","PeriodicalId":18069,"journal":{"name":"Light-Science & Applications","volume":"180 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2024-11-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142684323","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
OFC: Outside Front Cover OFC:封面外侧
IF 9.1
Green Chemical Engineering Pub Date : 2024-11-21 DOI: 10.1016/S2666-9528(24)00070-0
{"title":"OFC: Outside Front Cover","authors":"","doi":"10.1016/S2666-9528(24)00070-0","DOIUrl":"10.1016/S2666-9528(24)00070-0","url":null,"abstract":"","PeriodicalId":66474,"journal":{"name":"Green Chemical Engineering","volume":"6 1","pages":"Page OFC"},"PeriodicalIF":9.1,"publicationDate":"2024-11-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142704748","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Outside Back Cover 封底外侧
IF 9.1
Green Chemical Engineering Pub Date : 2024-11-21 DOI: 10.1016/S2666-9528(24)00079-7
{"title":"Outside Back Cover","authors":"","doi":"10.1016/S2666-9528(24)00079-7","DOIUrl":"10.1016/S2666-9528(24)00079-7","url":null,"abstract":"","PeriodicalId":66474,"journal":{"name":"Green Chemical Engineering","volume":"6 1","pages":"Page OBC"},"PeriodicalIF":9.1,"publicationDate":"2024-11-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142704747","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Improved biohydrogen production from lactic acid bacteria contaminating substrates by enriched hydrogen-producing consortium with lactate-fermentation pathway 利用乳酸发酵途径的富集产氢联合体提高乳酸菌污染底物的生物制氢能力
IF 6.4 3区 环境科学与生态学
Carbon Resources Conversion Pub Date : 2024-11-17 DOI: 10.1016/j.crcon.2024.100295
Phonsini Ngamnurak , Alissara Reungsang , Pensri Plangklang
{"title":"Improved biohydrogen production from lactic acid bacteria contaminating substrates by enriched hydrogen-producing consortium with lactate-fermentation pathway","authors":"Phonsini Ngamnurak ,&nbsp;Alissara Reungsang ,&nbsp;Pensri Plangklang","doi":"10.1016/j.crcon.2024.100295","DOIUrl":"10.1016/j.crcon.2024.100295","url":null,"abstract":"<div><div>The hydrogen-producing consortium conveying the lactate-fermentation pathway was enriched and used as a co-inoculum with the non-enriched hydrogen-producing consortium for biohydrogen production in the presence of lactic acid bacteria (LAB). The co-inoculum treatment achieved superior hydrogen production performance compared to that of the non-enriched consortium treatment. The effects of enriched consortium concentration, initial pH, and glucose concentration were evaluated, and hydrogen production potential (HP) of 1,605 ± 161 mL-H<sub>2</sub>/L and a maximum hydrogen production rate (HPR) of 87.17 ± 15.85 mL-H<sub>2</sub>/L.h were achieved under optimal conditions. Biohydrogen production from food waste using the co-inoculum was 1,137 mL-H<sub>2</sub>/L from non-autoclaved food waste, corresponding to 56.85 mL-H<sub>2</sub>/g-VS<sub>added</sub>. Metabolite product and microbial community analyses during food waste fermentation indicated positive cross-feeding activity of hydrogen producers, LAB, and acetogenic bacteria. This study provides valuable information on the use of an efficient, enriched hydrogen-producing consortium to improve biohydrogen production from LAB-contaminated feedstock.</div></div>","PeriodicalId":52958,"journal":{"name":"Carbon Resources Conversion","volume":"8 1","pages":"Article 100295"},"PeriodicalIF":6.4,"publicationDate":"2024-11-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142699465","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
The brightest multi-colour phonon lasers 最亮的多色声子激光器
Light-Science & Applications Pub Date : 2024-11-13 DOI: 10.1038/s41377-024-01648-2
Mishkat Bhattacharya
{"title":"The brightest multi-colour phonon lasers","authors":"Mishkat Bhattacharya","doi":"10.1038/s41377-024-01648-2","DOIUrl":"https://doi.org/10.1038/s41377-024-01648-2","url":null,"abstract":"<p>A new device applies a single-colour electronic injection to create the brightest multi-colour phonon laser, with ten times more power and much narrower linewidth than others.</p>","PeriodicalId":18069,"journal":{"name":"Light-Science & Applications","volume":"95 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2024-11-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142601018","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Innovative CQD detector for broadband multispectral imaging 用于宽带多光谱成像的创新型 CQD 探测器
Light-Science & Applications Pub Date : 2024-11-12 DOI: 10.1038/s41377-024-01621-z
Shengli Sun, Yaran Li, Fansheng Chen
{"title":"Innovative CQD detector for broadband multispectral imaging","authors":"Shengli Sun, Yaran Li, Fansheng Chen","doi":"10.1038/s41377-024-01621-z","DOIUrl":"https://doi.org/10.1038/s41377-024-01621-z","url":null,"abstract":"<p><i>Nature Photonics</i> <b>18</b>, 1147–1154 (2024)</p>","PeriodicalId":18069,"journal":{"name":"Light-Science & Applications","volume":"18 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2024-11-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142599527","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Bessel beam optical coherence microscopy enables multiscale assessment of cerebrovascular network morphology and function 贝塞尔光束光学相干显微镜可对脑血管网络的形态和功能进行多尺度评估
Light-Science & Applications Pub Date : 2024-11-11 DOI: 10.1038/s41377-024-01649-1
Lukas Glandorf, Bastian Wittmann, Jeanne Droux, Chaim Glück, Bruno Weber, Susanne Wegener, Mohamad El Amki, Rainer Leitgeb, Bjoern Menze, Daniel Razansky
{"title":"Bessel beam optical coherence microscopy enables multiscale assessment of cerebrovascular network morphology and function","authors":"Lukas Glandorf, Bastian Wittmann, Jeanne Droux, Chaim Glück, Bruno Weber, Susanne Wegener, Mohamad El Amki, Rainer Leitgeb, Bjoern Menze, Daniel Razansky","doi":"10.1038/s41377-024-01649-1","DOIUrl":"https://doi.org/10.1038/s41377-024-01649-1","url":null,"abstract":"<p>Understanding the morphology and function of large-scale cerebrovascular networks is crucial for studying brain health and disease. However, reconciling the demands for imaging on a broad scale with the precision of high-resolution volumetric microscopy has been a persistent challenge. In this study, we introduce Bessel beam optical coherence microscopy with an extended focus to capture the full cortical vascular hierarchy in mice over 1000 × 1000 × 360 μm<sup>3</sup> field-of-view at capillary level resolution. The post-processing pipeline leverages a supervised deep learning approach for precise 3D segmentation of high-resolution angiograms, hence permitting reliable examination of microvascular structures at multiple spatial scales. Coupled with high-sensitivity Doppler optical coherence tomography, our method enables the computation of both axial and transverse blood velocity components as well as vessel-specific blood flow direction, facilitating a detailed assessment of morpho-functional characteristics across all vessel dimensions. Through graph-based analysis, we deliver insights into vascular connectivity, all the way from individual capillaries to broader network interactions, a task traditionally challenging for in vivo studies. The new imaging and analysis framework extends the frontiers of research into cerebrovascular function and neurovascular pathologies.</p>","PeriodicalId":18069,"journal":{"name":"Light-Science & Applications","volume":"70 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2024-11-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142597404","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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