ANTARES:空间分辨电子结构

IF 1.8 4区 物理与天体物理 Q2 SPECTROSCOPY
J. Avila, S. Lorcy, P. Dudin
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引用次数: 0

摘要

空间分辨ARPES (nanoARPES)是在传统ARPES技术的基础上发展起来的,通过将光聚焦到亚微米尺度的光斑上实现空间分辨。这一发展主要用于小样本的研究,例如,二维材料薄片的异质结构构建,微晶或多晶样品,不同晶体终止,电子结构域。ANTARES从2010年开始向用户社区提供nanoARPES技术,到目前为止,该仪器已用于各种类型的样品,这有助于积累具体的经验。本文报道了同步加速器SOLEIL上ANTARES仪器的现状布局和实际性能,以及最典型的应用领域。最重要的和最新的升级包括聚焦光学和操作中的设置。新的光学单元提供增加通量的样品,以及选择改变光子能量。在操作中设置提供了与纳米arpes正在研究的样品电连接的选择,这保证了各种应用,其中现在最需要的是用施加电压控制电荷载流子密度。这种“栅掺杂”通常应用于二维材料的异质结构,可以有目的地设计和构建。二维异质结构可能是该仪器最典型的应用领域,有或没有操作选项。与此同时,ANTARES仪器的使用案例仍在开发中,实现了新型样品和新型实验。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
ANTARES: Space-resolved electronic structure

The spatially resolved ARPES (nanoARPES) is a development of conventional ARPES technique achieved with the focusing of light on the sample into the spot with submicron sizes. This development is used in research of essentially small samples, for example, heterostructures build of flakes of 2D materials, micro-crystals or polycrystalline samples, different crystal termination, domains in electronic structure. ANTARES is delivering the nanoARPES technique to user community since 2010, up to now the instrument was used with samples of various types, and that was useful to accumulate the specific experience. In this paper we report the current layout and actual performance of the ANTARES instrument at Synchrotron SOLEIL, as well as the most typical application areas. The most important and recent upgrades include focusing optics and in-operando setup. The new optical units deliver the increased flux on sample as well as the option to vary the photon energy. The in-operando setup offers the option of electrical connection to the sample being studied with nanoARPES, that promises various applications, where the most demanded now is the control of charge carrier density with applied voltage. This “gate-doping” is often applied to the heterostructures of 2D materials, that could be designed and build on purpose. The 2D heterostructures is probably the most typical field of application of the instrument, with or without in-operando option. At the same time the use case of the ANTARES instrument is still in the development by the realisation of new kinds of samples and of the new types of the experiments.

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来源期刊
CiteScore
3.30
自引率
5.30%
发文量
64
审稿时长
60 days
期刊介绍: The Journal of Electron Spectroscopy and Related Phenomena publishes experimental, theoretical and applied work in the field of electron spectroscopy and electronic structure, involving techniques which use high energy photons (>10 eV) or electrons as probes or detected particles in the investigation.
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