{"title":"用于离子软着陆研究的紧凑型窄能量扩散特高压负卤素离子源。","authors":"Qiwei Chen, Xianzheng Liu, Yuchen Bai, Liluo He, Zhongyi Wu, Haoyang Deng, Xiong Zhou, Jing Liu, Kai Wu","doi":"10.1063/5.0272024","DOIUrl":null,"url":null,"abstract":"<p><p>A compact ultrahigh vacuum negative halogen ion source has been developed to generate ion beams with small energy spread for soft-landing applications. Thermionic emission of a halogen atom from a hot tantalum surface carries an extra electron to form a negative halogen ion. Based on this principle, a tantalum helical ionizer is designed to efficiently produce Cl- ions from Cl atoms generated by CuCl2 decomposition. The intrinsic kinetic energy distribution, quantified by a retarding field energy analyzer, exhibits a full width at half maximum of ∼0.83 eV. Beam profiling confirms a controllable diameter within 8 mm. Isotopes of 35Cl- and 37Cl- have been successfully resolved with a Wien filter. The compact ion source has been integrated into an ion transport study apparatus, with initial experiments verifying ion soft-landing and surface charge dynamics. This ion source provides a reliable tool for probing ion-involved interfacial processes under ultra-high vacuum conditions, while advancing ion chemistry and relating sciences as well.</p>","PeriodicalId":21111,"journal":{"name":"Review of Scientific Instruments","volume":"96 9","pages":""},"PeriodicalIF":1.7000,"publicationDate":"2025-09-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"A compact UHV negative halogen ion source with narrow energy spread for ion soft-landing study.\",\"authors\":\"Qiwei Chen, Xianzheng Liu, Yuchen Bai, Liluo He, Zhongyi Wu, Haoyang Deng, Xiong Zhou, Jing Liu, Kai Wu\",\"doi\":\"10.1063/5.0272024\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p><p>A compact ultrahigh vacuum negative halogen ion source has been developed to generate ion beams with small energy spread for soft-landing applications. Thermionic emission of a halogen atom from a hot tantalum surface carries an extra electron to form a negative halogen ion. Based on this principle, a tantalum helical ionizer is designed to efficiently produce Cl- ions from Cl atoms generated by CuCl2 decomposition. The intrinsic kinetic energy distribution, quantified by a retarding field energy analyzer, exhibits a full width at half maximum of ∼0.83 eV. Beam profiling confirms a controllable diameter within 8 mm. Isotopes of 35Cl- and 37Cl- have been successfully resolved with a Wien filter. The compact ion source has been integrated into an ion transport study apparatus, with initial experiments verifying ion soft-landing and surface charge dynamics. This ion source provides a reliable tool for probing ion-involved interfacial processes under ultra-high vacuum conditions, while advancing ion chemistry and relating sciences as well.</p>\",\"PeriodicalId\":21111,\"journal\":{\"name\":\"Review of Scientific Instruments\",\"volume\":\"96 9\",\"pages\":\"\"},\"PeriodicalIF\":1.7000,\"publicationDate\":\"2025-09-01\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Review of Scientific Instruments\",\"FirstCategoryId\":\"5\",\"ListUrlMain\":\"https://doi.org/10.1063/5.0272024\",\"RegionNum\":4,\"RegionCategory\":\"工程技术\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q3\",\"JCRName\":\"INSTRUMENTS & INSTRUMENTATION\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Review of Scientific Instruments","FirstCategoryId":"5","ListUrlMain":"https://doi.org/10.1063/5.0272024","RegionNum":4,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"INSTRUMENTS & INSTRUMENTATION","Score":null,"Total":0}
A compact UHV negative halogen ion source with narrow energy spread for ion soft-landing study.
A compact ultrahigh vacuum negative halogen ion source has been developed to generate ion beams with small energy spread for soft-landing applications. Thermionic emission of a halogen atom from a hot tantalum surface carries an extra electron to form a negative halogen ion. Based on this principle, a tantalum helical ionizer is designed to efficiently produce Cl- ions from Cl atoms generated by CuCl2 decomposition. The intrinsic kinetic energy distribution, quantified by a retarding field energy analyzer, exhibits a full width at half maximum of ∼0.83 eV. Beam profiling confirms a controllable diameter within 8 mm. Isotopes of 35Cl- and 37Cl- have been successfully resolved with a Wien filter. The compact ion source has been integrated into an ion transport study apparatus, with initial experiments verifying ion soft-landing and surface charge dynamics. This ion source provides a reliable tool for probing ion-involved interfacial processes under ultra-high vacuum conditions, while advancing ion chemistry and relating sciences as well.
期刊介绍:
Review of Scientific Instruments, is committed to the publication of advances in scientific instruments, apparatuses, and techniques. RSI seeks to meet the needs of engineers and scientists in physics, chemistry, and the life sciences.