{"title":"$$\\widehat{P}\\widehat{{T}}$$ 对称控制磁序开关","authors":"Ziyu Niu, Jing Sun, Zekun Zhang, Xiaohong Zheng, Xixiang Jing, Jingjing Wan, Jing Wang, Junqin Shi, Li-min Liu, Weimin Liu, Xiaoli Fan, Tengfei Cao","doi":"10.1038/s41524-025-01699-y","DOIUrl":null,"url":null,"abstract":"<p>Precise electric control of magnetic order and anomalous Hall conductivity (AHC) is pivotal for spintronics. While electric-field control of magnetic order and AHC has been explored in magneto-electric materials, achieving precise and energy-efficient magnetic order switching between two <span>\\(\\hat{P}\\hat{{T}}\\)</span> symmetry-connected magnetic states remains challenging. Here, we propose the utilization of the combined <span>\\(\\widehat{P}\\widehat{{T}}\\)</span> symmetry that establishes a direct connection between electric polarization and magnetic orders, to electrically manipulate magnetic order and the AHC. Using 3MnB₂T₄·2B₂T₃ (B = Sb/Bi, T = Se/Te) as an example, we demonstrate that the <span>\\(\\widehat{P}\\widehat{{T}}\\)</span> connected <i>up-up-down</i> (UUD) and <i>up-down-down</i> (UDD) states exhibit switchable magnetic configurations via electric polarization. The energy difference between the UUD and UDD states is linearly modulated by electric polarizations, enabling full control of the magnetic states via electric field, spontaneous polarization, or even weak sliding ferroelectricity. The findings demonstrate that <span>\\(\\widehat{P}\\widehat{{T}}\\)</span> symmetry can be well utilized to design electric polarization-controlled magnetic orders and will find important applications in spintronics.</p>","PeriodicalId":19342,"journal":{"name":"npj Computational Materials","volume":"647 1","pages":""},"PeriodicalIF":11.9000,"publicationDate":"2025-07-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"$$\\\\widehat{P}\\\\widehat{{T}}$$ symmetry controlled magnetic order switching\",\"authors\":\"Ziyu Niu, Jing Sun, Zekun Zhang, Xiaohong Zheng, Xixiang Jing, Jingjing Wan, Jing Wang, Junqin Shi, Li-min Liu, Weimin Liu, Xiaoli Fan, Tengfei Cao\",\"doi\":\"10.1038/s41524-025-01699-y\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p>Precise electric control of magnetic order and anomalous Hall conductivity (AHC) is pivotal for spintronics. While electric-field control of magnetic order and AHC has been explored in magneto-electric materials, achieving precise and energy-efficient magnetic order switching between two <span>\\\\(\\\\hat{P}\\\\hat{{T}}\\\\)</span> symmetry-connected magnetic states remains challenging. Here, we propose the utilization of the combined <span>\\\\(\\\\widehat{P}\\\\widehat{{T}}\\\\)</span> symmetry that establishes a direct connection between electric polarization and magnetic orders, to electrically manipulate magnetic order and the AHC. Using 3MnB₂T₄·2B₂T₃ (B = Sb/Bi, T = Se/Te) as an example, we demonstrate that the <span>\\\\(\\\\widehat{P}\\\\widehat{{T}}\\\\)</span> connected <i>up-up-down</i> (UUD) and <i>up-down-down</i> (UDD) states exhibit switchable magnetic configurations via electric polarization. The energy difference between the UUD and UDD states is linearly modulated by electric polarizations, enabling full control of the magnetic states via electric field, spontaneous polarization, or even weak sliding ferroelectricity. The findings demonstrate that <span>\\\\(\\\\widehat{P}\\\\widehat{{T}}\\\\)</span> symmetry can be well utilized to design electric polarization-controlled magnetic orders and will find important applications in spintronics.</p>\",\"PeriodicalId\":19342,\"journal\":{\"name\":\"npj Computational Materials\",\"volume\":\"647 1\",\"pages\":\"\"},\"PeriodicalIF\":11.9000,\"publicationDate\":\"2025-07-02\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"npj Computational Materials\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://doi.org/10.1038/s41524-025-01699-y\",\"RegionNum\":1,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"CHEMISTRY, PHYSICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"npj Computational Materials","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1038/s41524-025-01699-y","RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
引用次数: 0
摘要
磁序和异常霍尔电导率的精确电气控制是自旋电子学的关键。虽然在磁电材料中已经探索了磁序和AHC的电场控制,但在两个\(\hat{P}\hat{{T}}\)对称连接的磁态之间实现精确和节能的磁序切换仍然是一个挑战。在这里,我们提出利用联合\(\widehat{P}\widehat{{T}}\)对称,建立电极化和磁序之间的直接联系,以电操纵磁序和AHC。以3MnB₂T₄·2B₂T₃(B = Sb/Bi, T = Se/Te)为例,我们证明了\(\widehat{P}\widehat{{T}}\)连接的up-up-down (UUD)和up-down-down (UDD)态通过电极化表现出可切换的磁构型。UUD和UDD状态之间的能量差由电极化线性调制,从而可以通过电场、自发极化甚至弱滑动铁电来完全控制磁性状态。研究结果表明,\(\widehat{P}\widehat{{T}}\)对称性可以很好地用于设计电极化控制磁序,并将在自旋电子学中找到重要的应用。
$$\widehat{P}\widehat{{T}}$$ symmetry controlled magnetic order switching
Precise electric control of magnetic order and anomalous Hall conductivity (AHC) is pivotal for spintronics. While electric-field control of magnetic order and AHC has been explored in magneto-electric materials, achieving precise and energy-efficient magnetic order switching between two \(\hat{P}\hat{{T}}\) symmetry-connected magnetic states remains challenging. Here, we propose the utilization of the combined \(\widehat{P}\widehat{{T}}\) symmetry that establishes a direct connection between electric polarization and magnetic orders, to electrically manipulate magnetic order and the AHC. Using 3MnB₂T₄·2B₂T₃ (B = Sb/Bi, T = Se/Te) as an example, we demonstrate that the \(\widehat{P}\widehat{{T}}\) connected up-up-down (UUD) and up-down-down (UDD) states exhibit switchable magnetic configurations via electric polarization. The energy difference between the UUD and UDD states is linearly modulated by electric polarizations, enabling full control of the magnetic states via electric field, spontaneous polarization, or even weak sliding ferroelectricity. The findings demonstrate that \(\widehat{P}\widehat{{T}}\) symmetry can be well utilized to design electric polarization-controlled magnetic orders and will find important applications in spintronics.
期刊介绍:
npj Computational Materials is a high-quality open access journal from Nature Research that publishes research papers applying computational approaches for the design of new materials and enhancing our understanding of existing ones. The journal also welcomes papers on new computational techniques and the refinement of current approaches that support these aims, as well as experimental papers that complement computational findings.
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