V. Bruevich, Y. Patel, J. P. Singer and V. Podzorov
{"title":"新出现的薄膜晶体管研究中普遍存在明显的焦耳自热现象†。","authors":"V. Bruevich, Y. Patel, J. P. Singer and V. Podzorov","doi":"10.1039/D4TC02612H","DOIUrl":null,"url":null,"abstract":"<p >In this Perspective, recent literature on field-effect transistors based on emergent semiconducting materials, including metal-halide perovskites, conjugated polymers, and small-molecule organic semiconductors, is analyzed in terms of electric power and power density reached in transistors’ channel during their measurements. We used an <em>in situ</em> IR imaging to directly obtain the surface temperature distribution of biased devices under the experimental conditions commonly used in the literature. It is shown that at such conditions, the semiconducting channel would be resistively self-heated to significant temperatures, easily in excess of 150 °C. This implies a non-equilibrium device operation, possible materials’ degradation, parameter drift, and, in the best-case scenario, a non-room-temperature mobility extracted from such measurements. We show that this problem is rather common in various subfields represented in the literature, indicating that paying attention to the biasing conditions in transistor research and monitoring the local temperature of the semiconducting channel are necessary.</p>","PeriodicalId":84,"journal":{"name":"Journal of Materials Chemistry C","volume":" 44","pages":" 17802-17806"},"PeriodicalIF":5.7000,"publicationDate":"2024-10-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.rsc.org/en/content/articlepdf/2024/tc/d4tc02612h?page=search","citationCount":"0","resultStr":"{\"title\":\"Significant Joule self-heating pervasive in the emergent thin-film transistor studies†\",\"authors\":\"V. Bruevich, Y. Patel, J. P. Singer and V. Podzorov\",\"doi\":\"10.1039/D4TC02612H\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p >In this Perspective, recent literature on field-effect transistors based on emergent semiconducting materials, including metal-halide perovskites, conjugated polymers, and small-molecule organic semiconductors, is analyzed in terms of electric power and power density reached in transistors’ channel during their measurements. We used an <em>in situ</em> IR imaging to directly obtain the surface temperature distribution of biased devices under the experimental conditions commonly used in the literature. It is shown that at such conditions, the semiconducting channel would be resistively self-heated to significant temperatures, easily in excess of 150 °C. This implies a non-equilibrium device operation, possible materials’ degradation, parameter drift, and, in the best-case scenario, a non-room-temperature mobility extracted from such measurements. We show that this problem is rather common in various subfields represented in the literature, indicating that paying attention to the biasing conditions in transistor research and monitoring the local temperature of the semiconducting channel are necessary.</p>\",\"PeriodicalId\":84,\"journal\":{\"name\":\"Journal of Materials Chemistry C\",\"volume\":\" 44\",\"pages\":\" 17802-17806\"},\"PeriodicalIF\":5.7000,\"publicationDate\":\"2024-10-21\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"https://pubs.rsc.org/en/content/articlepdf/2024/tc/d4tc02612h?page=search\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Journal of Materials Chemistry C\",\"FirstCategoryId\":\"1\",\"ListUrlMain\":\"https://pubs.rsc.org/en/content/articlelanding/2024/tc/d4tc02612h\",\"RegionNum\":2,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"MATERIALS SCIENCE, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Journal of Materials Chemistry C","FirstCategoryId":"1","ListUrlMain":"https://pubs.rsc.org/en/content/articlelanding/2024/tc/d4tc02612h","RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"MATERIALS SCIENCE, MULTIDISCIPLINARY","Score":null,"Total":0}
Significant Joule self-heating pervasive in the emergent thin-film transistor studies†
In this Perspective, recent literature on field-effect transistors based on emergent semiconducting materials, including metal-halide perovskites, conjugated polymers, and small-molecule organic semiconductors, is analyzed in terms of electric power and power density reached in transistors’ channel during their measurements. We used an in situ IR imaging to directly obtain the surface temperature distribution of biased devices under the experimental conditions commonly used in the literature. It is shown that at such conditions, the semiconducting channel would be resistively self-heated to significant temperatures, easily in excess of 150 °C. This implies a non-equilibrium device operation, possible materials’ degradation, parameter drift, and, in the best-case scenario, a non-room-temperature mobility extracted from such measurements. We show that this problem is rather common in various subfields represented in the literature, indicating that paying attention to the biasing conditions in transistor research and monitoring the local temperature of the semiconducting channel are necessary.
期刊介绍:
The Journal of Materials Chemistry is divided into three distinct sections, A, B, and C, each catering to specific applications of the materials under study:
Journal of Materials Chemistry A focuses primarily on materials intended for applications in energy and sustainability.
Journal of Materials Chemistry B specializes in materials designed for applications in biology and medicine.
Journal of Materials Chemistry C is dedicated to materials suitable for applications in optical, magnetic, and electronic devices.
Example topic areas within the scope of Journal of Materials Chemistry C are listed below. This list is neither exhaustive nor exclusive.
Bioelectronics
Conductors
Detectors
Dielectrics
Displays
Ferroelectrics
Lasers
LEDs
Lighting
Liquid crystals
Memory
Metamaterials
Multiferroics
Photonics
Photovoltaics
Semiconductors
Sensors
Single molecule conductors
Spintronics
Superconductors
Thermoelectrics
Topological insulators
Transistors