Haoyu Dong , Xi Huang , Zhipeng Wu , Aofei Mao , Peizi Li , Bai Cui , Jean-François Silvain , Yusong Li , Yongfeng Lu
{"title":"在正十六烷液体中通过单步飞秒激光诱导加工实现聚丙烯表面的不粘超疏水性","authors":"Haoyu Dong , Xi Huang , Zhipeng Wu , Aofei Mao , Peizi Li , Bai Cui , Jean-François Silvain , Yusong Li , Yongfeng Lu","doi":"10.1016/j.optlastec.2024.111843","DOIUrl":null,"url":null,"abstract":"<div><div>The preparation of superhydrophobic polypropylene (PP) surfaces for biosafety is a pressing challenge in the food and medical industries. We achieve superhydrophobicity on commercial PP using a single-step process based on femtosecond (fs) laser-induced micro/nano texturing in n-hexadecane. Analysis of the wetting behavior after fs laser texturing revealed that 120 times of repetitive texturing, with a contact angle (CA) exceeding 150° and a rolling angle below 1° yielded optimal results. The generation, growth, and evolution of micro/nanostructures over processing times were investigated to establish a direct correlation between the micro/nanostructures and hydrophobicity. Furthermore, we elucidated the interactions between fs laser pulses and different material types in air, water, and n-hexadecane to explain the formation of micro/nanostructures formed in n-hexadecane.</div></div>","PeriodicalId":4,"journal":{"name":"ACS Applied Energy Materials","volume":null,"pages":null},"PeriodicalIF":5.4000,"publicationDate":"2024-09-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Non-sticky superhydrophobicity on polypropylene surfaces achieved via single-step femtosecond laser-induced processing in n-hexadecane liquid\",\"authors\":\"Haoyu Dong , Xi Huang , Zhipeng Wu , Aofei Mao , Peizi Li , Bai Cui , Jean-François Silvain , Yusong Li , Yongfeng Lu\",\"doi\":\"10.1016/j.optlastec.2024.111843\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><div>The preparation of superhydrophobic polypropylene (PP) surfaces for biosafety is a pressing challenge in the food and medical industries. We achieve superhydrophobicity on commercial PP using a single-step process based on femtosecond (fs) laser-induced micro/nano texturing in n-hexadecane. Analysis of the wetting behavior after fs laser texturing revealed that 120 times of repetitive texturing, with a contact angle (CA) exceeding 150° and a rolling angle below 1° yielded optimal results. The generation, growth, and evolution of micro/nanostructures over processing times were investigated to establish a direct correlation between the micro/nanostructures and hydrophobicity. Furthermore, we elucidated the interactions between fs laser pulses and different material types in air, water, and n-hexadecane to explain the formation of micro/nanostructures formed in n-hexadecane.</div></div>\",\"PeriodicalId\":4,\"journal\":{\"name\":\"ACS Applied Energy Materials\",\"volume\":null,\"pages\":null},\"PeriodicalIF\":5.4000,\"publicationDate\":\"2024-09-21\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"ACS Applied Energy Materials\",\"FirstCategoryId\":\"101\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S003039922401301X\",\"RegionNum\":3,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"CHEMISTRY, PHYSICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"ACS Applied Energy Materials","FirstCategoryId":"101","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S003039922401301X","RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
Non-sticky superhydrophobicity on polypropylene surfaces achieved via single-step femtosecond laser-induced processing in n-hexadecane liquid
The preparation of superhydrophobic polypropylene (PP) surfaces for biosafety is a pressing challenge in the food and medical industries. We achieve superhydrophobicity on commercial PP using a single-step process based on femtosecond (fs) laser-induced micro/nano texturing in n-hexadecane. Analysis of the wetting behavior after fs laser texturing revealed that 120 times of repetitive texturing, with a contact angle (CA) exceeding 150° and a rolling angle below 1° yielded optimal results. The generation, growth, and evolution of micro/nanostructures over processing times were investigated to establish a direct correlation between the micro/nanostructures and hydrophobicity. Furthermore, we elucidated the interactions between fs laser pulses and different material types in air, water, and n-hexadecane to explain the formation of micro/nanostructures formed in n-hexadecane.
期刊介绍:
ACS Applied Energy Materials is an interdisciplinary journal publishing original research covering all aspects of materials, engineering, chemistry, physics and biology relevant to energy conversion and storage. The journal is devoted to reports of new and original experimental and theoretical research of an applied nature that integrate knowledge in the areas of materials, engineering, physics, bioscience, and chemistry into important energy applications.