Zhuoqun Fang, Melissa Alzate-Banguero, Amit R. Rajapurohita, Forrest Simmons, Erica W. Carlson, Zhuoying Chen, Lionel Aigouy, Alexandre Zimmers
{"title":"通过聚焦激光束和原子力显微镜调节 VO2 结的电阻","authors":"Zhuoqun Fang, Melissa Alzate-Banguero, Amit R. Rajapurohita, Forrest Simmons, Erica W. Carlson, Zhuoying Chen, Lionel Aigouy, Alexandre Zimmers","doi":"10.1002/aelm.202400249","DOIUrl":null,"url":null,"abstract":"Vanadium Dioxide (VO<sub>2</sub>) is a material that exhibits a phase transition from an insulating state to a metallic state at ≈68 °C. During a temperature cycle consisting of warming followed by cooling, the resistivity of VO<sub>2</sub> changes by several orders of magnitude over the course of the hysteresis loop. Using a focused laser beam (λ = 532 nm), it is shown that it is possible to optically generate micron-sized metallic patterns within the insulating phase of a VO<sub>2</sub> planar junction which can be used to tune, on demand, the resistance of the VO<sub>2</sub> junction. A resistor network simulation is used to characterize the resulting resistance drops in the devices. These patterns persist while the base temperature is held constant within the hysteretic region while being easily removed totally by simply lowering the base temperature. Surprisingly, it is also observed that the pattern can be partially erased using an atomic force microscope (AFM) tip on the submicron scale. This erasing process can be qualitatively explained by the temperature difference between the VO<sub>2</sub> surface and the tip which acts as a local cooler. This optical and AFM resistive fine-tuning offers the possibility of creating controllable synaptic weights between room-temperature VO<sub>2</sub> neuristors.","PeriodicalId":110,"journal":{"name":"Advanced Electronic Materials","volume":"49 1","pages":""},"PeriodicalIF":5.3000,"publicationDate":"2024-09-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Tuning the Resistance of a VO2 Junction by Focused Laser Beam and Atomic Force Microscopy\",\"authors\":\"Zhuoqun Fang, Melissa Alzate-Banguero, Amit R. Rajapurohita, Forrest Simmons, Erica W. Carlson, Zhuoying Chen, Lionel Aigouy, Alexandre Zimmers\",\"doi\":\"10.1002/aelm.202400249\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"Vanadium Dioxide (VO<sub>2</sub>) is a material that exhibits a phase transition from an insulating state to a metallic state at ≈68 °C. During a temperature cycle consisting of warming followed by cooling, the resistivity of VO<sub>2</sub> changes by several orders of magnitude over the course of the hysteresis loop. Using a focused laser beam (λ = 532 nm), it is shown that it is possible to optically generate micron-sized metallic patterns within the insulating phase of a VO<sub>2</sub> planar junction which can be used to tune, on demand, the resistance of the VO<sub>2</sub> junction. A resistor network simulation is used to characterize the resulting resistance drops in the devices. These patterns persist while the base temperature is held constant within the hysteretic region while being easily removed totally by simply lowering the base temperature. Surprisingly, it is also observed that the pattern can be partially erased using an atomic force microscope (AFM) tip on the submicron scale. This erasing process can be qualitatively explained by the temperature difference between the VO<sub>2</sub> surface and the tip which acts as a local cooler. This optical and AFM resistive fine-tuning offers the possibility of creating controllable synaptic weights between room-temperature VO<sub>2</sub> neuristors.\",\"PeriodicalId\":110,\"journal\":{\"name\":\"Advanced Electronic Materials\",\"volume\":\"49 1\",\"pages\":\"\"},\"PeriodicalIF\":5.3000,\"publicationDate\":\"2024-09-11\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Advanced Electronic Materials\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://doi.org/10.1002/aelm.202400249\",\"RegionNum\":2,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"MATERIALS SCIENCE, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Advanced Electronic Materials","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1002/aelm.202400249","RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"MATERIALS SCIENCE, MULTIDISCIPLINARY","Score":null,"Total":0}
Tuning the Resistance of a VO2 Junction by Focused Laser Beam and Atomic Force Microscopy
Vanadium Dioxide (VO2) is a material that exhibits a phase transition from an insulating state to a metallic state at ≈68 °C. During a temperature cycle consisting of warming followed by cooling, the resistivity of VO2 changes by several orders of magnitude over the course of the hysteresis loop. Using a focused laser beam (λ = 532 nm), it is shown that it is possible to optically generate micron-sized metallic patterns within the insulating phase of a VO2 planar junction which can be used to tune, on demand, the resistance of the VO2 junction. A resistor network simulation is used to characterize the resulting resistance drops in the devices. These patterns persist while the base temperature is held constant within the hysteretic region while being easily removed totally by simply lowering the base temperature. Surprisingly, it is also observed that the pattern can be partially erased using an atomic force microscope (AFM) tip on the submicron scale. This erasing process can be qualitatively explained by the temperature difference between the VO2 surface and the tip which acts as a local cooler. This optical and AFM resistive fine-tuning offers the possibility of creating controllable synaptic weights between room-temperature VO2 neuristors.
期刊介绍:
Advanced Electronic Materials is an interdisciplinary forum for peer-reviewed, high-quality, high-impact research in the fields of materials science, physics, and engineering of electronic and magnetic materials. It includes research on physics and physical properties of electronic and magnetic materials, spintronics, electronics, device physics and engineering, micro- and nano-electromechanical systems, and organic electronics, in addition to fundamental research.