Self-activated nonreciprocal transmission isolation via absorption-asymmetry-triggered directional phase transition in VO2-based terahertz metamaterials

IF 5.1 2区 材料科学 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY
Chenxi Liu, Yanlin Xu, Hanqing Liu and He Ma
{"title":"Self-activated nonreciprocal transmission isolation via absorption-asymmetry-triggered directional phase transition in VO2-based terahertz metamaterials","authors":"Chenxi Liu, Yanlin Xu, Hanqing Liu and He Ma","doi":"10.1039/D5TC02947C","DOIUrl":null,"url":null,"abstract":"<p >This study theoretically and numerically establishes a novel strategy for self-activated nonreciprocal transmission isolation in terahertz metamaterials, exploiting the absorption asymmetry of a vanadium dioxide (VO<small><sub>2</sub></small>)-based structure to trigger directional phase transition under high-intensity illumination. Through coupled electromagnetic-thermal simulations, we analyze a tri-layer design where asymmetric absorption at specific frequencies—depending on incidence direction—induces markedly different thermal profiles. Crucially, high-intensity waves incident from the VO<small><sub>2</sub></small> side generate sufficient absorption-induced heating to surpass the phase transition threshold locally. This self-triggered phase change drastically suppresses transmission selectively for this direction, while waves incident from the opposing side experience significantly lower absorption and heating, maintaining high transmission. This fundamental asymmetry in thermal response enables nonreciprocal isolation without external excitation. Additionally, the transmission and absorption spectra are analyzed and the influences of absorption asymmetry, irradiation duration, incident power, and polarization direction are also investigated. This work demonstrates that harnessing absorption asymmetry to directionally control phase transition establishes a new paradigm for achieving nonreciprocal electromagnetic wave manipulation.</p>","PeriodicalId":84,"journal":{"name":"Journal of Materials Chemistry C","volume":" 40","pages":" 20491-20499"},"PeriodicalIF":5.1000,"publicationDate":"2025-09-09","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.rsc.org/en/content/articlepdf/2025/tc/d5tc02947c?page=search","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Journal of Materials Chemistry C","FirstCategoryId":"1","ListUrlMain":"https://pubs.rsc.org/en/content/articlelanding/2025/tc/d5tc02947c","RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"MATERIALS SCIENCE, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0

Abstract

This study theoretically and numerically establishes a novel strategy for self-activated nonreciprocal transmission isolation in terahertz metamaterials, exploiting the absorption asymmetry of a vanadium dioxide (VO2)-based structure to trigger directional phase transition under high-intensity illumination. Through coupled electromagnetic-thermal simulations, we analyze a tri-layer design where asymmetric absorption at specific frequencies—depending on incidence direction—induces markedly different thermal profiles. Crucially, high-intensity waves incident from the VO2 side generate sufficient absorption-induced heating to surpass the phase transition threshold locally. This self-triggered phase change drastically suppresses transmission selectively for this direction, while waves incident from the opposing side experience significantly lower absorption and heating, maintaining high transmission. This fundamental asymmetry in thermal response enables nonreciprocal isolation without external excitation. Additionally, the transmission and absorption spectra are analyzed and the influences of absorption asymmetry, irradiation duration, incident power, and polarization direction are also investigated. This work demonstrates that harnessing absorption asymmetry to directionally control phase transition establishes a new paradigm for achieving nonreciprocal electromagnetic wave manipulation.

Abstract Image

通过吸收不对称触发的vo2基太赫兹超材料的定向相变的自激活非互易传输隔离
本研究从理论上和数值上建立了一种在太赫兹超材料中自激活非互易传输隔离的新策略,利用二氧化钒(VO2)基结构的吸收不对称性来触发高强度照明下的定向相变。通过耦合电磁-热模拟,我们分析了三层设计,其中特定频率的不对称吸收-取决于入射方向-诱导显着不同的热剖面。至关重要的是,从VO2侧入射的高强度波产生足够的吸收诱导加热,从而在局部超过相变阈值。这种自触发的相变极大地选择性地抑制了该方向的传输,而从相反方向入射的波的吸收和加热明显降低,保持了高传输。热响应的这种基本不对称性使得无需外部激励的非互易隔离成为可能。分析了吸收和透射光谱,探讨了吸收不对称度、辐照时间、入射功率和偏振方向的影响。这项工作表明,利用吸收不对称来定向控制相变,为实现非互易电磁波操纵建立了一个新的范例。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
求助全文
约1分钟内获得全文 求助全文
来源期刊
Journal of Materials Chemistry C
Journal of Materials Chemistry C MATERIALS SCIENCE, MULTIDISCIPLINARY-PHYSICS, APPLIED
CiteScore
10.80
自引率
6.20%
发文量
1468
期刊介绍: The Journal of Materials Chemistry is divided into three distinct sections, A, B, and C, each catering to specific applications of the materials under study: Journal of Materials Chemistry A focuses primarily on materials intended for applications in energy and sustainability. Journal of Materials Chemistry B specializes in materials designed for applications in biology and medicine. Journal of Materials Chemistry C is dedicated to materials suitable for applications in optical, magnetic, and electronic devices. Example topic areas within the scope of Journal of Materials Chemistry C are listed below. This list is neither exhaustive nor exclusive. Bioelectronics Conductors Detectors Dielectrics Displays Ferroelectrics Lasers LEDs Lighting Liquid crystals Memory Metamaterials Multiferroics Photonics Photovoltaics Semiconductors Sensors Single molecule conductors Spintronics Superconductors Thermoelectrics Topological insulators Transistors
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
确定
请完成安全验证×
copy
已复制链接
快去分享给好友吧!
我知道了
右上角分享
点击右上角分享
0
联系我们:info@booksci.cn Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。 Copyright © 2023 布克学术 All rights reserved.
京ICP备2023020795号-1
ghs 京公网安备 11010802042870号
Book学术文献互助
Book学术文献互助群
群 号:604180095
Book学术官方微信