Sensory score prediction and key aroma compounds characterization in fermented chopped pepper

IF 8.2 1区 农林科学 Q1 CHEMISTRY, APPLIED
Yuan Liu , Lingyan Zhao , Chunya Yang , Yeyou Qin , Li Zhu , Fangming Deng
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Abstract

Fermented chopped pepper (FCP) exhibits complex and variable aroma profiles, making it challenging to accurately predict its sensory scores and identify key aroma compounds. In this study, electronic nose (E-nose) combined with machine learning methods were applied for the prediction of FCPs sensory scores. The random forest (RF) demonstrated the highest predictive accuracy among support vector machine (SVM), multiple linear regression (MLR), and back propagation neural network (BPNN). E-nose combined with the trained RF was used to predict the sensory scores of FCPs from eight regions. Totally, 97 volatile compounds and 19 odor-active compounds were detected by GC × GC-O-Q-TOF-MS in the top-performing sample (FCP-1). Among these, 34 compounds exhibited odor activity values (OAV) greater than 1. Aroma recombination and omission experiments confirmed that linalool, phenethyl alcohol, methional, 3-isobutyl-2-methoxypyrazine, ethyl trans-4-decenoate, β-ionone, spiroxide, ethyl 2-methylbutyrate, α-terpineol, 4-ethylphenol, β-damascenone, and nerolidol were the key aroma compounds in FCP-1.

Abstract Image

发酵辣椒感官评分预测及关键香气物质表征
发酵碎椒(FCP)具有复杂多变的香气特征,这给准确预测其感官评分和识别关键香气化合物带来了挑战。本研究将电子鼻(E-nose)与机器学习方法相结合,用于预测fcp感官评分。在支持向量机(SVM)、多元线性回归(MLR)和反向传播神经网络(BPNN)中,随机森林(RF)的预测精度最高。利用电子鼻结合训练射频预测8个区域的fcp感官评分。用GC × GC- o - q - tof - ms对最佳样品(FCP-1)共检测出97种挥发性化合物和19种气味活性化合物。其中34种化合物的气味活性值(OAV)大于1。香气重组和遗漏实验证实,芳樟醇、苯乙醇、甲基、3-异丁基-2-甲氧基吡嗪、反式-4-十烯酸乙酯、β-离子酮、螺旋氧化物、2-甲基丁酸乙酯、α-松油醇、4-乙基酚、β-大马马酮和神经樟醇是FCP-1的主要香气化合物。
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来源期刊
Food Chemistry: X
Food Chemistry: X CHEMISTRY, APPLIED-
CiteScore
4.90
自引率
6.60%
发文量
315
审稿时长
55 days
期刊介绍: Food Chemistry: X, one of three Open Access companion journals to Food Chemistry, follows the same aims, scope, and peer-review process. It focuses on papers advancing food and biochemistry or analytical methods, prioritizing research novelty. Manuscript evaluation considers novelty, scientific rigor, field advancement, and reader interest. Excluded are studies on food molecular sciences or disease cure/prevention. Topics include food component chemistry, bioactives, processing effects, additives, contaminants, and analytical methods. The journal welcome Analytical Papers addressing food microbiology, sensory aspects, and more, emphasizing new methods with robust validation and applicability to diverse foods or regions.
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