Chemical characterization and sensory evaluation of a phenolic-rich melanoidin isolate contributing to coffee astringency.

IF 5.1 1区 农林科学 Q1 BIOCHEMISTRY & MOLECULAR BIOLOGY
Food & Function Pub Date : 2025-03-21 DOI:10.1039/d4fo04934a
Brianne M Linne, Edisson Tello, Christopher T Simons, Devin G Peterson
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引用次数: 0

Abstract

The tactile flavor sensations of coffee are an important indicator of product quality, yet the stimuli contributing to these percepts remain insufficiently defined. In the present work, compounds that contribute to astringency in coffee were investigated. A multi-dimensional sensory-guided fractionation method was employed whereby preparative-scale liquid chromatography was leveraged to separate the coffee brew into subfractions, and then followed by sensory evaluation to identify fractions with perceptual impact. This process, paired with high-resolution chemical characterization via Fourier-transform ion cyclotron resonance/mass spectrometry, revealed a complex, phenolic-dominant, melanoidin fraction. Further sensory recombination testing confirmed this fraction imparted a perceptible astringent sensation at coffee-relevant concentrations in both water and coffee matrices. We hereby provide the first evidence of melanoidins contributing to the complex tactile flavor profile of coffee.

咖啡的触觉风味感觉是产品质量的重要指标,但导致这些感觉的刺激物仍未得到充分定义。本研究对造成咖啡涩味的化合物进行了调查。研究采用了一种多维感官引导分馏法,利用制备规模液相色谱法将咖啡冲泡物分离成子馏分,然后进行感官评估,以确定对感官有影响的馏分。这一过程与通过傅立叶变换离子回旋共振/质谱进行的高分辨率化学特性分析相结合,发现了一种复杂的、以酚类为主的类黑色素馏分。进一步的感官重组测试证实,在水和咖啡基质中,当达到与咖啡相关的浓度时,这种馏分会带来明显的涩味。我们在此首次证明了类黑色素对咖啡复杂的触觉风味的贡献。
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来源期刊
Food & Function
Food & Function BIOCHEMISTRY & MOLECULAR BIOLOGY-FOOD SCIENCE & TECHNOLOGY
CiteScore
10.10
自引率
6.60%
发文量
957
审稿时长
1.8 months
期刊介绍: Food & Function provides a unique venue for physicists, chemists, biochemists, nutritionists and other food scientists to publish work at the interface of the chemistry, physics and biology of food. The journal focuses on food and the functions of food in relation to health.
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