Zeming Li , Rensheng Shen , Yuantao Zhang , Guoqiang Zhong , Yuchun Chang , Hongwei Liang , Gaoqiang Deng , Xiaochuan Xia , Wancheng Li , Baolin Zhang
{"title":"Ultrahigh responsivity solar-blind high electron mobility photodetector utilizing a β-Ga2O3/GaN heterojunction","authors":"Zeming Li , Rensheng Shen , Yuantao Zhang , Guoqiang Zhong , Yuchun Chang , Hongwei Liang , Gaoqiang Deng , Xiaochuan Xia , Wancheng Li , Baolin Zhang","doi":"10.1016/j.mtphys.2025.101683","DOIUrl":null,"url":null,"abstract":"<div><div>β gallium oxide (β-Ga<sub>2</sub>O<sub>3</sub>) is considered as a primary choice for solar-blind ultraviolet (SBUV) detection because of its advantages such as intrinsic solar-blindness and robust stability. Nevertheless, the inherent low electron mobility of β-Ga<sub>2</sub>O<sub>3</sub> poses a significant challenge to its application. Here, β-Ga<sub>2</sub>O<sub>3</sub> films were integrated with gallium nitride (GaN) substrates through metal-organic chemical vapor deposition (MOCVD). Based on the obtained heterojunctions, a solar-blind high electron mobility photodetector (HEMPD) was developed. With the help of the minimal conduction band offset (0.12 eV), the photo-generated carriers are able to almost unhindered move between β-Ga<sub>2</sub>O<sub>3</sub> and GaN, and drift in GaN under an external field. Leveraging the high electron mobility advantage of GaN, the HEMPD achieves a responsivity (R) of 2.96 × 10<sup>4</sup> A/W and an external quantum efficiency (EQE) of 1.44 × 10<sup>7</sup> %, even surpassing some β-Ga<sub>2</sub>O<sub>3</sub>-based avalanche photodetectors (APDs). Furthermore, the indirect contact between GaN and electrodes significantly improves the SBUV/UV-A rejection ratio of our HEMPD compared to other vertical PDs based on β-Ga<sub>2</sub>O<sub>3</sub>/GaN heterojunctions. This study provides crucial insights for overcoming the low electron mobility limit of β-Ga<sub>2</sub>O<sub>3</sub>-based PDs.</div></div>","PeriodicalId":18253,"journal":{"name":"Materials Today Physics","volume":"52 ","pages":"Article 101683"},"PeriodicalIF":10.0000,"publicationDate":"2025-03-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Materials Today Physics","FirstCategoryId":"88","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S2542529325000392","RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"MATERIALS SCIENCE, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0
Abstract
β gallium oxide (β-Ga2O3) is considered as a primary choice for solar-blind ultraviolet (SBUV) detection because of its advantages such as intrinsic solar-blindness and robust stability. Nevertheless, the inherent low electron mobility of β-Ga2O3 poses a significant challenge to its application. Here, β-Ga2O3 films were integrated with gallium nitride (GaN) substrates through metal-organic chemical vapor deposition (MOCVD). Based on the obtained heterojunctions, a solar-blind high electron mobility photodetector (HEMPD) was developed. With the help of the minimal conduction band offset (0.12 eV), the photo-generated carriers are able to almost unhindered move between β-Ga2O3 and GaN, and drift in GaN under an external field. Leveraging the high electron mobility advantage of GaN, the HEMPD achieves a responsivity (R) of 2.96 × 104 A/W and an external quantum efficiency (EQE) of 1.44 × 107 %, even surpassing some β-Ga2O3-based avalanche photodetectors (APDs). Furthermore, the indirect contact between GaN and electrodes significantly improves the SBUV/UV-A rejection ratio of our HEMPD compared to other vertical PDs based on β-Ga2O3/GaN heterojunctions. This study provides crucial insights for overcoming the low electron mobility limit of β-Ga2O3-based PDs.
期刊介绍:
Materials Today Physics is a multi-disciplinary journal focused on the physics of materials, encompassing both the physical properties and materials synthesis. Operating at the interface of physics and materials science, this journal covers one of the largest and most dynamic fields within physical science. The forefront research in materials physics is driving advancements in new materials, uncovering new physics, and fostering novel applications at an unprecedented pace.