High stability modified CsPb(ClBr)3@glass@PS for wide color gamut mini-LED backlight displays†

IF 5.7 2区 材料科学 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY
Enrou Mei, Jiapeng Yang, Yanling Lin, Zhaoping Chen, Xiaojuan Liang and Weidong Xiang
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Abstract

Perovskite quantum dots (QDs) were considered as a new generation of emitters for lighting and displays due to their high photoluminescence (PL) efficiency and pure color. However, their commercialization process was currently hampered by stability issues and challenges in mass production. Amorphous glass-protected CsPbX3 perovskite nanocrystals (PNCs) have ultra-pure green light emission and excellent long-term stability. This work demonstrated that CsPb(Cl/Br)3@glass PNCs were successfully deposited in germane–silicate glass, and CsPbBr3@glass had bright green luminescence under ultraviolet irradiation, a narrow half-peak width (FWHM) and a high photoluminescence quantum yield (PLQY, 91.5%). The color gamut of the prepared WLED almost covered 123% of the NTSC 1953 standard and 91.8% of the Rec 2020 standard. It was proposed that a one-step mixed pressure film forming method using perovskite glass materials and PS materials can successfully obtain a high-quality, high-luminescence light conversion film, which can accelerate the commercialization of PQDs in display and lighting industries.

Abstract Image

Perovskite 量子点(QDs)具有高光致发光(PL)效率和纯色,被认为是用于照明和显示器的新一代发光体。然而,其商业化进程目前受到稳定性问题和大规模生产挑战的阻碍。非晶玻璃保护的 CsPbX3 包晶体纳米晶体(PNCs)具有超纯绿光发射和出色的长期稳定性。该研究表明,CsPb(Cl/Br)3@玻璃 PNCs 成功沉积在德国硅酸盐玻璃中,CsPbBr3@玻璃在紫外线照射下发出明亮的绿色荧光,具有较窄的半峰宽度(FWHM)和较高的光致发光量子产率(PLQY,91.5%)。制备的 WLED 色域几乎覆盖了 NTSC 1953 标准的 123% 和 Rec 2020 标准的 91.8%。该研究提出了一种使用包晶玻璃材料和 PS 材料的一步混合压力成膜方法,可成功获得高质量、高发光的光转换薄膜,从而加快 PQDs 在显示和照明行业的商业化进程。
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来源期刊
Journal of Materials Chemistry C
Journal of Materials Chemistry C MATERIALS SCIENCE, MULTIDISCIPLINARY-PHYSICS, APPLIED
CiteScore
10.80
自引率
6.20%
发文量
1468
期刊介绍: The Journal of Materials Chemistry is divided into three distinct sections, A, B, and C, each catering to specific applications of the materials under study: Journal of Materials Chemistry A focuses primarily on materials intended for applications in energy and sustainability. Journal of Materials Chemistry B specializes in materials designed for applications in biology and medicine. Journal of Materials Chemistry C is dedicated to materials suitable for applications in optical, magnetic, and electronic devices. Example topic areas within the scope of Journal of Materials Chemistry C are listed below. This list is neither exhaustive nor exclusive. Bioelectronics Conductors Detectors Dielectrics Displays Ferroelectrics Lasers LEDs Lighting Liquid crystals Memory Metamaterials Multiferroics Photonics Photovoltaics Semiconductors Sensors Single molecule conductors Spintronics Superconductors Thermoelectrics Topological insulators Transistors
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