Capture and Conversion of CO2 from Ambient Air Using Ionic Liquid-Plasma Combination

IF 2.6 3区 物理与天体物理 Q3 ENGINEERING, CHEMICAL
Sukma Wahyu Fitriani, Takamasa Okumura, Kunihiro Kamataki, Kazunori Koga, Masaharu Shiratani, Pankaj Attri
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引用次数: 0

Abstract

Climate change is considered one of the main challenges in this century, and CO2 emissions significantly cause it. Integrating CO2 capture, storage, and conversion is proposed to solve this problem. 1-Butyl-3-methylimidazolium chloride ([Bmim]Cl) ionic liquid was employed to capture and store CO2 from the air and subsequently converted into CO using non-thermal plasma. Moreover, we also tested the CO2 capture and storage capacity of water from different sources, e.g., Milli-Q, deionized water, and tap water. [Bmim]Cl solution captured CO2 from the air and then converted to CO after 24 h using plasma. In comparison with water (Milli-Q water, deionized water, and tap water), CO production was increased by 28.31% in the presence of water (Milli-Q water, deionized water, and tap water) + [Bmim]Cl. It suggests that this method could be a promising way to capture, store, and convert CO2 from air at atmospheric pressure and room temperature as an effort to reduce carbon emission.

Abstract Image

Abstract Image

利用离子液体-等离子体组合捕获和转化环境空气中的二氧化碳
气候变化被认为是本世纪的主要挑战之一,而二氧化碳排放是造成气候变化的主要原因。为了解决这一问题,人们提出了将二氧化碳捕集、封存和转化融为一体的方法。我们采用了 1-丁基-3-甲基氯化咪唑([Bmim]Cl)离子液体来捕获和储存空气中的二氧化碳,然后利用非热等离子体将其转化为一氧化碳。此外,我们还测试了不同水源(如 Milli-Q、去离子水和自来水)的二氧化碳捕获和储存能力。[Bmim]Cl溶液能捕获空气中的二氧化碳,并在24小时后利用等离子体转化为一氧化碳。与水(Milli-Q 水、去离子水和自来水)相比,在水(Milli-Q 水、去离子水和自来水)+[Bmim]Cl 的情况下,二氧化碳的生成量增加了 28.31%。这表明,这种方法是在常压和常温下从空气中捕获、储存和转化二氧化碳的一种可行方法,有助于减少碳排放。
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来源期刊
Plasma Chemistry and Plasma Processing
Plasma Chemistry and Plasma Processing 工程技术-工程:化工
CiteScore
5.90
自引率
8.30%
发文量
73
审稿时长
6-12 weeks
期刊介绍: Publishing original papers on fundamental and applied research in plasma chemistry and plasma processing, the scope of this journal includes processing plasmas ranging from non-thermal plasmas to thermal plasmas, and fundamental plasma studies as well as studies of specific plasma applications. Such applications include but are not limited to plasma catalysis, environmental processing including treatment of liquids and gases, biological applications of plasmas including plasma medicine and agriculture, surface modification and deposition, powder and nanostructure synthesis, energy applications including plasma combustion and reforming, resource recovery, coupling of plasmas and electrochemistry, and plasma etching. Studies of chemical kinetics in plasmas, and the interactions of plasmas with surfaces are also solicited. It is essential that submissions include substantial consideration of the role of the plasma, for example, the relevant plasma chemistry, plasma physics or plasma–surface interactions; manuscripts that consider solely the properties of materials or substances processed using a plasma are not within the journal’s scope.
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