北京某焦化化工厂土壤环境中多环芳烃的人体健康风险水平及分布

J. Jia, Haibin He, Zi-ying Wang, Shenwei Zhao, Linying Me, Jialin Liu, Shihai Zhang, Cunzhen Liang, Yinghua Zhang
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引用次数: 4

摘要

本研究采用索氏萃取-气相色谱法测定土壤样品中的多环芳烃(PAHs)有机污染物。通过口腔吸入、皮肤接触、从土壤表层吸入室外空气污染物、从土壤下层吸入室外空气污染物等4种主要暴露途径,对焦化化工厂5个不同采样点的人体健康风险进行了评价。结果表明,美国环保局对16种事前控制的多环芳烃的检出率为100%。三种主要污染物是Baa, Bbf, Bap。口服暴露途径ΣPAHs综合致癌风险是皮肤暴露途径致癌风险的498倍,是吸入土壤颗粒暴露途径致癌风险率的198倍。从土壤下层吸入室外空气污染物的致癌风险率几乎为0。土壤危害系数ΣPAHs主要空气污染物途径为口腔吸入和从土壤表面吸入室外空气。其总和接近90%,焦化厂区土壤危害系数ΣPAHs严重超标。焦化厂土壤中ΣPAHs的致癌风险主要暴露于口服摄入,致癌风险贡献率为99.3103%。结合中国焦化工业的发展特点、区域气候和地质特点,对ΣPAHs进行了人体健康风险评价。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Human Health Risk Levels and Distribution of PAHs in Soil Environment of a Coking Chemical Plant Located in Beijing, China
In this study, the polycyclic aromatic hydrocarbons (PAHs) organic pollutants in soil samples were determined by Soxhlet extraction- GCMS methods. Human health risks of as for 5 different sampling sites in the coking chemical plant were evaluated in four major Exposure routes, including oral intake, skin contact, inhalation the air pollutants of outdoor which from the soil surface, and inhalation the air pollutants of outdoor which from the soil lower layer. The results showed that the detection rate of 16 kinds precedent- controlled PAHs in the US Environmental Protection Agency was 100%. The three main pollutants are Baa, Bbf, Bap. The ΣPAHs comprehensive carcinogenicity risk of the oral exposure pathway is 498 times the carcinogenic risk of the skin exposure pathway, and 198 times the rate of carcinogenic risk of inhalation of soil particle Exposure route. And the rate of carcinogenic risk of Inhalation the air pollutants of outdoor which from the soil lower layer is almost 0. The hazard quotient of soil ΣPAHs main air pollutants pathway are oral intake and inhalation of outdoor air from the soil surface. The sum of them is close to 90%, The hazard quotient of soil ΣPAHs in the coking plant area is seriously exceeded. The risk of ΣPAHs in the soil of coking plant was mainly exposed to oral intake, and the contribution rate of carcinogenic risk was 99.3103%. Combined with the development characteristics of China's coking industry, regional climate and geological characteristics, make a human health risk assessment to ΣPAHs.
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