三角晶格上几何抑制的Ising反铁磁体的可能基态和磁场调谐相变

IF 16.4 1区 化学 Q1 CHEMISTRY, MULTIDISCIPLINARY
Thao Huong Pham
{"title":"三角晶格上几何抑制的Ising反铁磁体的可能基态和磁场调谐相变","authors":"Thao Huong Pham","doi":"10.1109/LMAG.2023.3274049","DOIUrl":null,"url":null,"abstract":"Possible average alignments of the spins in the ground state and the phase transitions of a geometrically frustrated Ising antiferromagnet in the presence of magnetic fields on a triangular lattice are studied in a mean field approximation. Starting from a zero-field clock phase, we can determine the phase boundaries from the curves of magnetic moments and their derivatives as functions of the fields. We also analyze the behavior of sublattice magnetic moments under the effect of the fields. The experimental relevances for TmMgGaO\n<sub>4</sub>\n and SrEr\n<sub>2</sub>\nO\n<sub>4</sub>\n are discussed. Besides, using a functional integral method, we have calculated a functional for free energy to obtain the contribution of spin fluctuations. From this, we can find that the role of the quantum spin fluctuations at very low temperatures is only prominent in the vicinity of the transition points. It can therefore be seen that the results, although given in the mean field approximation, describe quite well the phase transitions and rearrangements of the magnetic moment per spin under the effect of both the transverse and longitudinal fields.","PeriodicalId":1,"journal":{"name":"Accounts of Chemical Research","volume":null,"pages":null},"PeriodicalIF":16.4000,"publicationDate":"2023-03-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Possible Ground States and Magnetic-Field-Tuned Phase Transitions of a Geometrically Frustrated Ising Antiferromagnet on a Triangular Lattice\",\"authors\":\"Thao Huong Pham\",\"doi\":\"10.1109/LMAG.2023.3274049\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"Possible average alignments of the spins in the ground state and the phase transitions of a geometrically frustrated Ising antiferromagnet in the presence of magnetic fields on a triangular lattice are studied in a mean field approximation. Starting from a zero-field clock phase, we can determine the phase boundaries from the curves of magnetic moments and their derivatives as functions of the fields. We also analyze the behavior of sublattice magnetic moments under the effect of the fields. The experimental relevances for TmMgGaO\\n<sub>4</sub>\\n and SrEr\\n<sub>2</sub>\\nO\\n<sub>4</sub>\\n are discussed. Besides, using a functional integral method, we have calculated a functional for free energy to obtain the contribution of spin fluctuations. From this, we can find that the role of the quantum spin fluctuations at very low temperatures is only prominent in the vicinity of the transition points. It can therefore be seen that the results, although given in the mean field approximation, describe quite well the phase transitions and rearrangements of the magnetic moment per spin under the effect of both the transverse and longitudinal fields.\",\"PeriodicalId\":1,\"journal\":{\"name\":\"Accounts of Chemical Research\",\"volume\":null,\"pages\":null},\"PeriodicalIF\":16.4000,\"publicationDate\":\"2023-03-08\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Accounts of Chemical Research\",\"FirstCategoryId\":\"101\",\"ListUrlMain\":\"https://ieeexplore.ieee.org/document/10120918/\",\"RegionNum\":1,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"CHEMISTRY, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Accounts of Chemical Research","FirstCategoryId":"101","ListUrlMain":"https://ieeexplore.ieee.org/document/10120918/","RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0

摘要

在平均场近似下,研究了在三角形晶格上存在磁场的情况下,几何受抑的伊辛反铁磁体基态自旋的可能平均排列和相变。从零场时钟相位开始,我们可以根据磁矩及其导数作为场函数的曲线来确定相位边界。我们还分析了场作用下亚晶格磁矩的行为。讨论了TmMgGaO4和SrEr2O4的实验相关性。此外,利用泛函积分方法,我们计算了自由能的泛函,得到了自旋涨落的贡献。由此,我们可以发现,在非常低的温度下,量子自旋涨落的作用只在跃迁点附近突出。因此可以看出,尽管这些结果是在平均场近似中给出的,但它们很好地描述了在横向场和纵向场的影响下每自旋磁矩的相变和重排。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Possible Ground States and Magnetic-Field-Tuned Phase Transitions of a Geometrically Frustrated Ising Antiferromagnet on a Triangular Lattice
Possible average alignments of the spins in the ground state and the phase transitions of a geometrically frustrated Ising antiferromagnet in the presence of magnetic fields on a triangular lattice are studied in a mean field approximation. Starting from a zero-field clock phase, we can determine the phase boundaries from the curves of magnetic moments and their derivatives as functions of the fields. We also analyze the behavior of sublattice magnetic moments under the effect of the fields. The experimental relevances for TmMgGaO 4 and SrEr 2 O 4 are discussed. Besides, using a functional integral method, we have calculated a functional for free energy to obtain the contribution of spin fluctuations. From this, we can find that the role of the quantum spin fluctuations at very low temperatures is only prominent in the vicinity of the transition points. It can therefore be seen that the results, although given in the mean field approximation, describe quite well the phase transitions and rearrangements of the magnetic moment per spin under the effect of both the transverse and longitudinal fields.
求助全文
通过发布文献求助,成功后即可免费获取论文全文。 去求助
来源期刊
Accounts of Chemical Research
Accounts of Chemical Research 化学-化学综合
CiteScore
31.40
自引率
1.10%
发文量
312
审稿时长
2 months
期刊介绍: Accounts of Chemical Research presents short, concise and critical articles offering easy-to-read overviews of basic research and applications in all areas of chemistry and biochemistry. These short reviews focus on research from the author’s own laboratory and are designed to teach the reader about a research project. In addition, Accounts of Chemical Research publishes commentaries that give an informed opinion on a current research problem. Special Issues online are devoted to a single topic of unusual activity and significance. Accounts of Chemical Research replaces the traditional article abstract with an article "Conspectus." These entries synopsize the research affording the reader a closer look at the content and significance of an article. Through this provision of a more detailed description of the article contents, the Conspectus enhances the article's discoverability by search engines and the exposure for the research.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
确定
请完成安全验证×
copy
已复制链接
快去分享给好友吧!
我知道了
右上角分享
点击右上角分享
0
联系我们:info@booksci.cn Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。 Copyright © 2023 布克学术 All rights reserved.
京ICP备2023020795号-1
ghs 京公网安备 11010802042870号
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术官方微信