{"title":"印度德里季风和非季风季节PM10碳质气溶胶及其实时湿清除","authors":"Saurabh Sonwani, Umesh C. Kulshrestha","doi":"10.1007/s10874-019-09396-z","DOIUrl":null,"url":null,"abstract":"<p>Real-time simultaneous measurements of rainwater and PM<sub>10</sub> chemistry were carried out at Delhi during the year 2016–17 in order to assess the levels of carbonaceous species and their wet scavenging during monsoon and non-monsoon seasons at Delhi. The PM<sub>10</sub> samples were collected Before Rain (BR), During Rain (DR) and After Rain (AR) events, while rainwater samples collected on an event basis. The ambient OC levels were always higher than the levels of EC during both monsoon and non-monsoon seasons in ambient aerosol as well as in rainwater. On an average, during rain (DR) 30% of OC aerosols and 28.2% of EC aerosols removed via wet scavenging process. In after rain (AR), 26.2% OC and 1.8% EC aerosols further decreased in comparison to DR samples due to the presence of OC and EC free air parcel. Overall it observed that the OC concentration significantly lowered from BR to DR and AR. However, EC concentrations in AR were found to be higher than DR samples indicating their build-up after the rains. The Scavenging Ratios (SRs) of OC and rain intensity had a significant positive correlation, whereas the SRs of EC showed a weak correlation with rain intensity. The SRs of EC were significantly higher during non-monsoon as compared to monsoon season. Such characteristics can be explained based on the particles size, source and the hygroscopicity of both types of carbonaceous aerosol.</p>","PeriodicalId":611,"journal":{"name":"Journal of Atmospheric Chemistry","volume":"76 3","pages":"171 - 200"},"PeriodicalIF":3.0000,"publicationDate":"2019-08-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://sci-hub-pdf.com/10.1007/s10874-019-09396-z","citationCount":"32","resultStr":"{\"title\":\"PM10 carbonaceous aerosols and their real-time wet scavenging during monsoon and non-monsoon seasons at Delhi, India\",\"authors\":\"Saurabh Sonwani, Umesh C. Kulshrestha\",\"doi\":\"10.1007/s10874-019-09396-z\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p>Real-time simultaneous measurements of rainwater and PM<sub>10</sub> chemistry were carried out at Delhi during the year 2016–17 in order to assess the levels of carbonaceous species and their wet scavenging during monsoon and non-monsoon seasons at Delhi. The PM<sub>10</sub> samples were collected Before Rain (BR), During Rain (DR) and After Rain (AR) events, while rainwater samples collected on an event basis. The ambient OC levels were always higher than the levels of EC during both monsoon and non-monsoon seasons in ambient aerosol as well as in rainwater. On an average, during rain (DR) 30% of OC aerosols and 28.2% of EC aerosols removed via wet scavenging process. In after rain (AR), 26.2% OC and 1.8% EC aerosols further decreased in comparison to DR samples due to the presence of OC and EC free air parcel. Overall it observed that the OC concentration significantly lowered from BR to DR and AR. However, EC concentrations in AR were found to be higher than DR samples indicating their build-up after the rains. The Scavenging Ratios (SRs) of OC and rain intensity had a significant positive correlation, whereas the SRs of EC showed a weak correlation with rain intensity. The SRs of EC were significantly higher during non-monsoon as compared to monsoon season. Such characteristics can be explained based on the particles size, source and the hygroscopicity of both types of carbonaceous aerosol.</p>\",\"PeriodicalId\":611,\"journal\":{\"name\":\"Journal of Atmospheric Chemistry\",\"volume\":\"76 3\",\"pages\":\"171 - 200\"},\"PeriodicalIF\":3.0000,\"publicationDate\":\"2019-08-21\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"https://sci-hub-pdf.com/10.1007/s10874-019-09396-z\",\"citationCount\":\"32\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Journal of Atmospheric Chemistry\",\"FirstCategoryId\":\"89\",\"ListUrlMain\":\"https://link.springer.com/article/10.1007/s10874-019-09396-z\",\"RegionNum\":4,\"RegionCategory\":\"地球科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"ENVIRONMENTAL SCIENCES\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Journal of Atmospheric Chemistry","FirstCategoryId":"89","ListUrlMain":"https://link.springer.com/article/10.1007/s10874-019-09396-z","RegionNum":4,"RegionCategory":"地球科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"ENVIRONMENTAL SCIENCES","Score":null,"Total":0}
PM10 carbonaceous aerosols and their real-time wet scavenging during monsoon and non-monsoon seasons at Delhi, India
Real-time simultaneous measurements of rainwater and PM10 chemistry were carried out at Delhi during the year 2016–17 in order to assess the levels of carbonaceous species and their wet scavenging during monsoon and non-monsoon seasons at Delhi. The PM10 samples were collected Before Rain (BR), During Rain (DR) and After Rain (AR) events, while rainwater samples collected on an event basis. The ambient OC levels were always higher than the levels of EC during both monsoon and non-monsoon seasons in ambient aerosol as well as in rainwater. On an average, during rain (DR) 30% of OC aerosols and 28.2% of EC aerosols removed via wet scavenging process. In after rain (AR), 26.2% OC and 1.8% EC aerosols further decreased in comparison to DR samples due to the presence of OC and EC free air parcel. Overall it observed that the OC concentration significantly lowered from BR to DR and AR. However, EC concentrations in AR were found to be higher than DR samples indicating their build-up after the rains. The Scavenging Ratios (SRs) of OC and rain intensity had a significant positive correlation, whereas the SRs of EC showed a weak correlation with rain intensity. The SRs of EC were significantly higher during non-monsoon as compared to monsoon season. Such characteristics can be explained based on the particles size, source and the hygroscopicity of both types of carbonaceous aerosol.
期刊介绍：
The Journal of Atmospheric Chemistry is devoted to the study of the chemistry of the Earth''s atmosphere, the emphasis being laid on the region below about 100 km. The strongly interdisciplinary nature of atmospheric chemistry means that it embraces a great variety of sciences, but the journal concentrates on the following topics:
Observational, interpretative and modelling studies of the composition of air and precipitation and the physiochemical processes in the Earth''s atmosphere, excluding air pollution problems of local importance only.
The role of the atmosphere in biogeochemical cycles; the chemical interaction of the oceans, land surface and biosphere with the atmosphere.
Laboratory studies of the mechanics in homogeneous and heterogeneous transformation processes in the atmosphere.
Descriptions of major advances in instrumentation developed for the measurement of atmospheric composition and chemical properties.
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