改进性能的甲烷蒸汽重整多入口太阳能热化学反应器的设计

Pei-Yuan Dou, Xin-Yuan Tang, Wei-Wei Yang, Ya-Ling He
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引用次数: 7

摘要

反应器结构设计对太阳能热甲烷重整反应器的性能起着重要作用。在传统预热反应器的基础上,本研究提出了一种具有多个入口的圆柱形太阳能甲烷重整反应器,以改变温度场分布,从而提高了反应器中反应区的温度,从而提高反应器的性能。应用一个考虑质量、动量、物种、能量守恒以及甲烷重整热化学反应动力学的多物理模型,对反应器性能进行了数值研究,并分析了影响性能提高的因素。研究发现,与传统的预热反应器相比,所提出的具有用于气体进料的内部和外部入口的圆柱形反应器增强了从排出气体中的热回收,并为反应器中的反应提供了更合适的温度场。在不同的操作条件下,与传统设计相比,多入口圆柱形反应器中的甲烷转化率提高了9.5%至19.1%,氢气产量提高了12.1%至40.3%,尽管总反应催化剂体积减少了。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Design of a multi-inlet solar thermochemical reactor for steam methane reforming with improved performance

Reactor structure design plays an important role in the performance of solar-thermal methane reforming reactors. Based on a conventional preheating reactor, this study proposed a cylindrical solar methane reforming reactor with multiple inlets to vary the temperature field distribution, which improved the temperature of the reaction region in the reactor, thereby improving the reactor performance. A multi-physical model that considers mass, momentum, species, energy conservation, as well as thermochemical reaction kinetics of methane reforming, was applied to numerically investigate the reactor performance and analyze the factors that affect performance improvement. It was found that compared with a conventional preheating reactor, the proposed cylindrical reactor with inner and external inlets for gas feeding enhanced heat recovery from the exhausted gas and provided a more suitable temperature field for the reaction in the reactor. Under different operating conditions, the methane conversion in the cylindrical reactor with multi-inlet increased by 9.5% to 19.1%, and the hydrogen production was enhanced by 12.1% to 40.3% in comparison with the conventional design, even though the total reaction catalyst volume was reduced.

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