在CdS纳米棒上原位生长几层二硫化钼用于高效光催化制氢

IF 3.1 4区 工程技术 Q3 ENERGY & FUELS
Wei Chen, Xiang Liu, Shaojie Wei, Qianqian Heng, Binfen Wang, Shilong Liu, Li Gao, Liqun Mao
{"title":"在CdS纳米棒上原位生长几层二硫化钼用于高效光催化制氢","authors":"Wei Chen,&nbsp;Xiang Liu,&nbsp;Shaojie Wei,&nbsp;Qianqian Heng,&nbsp;Binfen Wang,&nbsp;Shilong Liu,&nbsp;Li Gao,&nbsp;Liqun Mao","doi":"10.1007/s11708-021-0779-3","DOIUrl":null,"url":null,"abstract":"<div><p>An ultrathin MoS<sub>2</sub> was grown on CdS nanorod by a solid state method using sulfur powder as sulfur source for photocatalytic H<sub>2</sub> production. The characterization result reveals that the ultrathin MoS<sub>2</sub> nanosheets loaded on CdS has a good contact state. The photoelectrochemical result shows that MoS<sub>2</sub> not only are beneficial for charge separation, but also works as active sites, thus enhancing photocatalytic activity. Compared with pure CdS, the photocatalytic activity of MoS<sub>2</sub> loaded CdS was significantly improved. The hydrogen evolution rate on <i>m</i>(MoS<sub>2</sub>): <i>m</i>(CdS) = 1: 50 (<i>m</i> is mass) reaches 542 μmol/h, which is 6 times of that on pure CdS (92 μmol/h). This work provides a new design for photocatalysts with high photocatalytic activities and provides a deeper understanding of the effect of MoS<sub>2</sub> on enhancing photocatalytic activity.</p></div>","PeriodicalId":570,"journal":{"name":"Frontiers in Energy","volume":"15 3","pages":"752 - 759"},"PeriodicalIF":3.1000,"publicationDate":"2021-09-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"3","resultStr":"{\"title\":\"In situ growth of a-few-layered MoS2 on CdS nanorod for high efficient photocatalytic H2 production\",\"authors\":\"Wei Chen,&nbsp;Xiang Liu,&nbsp;Shaojie Wei,&nbsp;Qianqian Heng,&nbsp;Binfen Wang,&nbsp;Shilong Liu,&nbsp;Li Gao,&nbsp;Liqun Mao\",\"doi\":\"10.1007/s11708-021-0779-3\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><p>An ultrathin MoS<sub>2</sub> was grown on CdS nanorod by a solid state method using sulfur powder as sulfur source for photocatalytic H<sub>2</sub> production. The characterization result reveals that the ultrathin MoS<sub>2</sub> nanosheets loaded on CdS has a good contact state. The photoelectrochemical result shows that MoS<sub>2</sub> not only are beneficial for charge separation, but also works as active sites, thus enhancing photocatalytic activity. Compared with pure CdS, the photocatalytic activity of MoS<sub>2</sub> loaded CdS was significantly improved. The hydrogen evolution rate on <i>m</i>(MoS<sub>2</sub>): <i>m</i>(CdS) = 1: 50 (<i>m</i> is mass) reaches 542 μmol/h, which is 6 times of that on pure CdS (92 μmol/h). This work provides a new design for photocatalysts with high photocatalytic activities and provides a deeper understanding of the effect of MoS<sub>2</sub> on enhancing photocatalytic activity.</p></div>\",\"PeriodicalId\":570,\"journal\":{\"name\":\"Frontiers in Energy\",\"volume\":\"15 3\",\"pages\":\"752 - 759\"},\"PeriodicalIF\":3.1000,\"publicationDate\":\"2021-09-15\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"3\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Frontiers in Energy\",\"FirstCategoryId\":\"5\",\"ListUrlMain\":\"https://link.springer.com/article/10.1007/s11708-021-0779-3\",\"RegionNum\":4,\"RegionCategory\":\"工程技术\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q3\",\"JCRName\":\"ENERGY & FUELS\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Frontiers in Energy","FirstCategoryId":"5","ListUrlMain":"https://link.springer.com/article/10.1007/s11708-021-0779-3","RegionNum":4,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"ENERGY & FUELS","Score":null,"Total":0}
引用次数: 3

摘要

以硫粉为硫源,采用固态法在CdS纳米棒上生长超薄二硫化钼,用于光催化制氢。表征结果表明,负载在CdS上的超薄二硫化钼纳米片具有良好的接触状态。光电化学结果表明,二硫化钼不仅有利于电荷分离,而且可以作为活性位点,从而提高光催化活性。与纯CdS相比,负载MoS2的CdS的光催化活性显著提高。当m(MoS2): m(CdS) = 1:50 (m为质量)时,析氢速率达到542 μmol/h,是纯CdS (92 μmol/h)的6倍。本研究为高光催化活性的光催化剂提供了一种新的设计思路,并对二硫化钼增强光催化活性的作用有了更深入的了解。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
In situ growth of a-few-layered MoS2 on CdS nanorod for high efficient photocatalytic H2 production

An ultrathin MoS2 was grown on CdS nanorod by a solid state method using sulfur powder as sulfur source for photocatalytic H2 production. The characterization result reveals that the ultrathin MoS2 nanosheets loaded on CdS has a good contact state. The photoelectrochemical result shows that MoS2 not only are beneficial for charge separation, but also works as active sites, thus enhancing photocatalytic activity. Compared with pure CdS, the photocatalytic activity of MoS2 loaded CdS was significantly improved. The hydrogen evolution rate on m(MoS2): m(CdS) = 1: 50 (m is mass) reaches 542 μmol/h, which is 6 times of that on pure CdS (92 μmol/h). This work provides a new design for photocatalysts with high photocatalytic activities and provides a deeper understanding of the effect of MoS2 on enhancing photocatalytic activity.

求助全文
通过发布文献求助,成功后即可免费获取论文全文。 去求助
来源期刊
Frontiers in Energy
Frontiers in Energy Energy-Energy Engineering and Power Technology
CiteScore
5.90
自引率
6.90%
发文量
708
期刊介绍: Frontiers in Energy, an interdisciplinary and peer-reviewed international journal launched in January 2007, seeks to provide a rapid and unique platform for reporting the most advanced research on energy technology and strategic thinking in order to promote timely communication between researchers, scientists, engineers, and policy makers in the field of energy. Frontiers in Energy aims to be a leading peer-reviewed platform and an authoritative source of information for analyses, reviews and evaluations in energy engineering and research, with a strong focus on energy analysis, energy modelling and prediction, integrated energy systems, energy conversion and conservation, energy planning and energy on economic and policy issues. Frontiers in Energy publishes state-of-the-art review articles, original research papers and short communications by individual researchers or research groups. It is strictly peer-reviewed and accepts only original submissions in English. The scope of the journal is broad and covers all latest focus in current energy research. High-quality papers are solicited in, but are not limited to the following areas: -Fundamental energy science -Energy technology, including energy generation, conversion, storage, renewables, transport, urban design and building efficiency -Energy and the environment, including pollution control, energy efficiency and climate change -Energy economics, strategy and policy -Emerging energy issue
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
确定
请完成安全验证×
copy
已复制链接
快去分享给好友吧!
我知道了
右上角分享
点击右上角分享
0
联系我们:info@booksci.cn Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。 Copyright © 2023 布克学术 All rights reserved.
京ICP备2023020795号-1
ghs 京公网安备 11010802042870号
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术官方微信