Jianxin Li , Yuhua Wang , Yitong Wang , Yao Guo , Shiding Zhang , Haixiang Song , Xianchang Li , Qianqian Gao , Wanyu Shang , Shuaishuai Hu , Huibin Zheng , Xifei Li
{"title":"MXene Ti3C2修饰的g-C3N4/ZnO光催化剂具有改善的光催化CO2还原性能","authors":"Jianxin Li , Yuhua Wang , Yitong Wang , Yao Guo , Shiding Zhang , Haixiang Song , Xianchang Li , Qianqian Gao , Wanyu Shang , Shuaishuai Hu , Huibin Zheng , Xifei Li","doi":"10.1016/j.nanoms.2023.02.003","DOIUrl":null,"url":null,"abstract":"<div><p>Photocatalytic reduction of CO<sub>2</sub> is considered as a kind of promising technologies for solving the greenhouse effect. Herein, a novel hybrid structure of g-C<sub>3</sub>N<sub>4</sub>/ZnO/Ti<sub>3</sub>C<sub>2</sub> photocatalysts was designed and fabricated to investigate their abilities for CO<sub>2</sub> reduction. As demonstration, heterojunction of g-C<sub>3</sub>N<sub>4</sub>/ZnO can improve photogenerated carriers’ separation, the addition of Ti<sub>3</sub>C<sub>2</sub> fragments can further facilitate the photocatalytic performance from CO<sub>2</sub> to CO. Hence, g-C<sub>3</sub>N<sub>4</sub>/ZnO/Ti<sub>3</sub>C<sub>2</sub> has efficiently increased CO production by 8 and 12 times than pristine g-C<sub>3</sub>N<sub>4</sub> and ZnO, respectively. Which is ascribed to the photogenerated charge migration promoted by metallic Ti<sub>3</sub>C<sub>2</sub>. This work provides a guideline for designing efficient hybrid catalysts on other applications in the renewable energy fields.</p></div>","PeriodicalId":33573,"journal":{"name":"Nano Materials Science","volume":"5 2","pages":"Pages 237-245"},"PeriodicalIF":9.9000,"publicationDate":"2023-06-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"17","resultStr":"{\"title\":\"MXene Ti3C2 decorated g-C3N4/ZnO photocatalysts with improved photocatalytic performance for CO2 reduction\",\"authors\":\"Jianxin Li , Yuhua Wang , Yitong Wang , Yao Guo , Shiding Zhang , Haixiang Song , Xianchang Li , Qianqian Gao , Wanyu Shang , Shuaishuai Hu , Huibin Zheng , Xifei Li\",\"doi\":\"10.1016/j.nanoms.2023.02.003\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><p>Photocatalytic reduction of CO<sub>2</sub> is considered as a kind of promising technologies for solving the greenhouse effect. Herein, a novel hybrid structure of g-C<sub>3</sub>N<sub>4</sub>/ZnO/Ti<sub>3</sub>C<sub>2</sub> photocatalysts was designed and fabricated to investigate their abilities for CO<sub>2</sub> reduction. As demonstration, heterojunction of g-C<sub>3</sub>N<sub>4</sub>/ZnO can improve photogenerated carriers’ separation, the addition of Ti<sub>3</sub>C<sub>2</sub> fragments can further facilitate the photocatalytic performance from CO<sub>2</sub> to CO. Hence, g-C<sub>3</sub>N<sub>4</sub>/ZnO/Ti<sub>3</sub>C<sub>2</sub> has efficiently increased CO production by 8 and 12 times than pristine g-C<sub>3</sub>N<sub>4</sub> and ZnO, respectively. Which is ascribed to the photogenerated charge migration promoted by metallic Ti<sub>3</sub>C<sub>2</sub>. This work provides a guideline for designing efficient hybrid catalysts on other applications in the renewable energy fields.</p></div>\",\"PeriodicalId\":33573,\"journal\":{\"name\":\"Nano Materials Science\",\"volume\":\"5 2\",\"pages\":\"Pages 237-245\"},\"PeriodicalIF\":9.9000,\"publicationDate\":\"2023-06-01\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"17\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Nano Materials Science\",\"FirstCategoryId\":\"1089\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S2589965123000065\",\"RegionNum\":2,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"Engineering\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Nano Materials Science","FirstCategoryId":"1089","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S2589965123000065","RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"Engineering","Score":null,"Total":0}
MXene Ti3C2 decorated g-C3N4/ZnO photocatalysts with improved photocatalytic performance for CO2 reduction
Photocatalytic reduction of CO2 is considered as a kind of promising technologies for solving the greenhouse effect. Herein, a novel hybrid structure of g-C3N4/ZnO/Ti3C2 photocatalysts was designed and fabricated to investigate their abilities for CO2 reduction. As demonstration, heterojunction of g-C3N4/ZnO can improve photogenerated carriers’ separation, the addition of Ti3C2 fragments can further facilitate the photocatalytic performance from CO2 to CO. Hence, g-C3N4/ZnO/Ti3C2 has efficiently increased CO production by 8 and 12 times than pristine g-C3N4 and ZnO, respectively. Which is ascribed to the photogenerated charge migration promoted by metallic Ti3C2. This work provides a guideline for designing efficient hybrid catalysts on other applications in the renewable energy fields.
期刊介绍:
Nano Materials Science (NMS) is an international and interdisciplinary, open access, scholarly journal. NMS publishes peer-reviewed original articles and reviews on nanoscale material science and nanometer devices, with topics encompassing preparation and processing; high-throughput characterization; material performance evaluation and application of material characteristics such as the microstructure and properties of one-dimensional, two-dimensional, and three-dimensional nanostructured and nanofunctional materials; design, preparation, and processing techniques; and performance evaluation technology and nanometer device applications.