氟化/掺氟纳米碳基材料在各种电池中的氟化途径、作用机理及应用综述

IF 13.1 1区 化学 Q1 Energy
Weicui Liu , Nanping Deng , Gang Wang , Ruru Yu , Xiaoxiao Wang , Bowen Cheng , Jingge Ju , Weimin Kang
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引用次数: 2

摘要

随着电子技术的普及和广泛应用,对电池材料的性能提出了更高的要求。由于氟原子和碳原子之间的电负性差异很大,在纳米碳基材料中掺杂氟原子被认为是提高废旧电池性能的有效途径。然而,对掺氟纳米结构碳材料在各种电池中的作用机理和研究进展进行系统综述仍存在空白。本文详细综述了不同氟源下氟化/氟掺杂纳米碳基材料的合成路线以及CFx在各种电池中的作用机理。随后,从纳米碳源的结构和电化学性能之间的相关性来看,回顾了基于不同尺寸(0D–3D)的CFx在一次电池应用中的进展,并对能量密度和功率密度之间的平衡进行了批判性的讨论。此外,还详细总结了近年来CFx材料在二次电池中的作用及其应用现状,以说明引入F原子的效果。最后,我们展望了CFx材料的前景,并提供了一些见解和建议,以促进CFx材料在各种高性能电池应用中的进一步探索。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Fluoridation routes, function mechanism and application of fluorinated/fluorine-doped nanocarbon-based materials for various batteries: A review

Fluoridation routes, function mechanism and application of fluorinated/fluorine-doped nanocarbon-based materials for various batteries: A review

With the popularity and widespread applications of electronics, higher demands are being placed on the performance of battery materials. Due to the large difference in electronegativity between fluorine and carbon atoms, doping fluorine atoms in nanocarbon-based materials is considered an effective way to improve the performance of used battery. However, there is still a blank in the systematic review of the mechanism and research progress of fluorine-doped nanostructured carbon materials in various batteries. In this review, the synthetic routes of fluorinated/fluorine-doped nanocarbon-based (CFx) materials under different fluorine sources and the function mechanism of CFx in various batteries are reviewed in detail. Subsequently, judging from the dependence between the structure and electrochemical performance of nanocarbon sources, the progress of CFx based on different dimensions (0D–3D) for primary battery applications is reviewed and the balance between energy density and power density is critically discussed. In addition, the roles of CFx materials in secondary batteries and their current applications in recent years are summarized in detail to illustrate the effect of introducing F atoms. Finally, we envisage the prospect of CFx materials and offer some insights and recommendations to facilitate the further exploration of CFx materials for various high-performance battery applications.

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来源期刊
Journal of Energy Chemistry
Journal of Energy Chemistry CHEMISTRY, APPLIED-CHEMISTRY, PHYSICAL
CiteScore
19.10
自引率
8.40%
发文量
3631
审稿时长
15 days
期刊介绍: The Journal of Energy Chemistry, the official publication of Science Press and the Dalian Institute of Chemical Physics, Chinese Academy of Sciences, serves as a platform for reporting creative research and innovative applications in energy chemistry. It mainly reports on creative researches and innovative applications of chemical conversions of fossil energy, carbon dioxide, electrochemical energy and hydrogen energy, as well as the conversions of biomass and solar energy related with chemical issues to promote academic exchanges in the field of energy chemistry and to accelerate the exploration, research and development of energy science and technologies. This journal focuses on original research papers covering various topics within energy chemistry worldwide, including: Optimized utilization of fossil energy Hydrogen energy Conversion and storage of electrochemical energy Capture, storage, and chemical conversion of carbon dioxide Materials and nanotechnologies for energy conversion and storage Chemistry in biomass conversion Chemistry in the utilization of solar energy
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