高温阴离子交换膜燃料电池

IF 5.4 Q2 CHEMISTRY, PHYSICAL
John C. Douglin , John R. Varcoe , Dario R. Dekel
{"title":"高温阴离子交换膜燃料电池","authors":"John C. Douglin ,&nbsp;John R. Varcoe ,&nbsp;Dario R. Dekel","doi":"10.1016/j.powera.2020.100023","DOIUrl":null,"url":null,"abstract":"<div><p>In the past few years, developments in anion exchange membranes (AEMs) have led to a significant increase in hydroxide conductivities, ultimately yielding striking improvements in the performance of anion exchange membrane fuel cells (AEMFCs) at low operating temperatures, usually at 40–80 °C. Aside from these remarkable achievements, the literature is void of any work on AEMFCs operated at temperatures above 100 °C, despite the consensus from various models remarking that working at higher cell temperatures may lead to many significant advantages. In this work, we present the first high-temperature AEMFC (HT-AEMFC) tested at 110 °C. The HT-AEMFC exhibits high performance, with a peak power density of 2.1 W cm<sup>−2</sup> and a current density of as high as 574 mA cm<sup>−2</sup> measured at 0.8 V. This initial work represents a significant landmark for the research and development of the fuel cell technology, opening a wide door for a new field of research we call hereafter, <em>HT-AEMFCs</em>.</p></div>","PeriodicalId":34318,"journal":{"name":"Journal of Power Sources Advances","volume":null,"pages":null},"PeriodicalIF":5.4000,"publicationDate":"2020-10-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://sci-hub-pdf.com/10.1016/j.powera.2020.100023","citationCount":"65","resultStr":"{\"title\":\"A high-temperature anion-exchange membrane fuel cell\",\"authors\":\"John C. Douglin ,&nbsp;John R. Varcoe ,&nbsp;Dario R. Dekel\",\"doi\":\"10.1016/j.powera.2020.100023\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><p>In the past few years, developments in anion exchange membranes (AEMs) have led to a significant increase in hydroxide conductivities, ultimately yielding striking improvements in the performance of anion exchange membrane fuel cells (AEMFCs) at low operating temperatures, usually at 40–80 °C. Aside from these remarkable achievements, the literature is void of any work on AEMFCs operated at temperatures above 100 °C, despite the consensus from various models remarking that working at higher cell temperatures may lead to many significant advantages. In this work, we present the first high-temperature AEMFC (HT-AEMFC) tested at 110 °C. The HT-AEMFC exhibits high performance, with a peak power density of 2.1 W cm<sup>−2</sup> and a current density of as high as 574 mA cm<sup>−2</sup> measured at 0.8 V. This initial work represents a significant landmark for the research and development of the fuel cell technology, opening a wide door for a new field of research we call hereafter, <em>HT-AEMFCs</em>.</p></div>\",\"PeriodicalId\":34318,\"journal\":{\"name\":\"Journal of Power Sources Advances\",\"volume\":null,\"pages\":null},\"PeriodicalIF\":5.4000,\"publicationDate\":\"2020-10-01\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"https://sci-hub-pdf.com/10.1016/j.powera.2020.100023\",\"citationCount\":\"65\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Journal of Power Sources Advances\",\"FirstCategoryId\":\"1085\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S2666248520300238\",\"RegionNum\":0,\"RegionCategory\":null,\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"CHEMISTRY, PHYSICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Journal of Power Sources Advances","FirstCategoryId":"1085","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S2666248520300238","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
引用次数: 65

摘要

在过去的几年里,阴离子交换膜(AEMs)的发展导致了氢氧化物电导率的显著增加,最终使阴离子交换膜燃料电池(aemfc)在低温(通常为40-80 °C)下的性能得到了显著改善。除了这些显著的成就之外,尽管各种模型一致认为在更高的电池温度下工作可能会带来许多显着的优势,但文献中没有任何关于在100 °C以上温度下工作的aemfc的工作。在这项工作中,我们提出了第一个在110 °C下测试的高温AEMFC (HT-AEMFC)。HT-AEMFC表现出高性能,峰值功率密度为2.1 W cm−2,在0.8 V下测量的电流密度高达574 mA cm−2。这项初步工作代表了燃料电池技术研究和发展的一个重要里程碑,为我们称之为ht - aemfc的新研究领域打开了广阔的大门。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

A high-temperature anion-exchange membrane fuel cell

A high-temperature anion-exchange membrane fuel cell

In the past few years, developments in anion exchange membranes (AEMs) have led to a significant increase in hydroxide conductivities, ultimately yielding striking improvements in the performance of anion exchange membrane fuel cells (AEMFCs) at low operating temperatures, usually at 40–80 °C. Aside from these remarkable achievements, the literature is void of any work on AEMFCs operated at temperatures above 100 °C, despite the consensus from various models remarking that working at higher cell temperatures may lead to many significant advantages. In this work, we present the first high-temperature AEMFC (HT-AEMFC) tested at 110 °C. The HT-AEMFC exhibits high performance, with a peak power density of 2.1 W cm−2 and a current density of as high as 574 mA cm−2 measured at 0.8 V. This initial work represents a significant landmark for the research and development of the fuel cell technology, opening a wide door for a new field of research we call hereafter, HT-AEMFCs.

求助全文
通过发布文献求助,成功后即可免费获取论文全文。 去求助
来源期刊
CiteScore
9.10
自引率
0.00%
发文量
18
审稿时长
64 days
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
确定
请完成安全验证×
copy
已复制链接
快去分享给好友吧!
我知道了
右上角分享
点击右上角分享
0
联系我们:info@booksci.cn Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。 Copyright © 2023 布克学术 All rights reserved.
京ICP备2023020795号-1
ghs 京公网安备 11010802042870号
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术官方微信