高果糖玉米糖浆的生产及其5-羟甲基糠醛和增值呋喃衍生物的新应用:前景与挑战

IF 20.2 Q1 MATERIALS SCIENCE, PAPER & WOOD
Aristide Laurel Mokale Kognou , Sarita Shrestha , Zihua Jiang , Chunbao (Charles) Xu , Fubao Sun , Wensheng Qin
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引用次数: 4

摘要

高果糖玉米糖浆是利用葡萄糖异构酶将葡萄糖转化为果糖而生产出来的,四聚体金属酶在工业生物催化中应用广泛。酶工程和葡萄糖异构酶商业化生产的进步为探索这些酶的更有效变体铺平了道路。5-羟甲基糠醛可以由高果糖玉米糖浆催化脱水制得,并可进一步通过化学或生物方法转化为各种呋喃类化合物,是一种很有前景的平台化学品,可用于各种工业应用。虽然5-羟甲基糠醛化学转化为呋喃化合物的研究近年来得到了广泛的研究,但由于化学反应条件恶劣,生物转化的条件温和,显示出了很大的前景。本文综述了提高葡萄糖异构酶产量的蛋白质工程潜力以及5-羟甲基糠醛生物转化为增值呋喃衍生物的最新进展。提出了5-羟甲基糠醛产业化的生物学策略。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
High-fructose corn syrup production and its new applications for 5-hydroxymethylfurfural and value-added furan derivatives: Promises and challenges

High fructose corn syrup has been industrially produced by converting glucose to fructose by glucose isomerases, tetrameric metalloenzymes widely used in industrial biocatalysis. Advances in enzyme engineering and commercial production of glucose isomerase have paved the way to explore more efficient variants of these enzymes. The 5-hydroxymethylfurfural can be produced from high fructose corn syrup catalytic dehydration, and it can be further converted into various furanic compounds chemically or biologically for various industrial applications as a promising platform chemical. Although the chemical conversion of 5-hydroxymethylfurfural into furanic compounds has been extensively investigated in recent years, bioconversion has shown promise for its mild conditions due to the harsh chemical reaction conditions. This review discusses protein engineering potential for improving glucose isomerase production and recent advancements in bioconversion of 5-hydroxymethylfurfural into value-added furanic derivatives. It suggests biological strategies for the industrial transformation of 5-hydroxymethylfurfural.

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来源期刊
Journal of Bioresources and Bioproducts
Journal of Bioresources and Bioproducts Agricultural and Biological Sciences-Forestry
CiteScore
39.30
自引率
0.00%
发文量
38
审稿时长
12 weeks
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