Thomas Warburton, Stuart K. Grange, James R. Hopkins, Stephen J. Andrews, Alastair C. Lewis, Neil Owen, Caroline Jordan, Greg Adamson and Bin Xia
{"title":"插入式散香器对住宅室内VOC浓度的影响","authors":"Thomas Warburton, Stuart K. Grange, James R. Hopkins, Stephen J. Andrews, Alastair C. Lewis, Neil Owen, Caroline Jordan, Greg Adamson and Bin Xia","doi":"10.1039/D2EM00444E","DOIUrl":null,"url":null,"abstract":"<p >Plug-in fragrance diffusers are one of myriad volatile organic compound-containing consumer products that are commonly found in homes. The perturbing effects of using a commercial diffuser indoors were evaluated using a study group of 60 homes in Ashford, UK. Air samples were taken over 3 day periods with the diffuser switched on and in a parallel set of control homes where it was off. At least four measurements were taken in each home using vacuum-release into 6 L silica-coated canisters and with >40 VOCs quantified using gas chromatography with FID and MS (GC-FID-QMS). Occupants self-reported their use of other VOC-containing products. The variability between homes was very high with the 72 hour sum of all measured VOCs ranging between 30 and >5000 μg m<small><sup>?3</sup></small>, dominated by <em>n</em>/i-butane, propane, and ethanol. For those homes in the lowest quartile of air exchange rate (identified using CO<small><sub>2</sub></small> and TVOC sensors as proxies) the use of a diffuser led to a statistically significant increase (<em>p</em>-value < 0.02) in the summed concentration of detectable fragrance VOCs and some individual species, <em>e.g.</em> alpha pinene rising from a median of 9 μg m<small><sup>?3</sup></small> to 15 μg m<small><sup>?3</sup></small> (<em>p</em>-value < 0.02). The observed increments were broadly in line with model-calculated estimates based on fragrance weight loss, room sizes and air exchange rates.</p>","PeriodicalId":74,"journal":{"name":"Environmental Science: Processes & Impacts","volume":" 4","pages":" 805-817"},"PeriodicalIF":4.3000,"publicationDate":"2023-03-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.rsc.org/en/content/articlepdf/2023/em/d2em00444e?page=search","citationCount":"2","resultStr":"{\"title\":\"The impact of plug-in fragrance diffusers on residential indoor VOC concentrations†\",\"authors\":\"Thomas Warburton, Stuart K. Grange, James R. Hopkins, Stephen J. Andrews, Alastair C. Lewis, Neil Owen, Caroline Jordan, Greg Adamson and Bin Xia\",\"doi\":\"10.1039/D2EM00444E\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p >Plug-in fragrance diffusers are one of myriad volatile organic compound-containing consumer products that are commonly found in homes. The perturbing effects of using a commercial diffuser indoors were evaluated using a study group of 60 homes in Ashford, UK. Air samples were taken over 3 day periods with the diffuser switched on and in a parallel set of control homes where it was off. At least four measurements were taken in each home using vacuum-release into 6 L silica-coated canisters and with >40 VOCs quantified using gas chromatography with FID and MS (GC-FID-QMS). Occupants self-reported their use of other VOC-containing products. The variability between homes was very high with the 72 hour sum of all measured VOCs ranging between 30 and >5000 μg m<small><sup>?3</sup></small>, dominated by <em>n</em>/i-butane, propane, and ethanol. For those homes in the lowest quartile of air exchange rate (identified using CO<small><sub>2</sub></small> and TVOC sensors as proxies) the use of a diffuser led to a statistically significant increase (<em>p</em>-value < 0.02) in the summed concentration of detectable fragrance VOCs and some individual species, <em>e.g.</em> alpha pinene rising from a median of 9 μg m<small><sup>?3</sup></small> to 15 μg m<small><sup>?3</sup></small> (<em>p</em>-value < 0.02). The observed increments were broadly in line with model-calculated estimates based on fragrance weight loss, room sizes and air exchange rates.</p>\",\"PeriodicalId\":74,\"journal\":{\"name\":\"Environmental Science: Processes & Impacts\",\"volume\":\" 4\",\"pages\":\" 805-817\"},\"PeriodicalIF\":4.3000,\"publicationDate\":\"2023-03-08\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"https://pubs.rsc.org/en/content/articlepdf/2023/em/d2em00444e?page=search\",\"citationCount\":\"2\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Environmental Science: Processes & Impacts\",\"FirstCategoryId\":\"93\",\"ListUrlMain\":\"https://pubs.rsc.org/en/content/articlelanding/2023/em/d2em00444e\",\"RegionNum\":3,\"RegionCategory\":\"环境科学与生态学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"CHEMISTRY, ANALYTICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Environmental Science: Processes & Impacts","FirstCategoryId":"93","ListUrlMain":"https://pubs.rsc.org/en/content/articlelanding/2023/em/d2em00444e","RegionNum":3,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, ANALYTICAL","Score":null,"Total":0}
The impact of plug-in fragrance diffusers on residential indoor VOC concentrations†
Plug-in fragrance diffusers are one of myriad volatile organic compound-containing consumer products that are commonly found in homes. The perturbing effects of using a commercial diffuser indoors were evaluated using a study group of 60 homes in Ashford, UK. Air samples were taken over 3 day periods with the diffuser switched on and in a parallel set of control homes where it was off. At least four measurements were taken in each home using vacuum-release into 6 L silica-coated canisters and with >40 VOCs quantified using gas chromatography with FID and MS (GC-FID-QMS). Occupants self-reported their use of other VOC-containing products. The variability between homes was very high with the 72 hour sum of all measured VOCs ranging between 30 and >5000 μg m?3, dominated by n/i-butane, propane, and ethanol. For those homes in the lowest quartile of air exchange rate (identified using CO2 and TVOC sensors as proxies) the use of a diffuser led to a statistically significant increase (p-value < 0.02) in the summed concentration of detectable fragrance VOCs and some individual species, e.g. alpha pinene rising from a median of 9 μg m?3 to 15 μg m?3 (p-value < 0.02). The observed increments were broadly in line with model-calculated estimates based on fragrance weight loss, room sizes and air exchange rates.
期刊介绍:
Environmental Science: Processes & Impacts publishes high quality papers in all areas of the environmental chemical sciences, including chemistry of the air, water, soil and sediment. We welcome studies on the environmental fate and effects of anthropogenic and naturally occurring contaminants, both chemical and microbiological, as well as related natural element cycling processes.