Flexible Torsional Photoactuators Based on MXene–Carbon Nanotube–Paraffin Wax Films

A flexible actuator, which can convert external stimuli to mechanical motion, is an essential component of every soft robot and determines its performance. As a novel two-dimensional material, MXene has been used to fabricate flexible actuators due to its excellent physical properties. Although MXene-based actuators exhibit excellent actuation performance, their bending deformation is solely due to the in-plane isotropy of the MXene film, and an MXene torsional actuator has not been reported. This study presents a flexible torsional actuator based on an MXene–carbon nanotube (CNT)–paraffin wax (PW) film. In this actuator, the MXene thin film acts as a light absorption layer with wavelength selectivity, superaligned CNT provides structural anisotropy for the composite film, and PW acts as the active layer. The chirality and helical structure of the actuator could be tuned by the orientation of the CNT film. Such an actuator delivers excellent actuation performance, including high work density (～1.2 J/cm³), low triggering power (77 mW/cm²), high rotational speed (320°/s), long lifetime (30,000 cycles), and wavelength selectivity. Inspired by vines, we used the torsional actuator as a spiral grabber, which lifted an object that weighs 20 times more than the actuator. The high-performance torsional actuator would be potentially used as a noncontact sensor, rotary motor, and grabbing tool in the soft robot system.