同步加速器红外纳米光谱学与成像

IF 8.2 1区 化学 Q1 CHEMISTRY, PHYSICAL
Hans A. Bechtel , Samuel C. Johnson , Omar Khatib , Eric A. Muller , Markus B. Raschke
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引用次数: 26

摘要

红外光谱学已经发展成为一种强大的分析技术,可以探测分子和晶格振动,低能电子激发和相关性,以及相关的集体表面等离子体,声子或其他极化共振。与扫描探针显微镜相结合,近场红外纳米光谱学和成像技术最近成为成像科学的前沿,使复杂的非均质材料的研究具有纳米尺度的空间分辨率和化学和量子态光谱特异性。在这里,我们描述了同步红外纳米光谱(SINS),它利用同步红外辐射的低噪声、宽带、高光谱辐照度和相干性,在纳米空间分辨率下进行中远红外近场红外测量。这种强大的组合为纳米尺度、中尺度和表面现象的宽带空间光谱分析提供了一种定性的新形式,这些现象以前很难用红外技术或任何形式的微光谱学进行研究。我们回顾了捷联惯导系统的发展,描述了它的技术实现,并重点介绍了在物理、化学、生物、材料科学、地质、大气和空间科学等领域快速增长的应用范围。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Synchrotron infrared nano-spectroscopy and -imaging

Infrared (IR) spectroscopy has evolved into a powerful analytical technique to probe molecular and lattice vibrations, low-energy electronic excitations and correlations, and related collective surface plasmon, phonon, or other polaritonic resonances. In combination with scanning probe microscopy, near-field infrared nano-spectroscopy and -imaging techniques have recently emerged as a frontier in imaging science, enabling the study of complex heterogeneous materials with simultaneous nanoscale spatial resolution and chemical and quantum state spectroscopic specificity. Here, we describe synchrotron infrared nano-spectroscopy (SINS), which takes advantage of the low-noise, broadband, high spectral irradiance, and coherence of synchrotron infrared radiation for near-field infrared measurements across the mid- to far-infrared with nanometer spatial resolution. This powerful combination provides a qualitatively new form of broadband spatio-spectral analysis of nanoscale, mesoscale, and surface phenomena that were previously difficult to study with IR techniques, or even any form of micro-spectroscopy in general. We review the development of SINS, describe its technical implementations, and highlight selected examples representative of the rapidly growing range of applications in physics, chemistry, biology, materials science, geology, and atmospheric and space sciences.

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来源期刊
Surface Science Reports
Surface Science Reports 化学-物理:凝聚态物理
CiteScore
15.90
自引率
2.00%
发文量
9
审稿时长
178 days
期刊介绍: Surface Science Reports is a journal that specializes in invited review papers on experimental and theoretical studies in the physics, chemistry, and pioneering applications of surfaces, interfaces, and nanostructures. The topics covered in the journal aim to contribute to a better understanding of the fundamental phenomena that occur on surfaces and interfaces, as well as the application of this knowledge to the development of materials, processes, and devices. In this journal, the term "surfaces" encompasses all interfaces between solids, liquids, polymers, biomaterials, nanostructures, soft matter, gases, and vacuum. Additionally, the journal includes reviews of experimental techniques and methods used to characterize surfaces and surface processes, such as those based on the interactions of photons, electrons, and ions with surfaces.
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