净尘沉降动力学对低风速的非单调响应

IF 5.7 1区 地球科学 Q1 ENVIRONMENTAL SCIENCES
Ruochen Jia,Chaoqun Ba,Chao Zhang,Wennong Kuang,Yuan Liu,Zhigang Wang,Fang Liu,Zhiming Xin,Yuting Liu,Qun Ma,Lu Zong,Wei Liang,Jianqiang Qian,Zhimin Liu
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引用次数: 0

摘要

干沉降是矿物粉尘的主要沉降源,但其在弱风条件下的沉降特性仍未得到很好的约束,且常与风速单调参数化。在这里,我们使用两阶段方案(在0,2,4和6 m s - 1时短暂的高风速加载,然后是低风速沉积)量化了闭环再循环风洞中大小分解的粉尘网积累动力学。累积滞留质量时间序列用收集盘阵列测量,初始悬浮粉尘负荷由在线浓度监测仪记录。通过激光衍射表征了颗粒的大小,并将其分为6个直径阈值类(PM 2.5 -PM 63)。一阶动力学模型描述了时间积累动力学,并产生了拟合的渐近保留质量(A)、有效净积累率系数(k)、特征时间尺度(τ=1/k)和初始净积累通量(J 0 = A k)。PM 2.5 -PM 30在2 m s−1时测得的j0最高,PM 40和PM 63在4 m s−1时测得的j0最高,而在6 m s−1时测得的j0显著下降。四个风速级别的二次拟合表明PM 2.5 -PM 40的潜在最大值在2-3 m s - 1附近。这些测量量化了有效表面保留对低风速的大小相关响应,并为耦合沉积、保留和再夹带参数化提供了基准行为。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Non-monotonic response of net dust deposition kinetics to low wind speeds
Dry deposition is a major sink for mineral dust, yet its behavior under weak winds remains poorly constrained and is often parameterized monotonically with wind speed. Here we quantify size-resolved dust net accumulation kinetics in a closed-circuit recirculating wind tunnel using a two-stage protocol (brief high-wind loading followed by low-wind deposition at 0, 2, 4, and 6 m s −1 ). Cumulative retained-mass time series were measured with an array of collection trays, with the initial suspended dust loading recorded by an online concentration monitor. Particle sizes were characterized by laser diffraction and grouped into six diameter-threshold classes (PM 2.5 –PM 63 ). A first-order kinetic model described the temporal accumulation dynamics and yielded a fitted asymptotic retained mass ( a ), effective net-accumulation rate coefficient ( k ), characteristic time scale (τ=1/k), and initial net accumulation flux ( J 0 = a k ). The observed  J 0 was highest at 2 m s −1 for PM 2.5 –PM 30 , and 4 m s −1 for PM 40 and PM 63 , while  J 0 declined markedly at 6 m s −1 for the lower diameter thresholds. Quadratic fits across the four wind-speed levels suggest a potential maximum near 2–3 m s −1 for PM 2.5 –PM 40 . These measurements quantify the size-dependent response of effective surface retention to low wind speeds and provide benchmark behavior for coupled deposition, retention, and re-entrainment parameterizations.
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来源期刊
Atmospheric Chemistry and Physics
Atmospheric Chemistry and Physics 地学-气象与大气科学
CiteScore
10.70
自引率
20.60%
发文量
702
审稿时长
6 months
期刊介绍: Atmospheric Chemistry and Physics (ACP) is a not-for-profit international scientific journal dedicated to the publication and public discussion of high-quality studies investigating the Earth''s atmosphere and the underlying chemical and physical processes. It covers the altitude range from the land and ocean surface up to the turbopause, including the troposphere, stratosphere, and mesosphere. The main subject areas comprise atmospheric modelling, field measurements, remote sensing, and laboratory studies of gases, aerosols, clouds and precipitation, isotopes, radiation, dynamics, biosphere interactions, and hydrosphere interactions. The journal scope is focused on studies with general implications for atmospheric science rather than investigations that are primarily of local or technical interest.
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