二氧化碳产品驱动的综合碳捕集与利用生产环状碳酸盐

IF 7.6 1区 化学 Q1 CHEMISTRY, MULTIDISCIPLINARY
Alejandro Belinchón,Pablo Navarro,Pedro Carvalho,José Palomar
{"title":"二氧化碳产品驱动的综合碳捕集与利用生产环状碳酸盐","authors":"Alejandro Belinchón,Pablo Navarro,Pedro Carvalho,José Palomar","doi":"10.1021/acssuschemeng.6c08760","DOIUrl":null,"url":null,"abstract":"There is an urgent need to develop energy-efficient solutions for CO2 capture and utilization, because current integrated processes remain limited by the compatibility of the capture and conversion stages. This work proposes a novel product-driven carbon capture and utilization concept, in which the CO2-derived cyclic carbonate product is sequentially employed as a physical CO2 absorbent and subsequently as the reaction medium for its own synthesis, eliminating the intermediate solvent regeneration step. Density, viscosity, and CO2 solubility were experimentally determined for four cyclic carbonates, while cycloaddition reactions were performed under representative integrated process conditions using the ionic liquid [bmim]I as a catalyst. The complete process for natural gas purification was evaluated through conductor-like screening model (COSMO)-based/Aspen process simulation and life cycle assessment. Experimental and computational results demonstrate that propylene, butylene, and hexylene carbonates provide competitive CO2 absorption performance, extending the applicability of the proposed concept to other CO2-derived cyclic carbonates. More importantly, the direct use of the CO2-rich cyclic carbonate stream as the reaction medium was experimentally validated without significant thermodynamic or kinetic limitations despite the high product concentration. The proposed concept achieves a competitive energy demand and CO2-related emissions while avoiding deep vacuum operation and intermediate solvent regeneration.","PeriodicalId":25,"journal":{"name":"ACS Sustainable Chemistry & Engineering","volume":"15 1","pages":""},"PeriodicalIF":7.6000,"publicationDate":"2026-10-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"CO2-Product-Driven Integrated Carbon Capture and Utilization to Produce Cyclic Carbonates\",\"authors\":\"Alejandro Belinchón,Pablo Navarro,Pedro Carvalho,José Palomar\",\"doi\":\"10.1021/acssuschemeng.6c08760\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"There is an urgent need to develop energy-efficient solutions for CO2 capture and utilization, because current integrated processes remain limited by the compatibility of the capture and conversion stages. This work proposes a novel product-driven carbon capture and utilization concept, in which the CO2-derived cyclic carbonate product is sequentially employed as a physical CO2 absorbent and subsequently as the reaction medium for its own synthesis, eliminating the intermediate solvent regeneration step. Density, viscosity, and CO2 solubility were experimentally determined for four cyclic carbonates, while cycloaddition reactions were performed under representative integrated process conditions using the ionic liquid [bmim]I as a catalyst. The complete process for natural gas purification was evaluated through conductor-like screening model (COSMO)-based/Aspen process simulation and life cycle assessment. Experimental and computational results demonstrate that propylene, butylene, and hexylene carbonates provide competitive CO2 absorption performance, extending the applicability of the proposed concept to other CO2-derived cyclic carbonates. More importantly, the direct use of the CO2-rich cyclic carbonate stream as the reaction medium was experimentally validated without significant thermodynamic or kinetic limitations despite the high product concentration. The proposed concept achieves a competitive energy demand and CO2-related emissions while avoiding deep vacuum operation and intermediate solvent regeneration.\",\"PeriodicalId\":25,\"journal\":{\"name\":\"ACS Sustainable Chemistry & Engineering\",\"volume\":\"15 1\",\"pages\":\"\"},\"PeriodicalIF\":7.6000,\"publicationDate\":\"2026-10-13\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"ACS Sustainable Chemistry & Engineering\",\"FirstCategoryId\":\"92\",\"ListUrlMain\":\"https://doi.org/10.1021/acssuschemeng.6c08760\",\"RegionNum\":1,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"CHEMISTRY, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"ACS Sustainable Chemistry & Engineering","FirstCategoryId":"92","ListUrlMain":"https://doi.org/10.1021/acssuschemeng.6c08760","RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0

摘要

迫切需要为二氧化碳的捕获和利用制定节能的解决办法,因为目前的综合过程仍然受到捕获和转换阶段的兼容性的限制。本研究提出了一种新的产品驱动的碳捕获和利用概念,其中二氧化碳衍生的环状碳酸盐产品依次被用作物理二氧化碳吸附剂,随后作为其自身合成的反应介质,从而消除了中间溶剂再生步骤。实验测定了四种环状碳酸盐的密度、粘度和CO2溶解度,并以离子液体[bmim]I为催化剂,在具有代表性的综合工艺条件下进行了环加成反应。通过基于类导体筛选模型(COSMO)的/Aspen过程模拟和生命周期评估,对天然气净化的整个过程进行了评估。实验和计算结果表明,丙烯、丁烯和己烯碳酸盐具有竞争性的二氧化碳吸收性能,将所提出的概念扩展到其他二氧化碳衍生的环状碳酸盐。更重要的是,直接使用富含co2的循环碳酸盐流作为反应介质得到了实验验证,尽管产物浓度很高,但没有明显的热力学或动力学限制。提出的概念实现了具有竞争力的能源需求和二氧化碳相关排放,同时避免了深真空操作和中间溶剂再生。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

CO2-Product-Driven Integrated Carbon Capture and Utilization to Produce Cyclic Carbonates

CO2-Product-Driven Integrated Carbon Capture and Utilization to Produce Cyclic Carbonates
There is an urgent need to develop energy-efficient solutions for CO2 capture and utilization, because current integrated processes remain limited by the compatibility of the capture and conversion stages. This work proposes a novel product-driven carbon capture and utilization concept, in which the CO2-derived cyclic carbonate product is sequentially employed as a physical CO2 absorbent and subsequently as the reaction medium for its own synthesis, eliminating the intermediate solvent regeneration step. Density, viscosity, and CO2 solubility were experimentally determined for four cyclic carbonates, while cycloaddition reactions were performed under representative integrated process conditions using the ionic liquid [bmim]I as a catalyst. The complete process for natural gas purification was evaluated through conductor-like screening model (COSMO)-based/Aspen process simulation and life cycle assessment. Experimental and computational results demonstrate that propylene, butylene, and hexylene carbonates provide competitive CO2 absorption performance, extending the applicability of the proposed concept to other CO2-derived cyclic carbonates. More importantly, the direct use of the CO2-rich cyclic carbonate stream as the reaction medium was experimentally validated without significant thermodynamic or kinetic limitations despite the high product concentration. The proposed concept achieves a competitive energy demand and CO2-related emissions while avoiding deep vacuum operation and intermediate solvent regeneration.
求助全文
通过发布文献求助,成功后即可免费获取论文全文。 去求助
来源期刊
ACS Sustainable Chemistry & Engineering
ACS Sustainable Chemistry & Engineering CHEMISTRY, MULTIDISCIPLINARY-ENGINEERING, CHEMICAL
CiteScore
13.80
自引率
4.80%
发文量
1470
审稿时长
1.7 months
期刊介绍: ACS Sustainable Chemistry & Engineering is a prestigious weekly peer-reviewed scientific journal published by the American Chemical Society. Dedicated to advancing the principles of green chemistry and green engineering, it covers a wide array of research topics including green chemistry, green engineering, biomass, alternative energy, and life cycle assessment. The journal welcomes submissions in various formats, including Letters, Articles, Features, and Perspectives (Reviews), that address the challenges of sustainability in the chemical enterprise and contribute to the advancement of sustainable practices. Join us in shaping the future of sustainable chemistry and engineering.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
确定
请完成安全验证×
copy
已复制链接
快去分享给好友吧!
我知道了
右上角分享
点击右上角分享
0
联系我们:info@booksci.cn Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。 Copyright © 2023 布克学术 All rights reserved.
京ICP备2023020795号-1
ghs 京公网安备 11010802042870号
Book学术文献互助
Book学术文献互助群
群 号:604180095
Book学术官方微信
小红书