你的DES有多深?多组分混合物中理想共晶预测的数值框架

IF 2.4 3区 工程技术 Q3 CHEMISTRY, MULTIDISCIPLINARY
Journal of Chemical & Engineering Data Pub Date : 2026-10-08 Epub Date: 2026-09-03 DOI:10.1021/acs.jced.6c00332
Gabriela A. Nogueira, Leandro dos Santos Silva, Mario H. Gonzalez, Milton A. Faria Neto, Thiago A. L. Burgo
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引用次数: 0

摘要

在这里,我们提出了一种简单且计算效率高的方法来确定理想的二元、三元和高阶混合物的共晶温度,为评估深度共晶溶剂(DES)的行为提供了定量参考。在DES文献中,三元体系通常被简化为伪二元体系,通过固定两个组分的摩尔比,并且只沿固定的组成线(等线)改变第三个组分。虽然这减少了实验的工作量,但它限制了液相映射到单一的组成途径,并且可能无法识别全局理想共晶。相比之下,我们的实现解决了所有组分的经典理想液相方程,假设拉乌尔定律理想和纯的,互不混溶的固相。使用纯组分熔融温度和摩尔熔合焓,该方法可以实现多维液面映射。通过分析对称混合解决方案、独立的80位计算、MATLAB实现、排列测试、3,521个压力测试系统和发布的基准测试验证了寻根实现。所有的应力测试系统都趋于一致,并在0.7 K范围内重现了公布的理想共晶温度。对文献报道的二元和三元混合物的应用进一步表明,与全局共晶的比较结合了明显的局部热偏差和非负的理想成分惩罚。因此,该框架为多组分共晶筛选提供了透明和可扩展的理想平衡基线。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
How Deep is Your DES? A Numerical Framework for Ideal Eutectic Prediction in Multicomponent Mixtures

Here, we present a simple and computationally efficient procedure to determine the eutectic temperatures of ideal binary, ternary, and higher-order mixtures, providing a quantitative reference for evaluating deep eutectic solvent (DES) behavior. In the DES literature, ternary systems are often simplified as pseudo-binaries by fixing the molar ratio of two components and varying only the third along a fixed-composition line (isopleth). Although this reduces the experimental effort, it restricts liquidus mapping to a single compositional pathway and may fail to identify the global ideal eutectic. In contrast, our implementation solves the classical ideal liquidus equations for all components, assuming Raoult-law ideality and pure, mutually immiscible solid phases. Using pure-component melting temperatures and molar fusion enthalpies, the method enables multidimensional liquidus-surface mapping. The root-finding implementation was verified against analytical symmetric-mixture solutions, independent 80-digit calculations, a MATLAB implementation, permutation tests, 3,521 stress-test systems, and published benchmarks. All stress-test systems converged, and published ideal eutectic temperatures were reproduced within 0.7 K. Application to literature-reported binary and ternary mixtures further showed that comparison with the global ideal eutectic combines an apparent local thermal deviation with a nonnegative ideal-composition penalty. The framework therefore provides a transparent and extensible ideal-equilibrium baseline for multicomponent eutectic screening.

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来源期刊
Journal of Chemical & Engineering Data
Journal of Chemical & Engineering Data 工程技术-工程:化工
CiteScore
5.20
自引率
19.20%
发文量
324
审稿时长
2.2 months
期刊介绍: The Journal of Chemical & Engineering Data is a monthly journal devoted to the publication of data obtained from both experiment and computation, which are viewed as complementary. It is the only American Chemical Society journal primarily concerned with articles containing data on the phase behavior and the physical, thermodynamic, and transport properties of well-defined materials, including complex mixtures of known compositions. While environmental and biological samples are of interest, their compositions must be known and reproducible. As a result, adsorption on natural product materials does not generally fit within the scope of Journal of Chemical & Engineering Data.
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