{"title":"基于核磁共振NOE对距离测量的全原子核酸力场集成精确细化。","authors":"Hyeonjun Kim,Youngshang Pak","doi":"10.1021/acs.jctc.5c01075","DOIUrl":null,"url":null,"abstract":"Accurately modeling nucleic acid structure and dynamics remains challenging for all-atom simulations, especially for noncanonical motifs such as small loops and G-quadruplexes. Despite these advances, current all-atom classical force fields often fail to reproduce ensembles consistent with high-resolution experimental data. We present a systematic refinement strategy for AMBER-based force fields that incorporates nuclear Overhauser effect distance data from NMR experiments within an ensemble-averaged optimization framework. By selectively tuning van der Waals interaction pairs, this approach markedly reduces simulation-experiment discrepancies, removes persistent artifacts, and generates free energy landscapes that better reflect experimental observations. We demonstrate broad applicability across diverse DNA and RNA systems including flexible loops and G-quadruplexes. Overall, this transferable strategy significantly improves structural accuracy and predictive power, enabling more reliable modeling of complex nucleic acid conformational ensembles.","PeriodicalId":45,"journal":{"name":"Journal of Chemical Theory and Computation","volume":"45 1","pages":""},"PeriodicalIF":5.5000,"publicationDate":"2025-10-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Ensemble-Based Precision Refinement of All-Atom Nucleic Acid Force Fields Guided by NMR NOE Pair-Distance Measurements.\",\"authors\":\"Hyeonjun Kim,Youngshang Pak\",\"doi\":\"10.1021/acs.jctc.5c01075\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"Accurately modeling nucleic acid structure and dynamics remains challenging for all-atom simulations, especially for noncanonical motifs such as small loops and G-quadruplexes. Despite these advances, current all-atom classical force fields often fail to reproduce ensembles consistent with high-resolution experimental data. We present a systematic refinement strategy for AMBER-based force fields that incorporates nuclear Overhauser effect distance data from NMR experiments within an ensemble-averaged optimization framework. By selectively tuning van der Waals interaction pairs, this approach markedly reduces simulation-experiment discrepancies, removes persistent artifacts, and generates free energy landscapes that better reflect experimental observations. We demonstrate broad applicability across diverse DNA and RNA systems including flexible loops and G-quadruplexes. Overall, this transferable strategy significantly improves structural accuracy and predictive power, enabling more reliable modeling of complex nucleic acid conformational ensembles.\",\"PeriodicalId\":45,\"journal\":{\"name\":\"Journal of Chemical Theory and Computation\",\"volume\":\"45 1\",\"pages\":\"\"},\"PeriodicalIF\":5.5000,\"publicationDate\":\"2025-10-24\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Journal of Chemical Theory and Computation\",\"FirstCategoryId\":\"92\",\"ListUrlMain\":\"https://doi.org/10.1021/acs.jctc.5c01075\",\"RegionNum\":1,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"CHEMISTRY, PHYSICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Journal of Chemical Theory and Computation","FirstCategoryId":"92","ListUrlMain":"https://doi.org/10.1021/acs.jctc.5c01075","RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
Ensemble-Based Precision Refinement of All-Atom Nucleic Acid Force Fields Guided by NMR NOE Pair-Distance Measurements.
Accurately modeling nucleic acid structure and dynamics remains challenging for all-atom simulations, especially for noncanonical motifs such as small loops and G-quadruplexes. Despite these advances, current all-atom classical force fields often fail to reproduce ensembles consistent with high-resolution experimental data. We present a systematic refinement strategy for AMBER-based force fields that incorporates nuclear Overhauser effect distance data from NMR experiments within an ensemble-averaged optimization framework. By selectively tuning van der Waals interaction pairs, this approach markedly reduces simulation-experiment discrepancies, removes persistent artifacts, and generates free energy landscapes that better reflect experimental observations. We demonstrate broad applicability across diverse DNA and RNA systems including flexible loops and G-quadruplexes. Overall, this transferable strategy significantly improves structural accuracy and predictive power, enabling more reliable modeling of complex nucleic acid conformational ensembles.
期刊介绍:
The Journal of Chemical Theory and Computation invites new and original contributions with the understanding that, if accepted, they will not be published elsewhere. Papers reporting new theories, methodology, and/or important applications in quantum electronic structure, molecular dynamics, and statistical mechanics are appropriate for submission to this Journal. Specific topics include advances in or applications of ab initio quantum mechanics, density functional theory, design and properties of new materials, surface science, Monte Carlo simulations, solvation models, QM/MM calculations, biomolecular structure prediction, and molecular dynamics in the broadest sense including gas-phase dynamics, ab initio dynamics, biomolecular dynamics, and protein folding. The Journal does not consider papers that are straightforward applications of known methods including DFT and molecular dynamics. The Journal favors submissions that include advances in theory or methodology with applications to compelling problems.