基于裂化热解动力学机制和无监督双阶段注意长短期记忆网络的多策略建模

IF 7.7 2区 工程技术 Q1 CHEMISTRY, APPLIED
Bin Wang , Kai Luo , Xiangming Chen , Kai Deng , Jian Long , Wenze Guo
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引用次数: 0

摘要

双提升管反应器催化裂化工艺对石化企业的发展具有重要意义。它的目的是在增加产量的同时减少燃料消耗。因此,为生产过程建模是一项必不可少的任务。然而,传统方法难以准确描述裂化/热解双反应路径中复杂的反应机理。此外,由于变量的耦合和动态特征的不足,捕获多变量时空依赖关系仍然具有挑战性。本文重点研究了目标工艺流程核心反应-再生单元内的产品产率和碳排放等关键指标。为了平衡反应途径,建立了集总动力学机理模型。采用变分模态分解(VMD)对耦合变量进行分解。采用无监督双阶段注意长短期记忆模型(UDA-LSTM)捕捉多尺度特征。为了充分利用这些优势,本文设计了三种多目标预测协同优化的混合模型。最后,通过一个实际的工业生产案例验证了所提出的混合建模框架的有效性。主要产品产率的预测均方误差(MSE)不超过0.2,所构建的工艺模型支持炼油厂对生产过程的实时监控。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Multi-strategy modeling integrating kinetics mechanism of cracking and pyrolysis and unsupervised dual-stage attention long and short-term memory network
The fluid catalytic cracking process utilizing the dual-riser reactors (MIP-LTAG) holds significant importance in the development of petrochemical enterprises. It aims to reduce fuel consumption while increasing output. Consequently, modeling for the production process is an essential task. However, traditional methods struggle to accurately describe the complex reaction mechanisms involved in the cracking/pyrolysis dual reaction pathways. Additionally, due to the coupling of variables and insufficiency of dynamic characteristics, capturing multi-variable spatio-temporal dependencies remains challenging. This paper focuses on key indicators such as product yield and carbon emissions within the core reaction-regeneration unit of the target technological process. A lumped kinetic mechanism model is constructed to balance the reaction pathway. Variational mode decomposition (VMD) is employed to perform decomposition of the coupled variables. The unsupervised dual-stage attentional long short term memory model (UDA-LSTM) is utilized to capture multi-scale characteristics. To leverage these advantages, this paper designs three hybrid model for collaborative optimization of multi-objective predictions. Finally, the effectiveness of the proposed hybrid modeling framework is validated through an actual industrial production case. The predicted mean squared error (MSE) of the main product yield does not exceed 0.2, and the constructed process model supports real-time monitoring of the production process by refineries.
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来源期刊
Fuel Processing Technology
Fuel Processing Technology 工程技术-工程:化工
CiteScore
13.20
自引率
9.30%
发文量
398
审稿时长
26 days
期刊介绍: Fuel Processing Technology (FPT) deals with the scientific and technological aspects of converting fossil and renewable resources to clean fuels, value-added chemicals, fuel-related advanced carbon materials and by-products. In addition to the traditional non-nuclear fossil fuels, biomass and wastes, papers on the integration of renewables such as solar and wind energy and energy storage into the fuel processing processes, as well as papers on the production and conversion of non-carbon-containing fuels such as hydrogen and ammonia, are also welcome. While chemical conversion is emphasized, papers on advanced physical conversion processes are also considered for publication in FPT. Papers on the fundamental aspects of fuel structure and properties will also be considered.
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