非振动颗粒系统中强空间约束和逐步冷却的结晶过程

IF 3.1 3区 物理与天体物理 Q2 PHYSICS, MULTIDISCIPLINARY
A. Escobar, F. Donado
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引用次数: 0

摘要

研究了交变磁场流化二维磁性颗粒体系中强约束对结晶的影响,交变磁场的幅值可控制有效温度。颗粒系统包括球形磁性颗粒,这些磁性颗粒被限制在一个稍微倾斜的棱柱状盒子内,以产生产生颗粒沉降的能量梯度。使用了三种不同的几何形状:六角形、圆形和矩形。系统从流体状态开始,通过线性或逐步冷却进入固体状态。研究发现,与没有壁面空间约束的情况相比,约束减少了结晶时间,并且在使用逐步冷却剖面时发现了额外的减少。在无约束情况下,体系结晶为六方密排构型。相反,强空间约束对粒子的最终构型施加了极端的限制。六角形的容器倾向于六角形的紧密排列,而矩形单元则倾向于正方形的顺序,而圆形单元则倾向于形成一个堆叠在另一个上面的项链状结构。取向序参量和径向分布函数的结果证实了这些观测结果。随着容器尺寸的增加,墙壁对散装订货的影响减小,现在在所有情况下都主导着六边形密装订单。然而,结构中的缺陷比没有墙的结构要多。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Crystallization process under strong spatial confinement and stepwise cooling in a nonvibrating granular system
We study the effects of strong confinement on crystallization in a 2D-dimensional magnetic granular system fluidized by an alternating magnetic field whose amplitude controls the effective temperature. The granular system comprises spherical magnetic particles confined within a prismatic box slightly tilted to create an energy gradient that produces particle sedimentation. Three different geometries were used: hexagonal, circular, and rectangular. The systems start from a fluid state and go to a solid state by following a linear or stepwise cooling down. It is found that confinement reduces the crystallization time compared to the case of no spatial confinement by walls, and an additional reduction is found when using a stepwise cooling profile. In the unconfined case, the system crystallizes in the hexagonal close-packed configuration. In contrast, strong spatial confinement imposes extreme restrictions on the final configuration of the particles. While the hexagonal container favors the hexagonal close-packed arrangement, the rectangular cell imposes the square order, and the circular cell favors the formation of necklace-like structures piled one over the other. The results of the orientational order parameter and the radial distribution function corroborate these observations. As the container size increases, the effects of the walls on bulk ordering decrease, now dominating the hexagonal close-packed order in all cases. However, defects in the structure are more numerous than those without walls.
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来源期刊
CiteScore
7.20
自引率
9.10%
发文量
852
审稿时长
6.6 months
期刊介绍: Physica A: Statistical Mechanics and its Applications Recognized by the European Physical Society Physica A publishes research in the field of statistical mechanics and its applications. Statistical mechanics sets out to explain the behaviour of macroscopic systems by studying the statistical properties of their microscopic constituents. Applications of the techniques of statistical mechanics are widespread, and include: applications to physical systems such as solids, liquids and gases; applications to chemical and biological systems (colloids, interfaces, complex fluids, polymers and biopolymers, cell physics); and other interdisciplinary applications to for instance biological, economical and sociological systems.
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