Nurul Hidayat , Arif Hidayat , Latifatul Aisyah Nabila , Siti Azimatul Luthfiyyah , Ahmad Taufiq , Muhammad Safwan Abd Aziz , Hazri Bakhtiar
{"title":"激光锥形光纤与LSPR激活增强折射率传感","authors":"Nurul Hidayat , Arif Hidayat , Latifatul Aisyah Nabila , Siti Azimatul Luthfiyyah , Ahmad Taufiq , Muhammad Safwan Abd Aziz , Hazri Bakhtiar","doi":"10.1016/j.sna.2025.117181","DOIUrl":null,"url":null,"abstract":"<div><div>The integration of localized surface plasmon resonance (LSPR) effects with tapered optical fibers has significantly improved refractive index (RI) sensing performance. This study introduces an optimized RI sensor using gold nanospheres (AuNSs) coated on tapered coreless termination fibers (TCTFs), which demonstrate a remarkable improvement in sensitivity. The TCTFs were optimized in terms of their taper waist diameter through the variation of CO<sub>2</sub> laser power. Subsequently, 11.26 nm average-sized AuNSs synthesized by citrate reduction method were strongly attached to the optimized TCTF surface via thiol-functionalization. The LSPR peak of AuNSs, recorded by ultraviolet visible spectroscopy (UV-Vis), was ∼522 nm. The face-centered cubic crystal structure and nanospherical shapes of AuNSs were respectively obtained from X-ray diffraction (XRD) and high-resolution transmission electron microscopy (HR-TEM) data. Furthermore, from the field emission scanning electron microscopy (FE-SEM) image, the average thickness of the attached AuNSs on the TCTF was 88 nm. The sensitivity of the unmodified CTF sensor was 50.97 ± 4.68 nm/RIU and the AuNSs-coated TCTF was 254.42 ± 20.75 nm/RIU. In other words, it exhibited a ∼400 % improvement in RI sensitivity. Five repetitive measurements indicated that fluctuation of sensitivity was ±3.93 nm/RIU, indicating good repeatability. The stability test for 20 min showed that the sensor experienced small wavelength shift variations of ±0.362 nm for refractive indices of 1.33 and 1.39, and ±0.726 nm for refractive index of 1.43. These results established AuNSs-coated TCTFs as a promising platform for high-performance RI sensing applications.</div></div>","PeriodicalId":21689,"journal":{"name":"Sensors and Actuators A-physical","volume":"396 ","pages":"Article 117181"},"PeriodicalIF":4.9000,"publicationDate":"2025-10-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Laser-tapered optical fibers with LSPR activation for enhanced refractive index sensing\",\"authors\":\"Nurul Hidayat , Arif Hidayat , Latifatul Aisyah Nabila , Siti Azimatul Luthfiyyah , Ahmad Taufiq , Muhammad Safwan Abd Aziz , Hazri Bakhtiar\",\"doi\":\"10.1016/j.sna.2025.117181\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><div>The integration of localized surface plasmon resonance (LSPR) effects with tapered optical fibers has significantly improved refractive index (RI) sensing performance. This study introduces an optimized RI sensor using gold nanospheres (AuNSs) coated on tapered coreless termination fibers (TCTFs), which demonstrate a remarkable improvement in sensitivity. The TCTFs were optimized in terms of their taper waist diameter through the variation of CO<sub>2</sub> laser power. Subsequently, 11.26 nm average-sized AuNSs synthesized by citrate reduction method were strongly attached to the optimized TCTF surface via thiol-functionalization. The LSPR peak of AuNSs, recorded by ultraviolet visible spectroscopy (UV-Vis), was ∼522 nm. The face-centered cubic crystal structure and nanospherical shapes of AuNSs were respectively obtained from X-ray diffraction (XRD) and high-resolution transmission electron microscopy (HR-TEM) data. Furthermore, from the field emission scanning electron microscopy (FE-SEM) image, the average thickness of the attached AuNSs on the TCTF was 88 nm. The sensitivity of the unmodified CTF sensor was 50.97 ± 4.68 nm/RIU and the AuNSs-coated TCTF was 254.42 ± 20.75 nm/RIU. In other words, it exhibited a ∼400 % improvement in RI sensitivity. Five repetitive measurements indicated that fluctuation of sensitivity was ±3.93 nm/RIU, indicating good repeatability. The stability test for 20 min showed that the sensor experienced small wavelength shift variations of ±0.362 nm for refractive indices of 1.33 and 1.39, and ±0.726 nm for refractive index of 1.43. These results established AuNSs-coated TCTFs as a promising platform for high-performance RI sensing applications.</div></div>\",\"PeriodicalId\":21689,\"journal\":{\"name\":\"Sensors and Actuators A-physical\",\"volume\":\"396 \",\"pages\":\"Article 117181\"},\"PeriodicalIF\":4.9000,\"publicationDate\":\"2025-10-17\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Sensors and Actuators A-physical\",\"FirstCategoryId\":\"5\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S0924424725009872\",\"RegionNum\":3,\"RegionCategory\":\"工程技术\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"ENGINEERING, ELECTRICAL & ELECTRONIC\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Sensors and Actuators A-physical","FirstCategoryId":"5","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S0924424725009872","RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"ENGINEERING, ELECTRICAL & ELECTRONIC","Score":null,"Total":0}
Laser-tapered optical fibers with LSPR activation for enhanced refractive index sensing
The integration of localized surface plasmon resonance (LSPR) effects with tapered optical fibers has significantly improved refractive index (RI) sensing performance. This study introduces an optimized RI sensor using gold nanospheres (AuNSs) coated on tapered coreless termination fibers (TCTFs), which demonstrate a remarkable improvement in sensitivity. The TCTFs were optimized in terms of their taper waist diameter through the variation of CO2 laser power. Subsequently, 11.26 nm average-sized AuNSs synthesized by citrate reduction method were strongly attached to the optimized TCTF surface via thiol-functionalization. The LSPR peak of AuNSs, recorded by ultraviolet visible spectroscopy (UV-Vis), was ∼522 nm. The face-centered cubic crystal structure and nanospherical shapes of AuNSs were respectively obtained from X-ray diffraction (XRD) and high-resolution transmission electron microscopy (HR-TEM) data. Furthermore, from the field emission scanning electron microscopy (FE-SEM) image, the average thickness of the attached AuNSs on the TCTF was 88 nm. The sensitivity of the unmodified CTF sensor was 50.97 ± 4.68 nm/RIU and the AuNSs-coated TCTF was 254.42 ± 20.75 nm/RIU. In other words, it exhibited a ∼400 % improvement in RI sensitivity. Five repetitive measurements indicated that fluctuation of sensitivity was ±3.93 nm/RIU, indicating good repeatability. The stability test for 20 min showed that the sensor experienced small wavelength shift variations of ±0.362 nm for refractive indices of 1.33 and 1.39, and ±0.726 nm for refractive index of 1.43. These results established AuNSs-coated TCTFs as a promising platform for high-performance RI sensing applications.
期刊介绍:
Sensors and Actuators A: Physical brings together multidisciplinary interests in one journal entirely devoted to disseminating information on all aspects of research and development of solid-state devices for transducing physical signals. Sensors and Actuators A: Physical regularly publishes original papers, letters to the Editors and from time to time invited review articles within the following device areas:
• Fundamentals and Physics, such as: classification of effects, physical effects, measurement theory, modelling of sensors, measurement standards, measurement errors, units and constants, time and frequency measurement. Modeling papers should bring new modeling techniques to the field and be supported by experimental results.
• Materials and their Processing, such as: piezoelectric materials, polymers, metal oxides, III-V and II-VI semiconductors, thick and thin films, optical glass fibres, amorphous, polycrystalline and monocrystalline silicon.
• Optoelectronic sensors, such as: photovoltaic diodes, photoconductors, photodiodes, phototransistors, positron-sensitive photodetectors, optoisolators, photodiode arrays, charge-coupled devices, light-emitting diodes, injection lasers and liquid-crystal displays.
• Mechanical sensors, such as: metallic, thin-film and semiconductor strain gauges, diffused silicon pressure sensors, silicon accelerometers, solid-state displacement transducers, piezo junction devices, piezoelectric field-effect transducers (PiFETs), tunnel-diode strain sensors, surface acoustic wave devices, silicon micromechanical switches, solid-state flow meters and electronic flow controllers.
Etc...