{"title":"用于日盲和弱光成像的超灵敏超快自供电紫外光电探测器阵列。","authors":"Weilong Deng,Xiangyu Fan,Yuxuan Du,Shengyu Ma,Hanxu Zhang,Mengting Liu,Hao Zhang,Shuo Chen,Qiang Fu,Yumin Zhang,Yang Li,Siyu Han,Yang Wang,Tai Yao,Xianjie Wang,Bo Song","doi":"10.1002/adma.202514968","DOIUrl":null,"url":null,"abstract":"Self-powered ultraviolet (UV) photodetectors (PDs) based on wide bandgap semiconductors (WBGSs) and their heterostructures face challenges in ultrasensitive and ultrafast weak-light detection capabilities. In this work, an 8 × 8 UV photodetector array based on CuNiO2/SiC p-n heterojunctions is demonstrated to operate in both solar-blind and weak-light conditions. The device achieves a weak-light detection limit of 4.6 nW·mm-2, a fast response time of 45 ns, and a high responsivity of 104.2 mA·W-1 and a detectivity of 3.4 × 1012 Jones, outperforming self-powered UV PDs based on SiC and Ga2O3-based WBGSs and their heterostructures. This excellent performance of the device originates from the high interface quality, large built-in electric field, Fowler-Nordheim tunneling (FNT) of charge transport, and enhancing light absorption at the heterostructures. Moreover, the detector exhibits a low noise power density below 10-22 A2·Hz-1 and a high cutoff frequency of 5 kHz, enabling it to maintain high-contrast real-time reflection imaging capability under solar illumination.","PeriodicalId":114,"journal":{"name":"Advanced Materials","volume":"101 1","pages":"e14968"},"PeriodicalIF":26.8000,"publicationDate":"2025-10-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Ultrasensitive and Ultrafast Self-Powered Ultraviolet Photodetector Array for Solar-Blind and Weak-Light Imaging.\",\"authors\":\"Weilong Deng,Xiangyu Fan,Yuxuan Du,Shengyu Ma,Hanxu Zhang,Mengting Liu,Hao Zhang,Shuo Chen,Qiang Fu,Yumin Zhang,Yang Li,Siyu Han,Yang Wang,Tai Yao,Xianjie Wang,Bo Song\",\"doi\":\"10.1002/adma.202514968\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"Self-powered ultraviolet (UV) photodetectors (PDs) based on wide bandgap semiconductors (WBGSs) and their heterostructures face challenges in ultrasensitive and ultrafast weak-light detection capabilities. In this work, an 8 × 8 UV photodetector array based on CuNiO2/SiC p-n heterojunctions is demonstrated to operate in both solar-blind and weak-light conditions. The device achieves a weak-light detection limit of 4.6 nW·mm-2, a fast response time of 45 ns, and a high responsivity of 104.2 mA·W-1 and a detectivity of 3.4 × 1012 Jones, outperforming self-powered UV PDs based on SiC and Ga2O3-based WBGSs and their heterostructures. This excellent performance of the device originates from the high interface quality, large built-in electric field, Fowler-Nordheim tunneling (FNT) of charge transport, and enhancing light absorption at the heterostructures. Moreover, the detector exhibits a low noise power density below 10-22 A2·Hz-1 and a high cutoff frequency of 5 kHz, enabling it to maintain high-contrast real-time reflection imaging capability under solar illumination.\",\"PeriodicalId\":114,\"journal\":{\"name\":\"Advanced Materials\",\"volume\":\"101 1\",\"pages\":\"e14968\"},\"PeriodicalIF\":26.8000,\"publicationDate\":\"2025-10-17\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Advanced Materials\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://doi.org/10.1002/adma.202514968\",\"RegionNum\":1,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"CHEMISTRY, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Advanced Materials","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1002/adma.202514968","RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
Ultrasensitive and Ultrafast Self-Powered Ultraviolet Photodetector Array for Solar-Blind and Weak-Light Imaging.
Self-powered ultraviolet (UV) photodetectors (PDs) based on wide bandgap semiconductors (WBGSs) and their heterostructures face challenges in ultrasensitive and ultrafast weak-light detection capabilities. In this work, an 8 × 8 UV photodetector array based on CuNiO2/SiC p-n heterojunctions is demonstrated to operate in both solar-blind and weak-light conditions. The device achieves a weak-light detection limit of 4.6 nW·mm-2, a fast response time of 45 ns, and a high responsivity of 104.2 mA·W-1 and a detectivity of 3.4 × 1012 Jones, outperforming self-powered UV PDs based on SiC and Ga2O3-based WBGSs and their heterostructures. This excellent performance of the device originates from the high interface quality, large built-in electric field, Fowler-Nordheim tunneling (FNT) of charge transport, and enhancing light absorption at the heterostructures. Moreover, the detector exhibits a low noise power density below 10-22 A2·Hz-1 and a high cutoff frequency of 5 kHz, enabling it to maintain high-contrast real-time reflection imaging capability under solar illumination.
期刊介绍:
Advanced Materials, one of the world's most prestigious journals and the foundation of the Advanced portfolio, is the home of choice for best-in-class materials science for more than 30 years. Following this fast-growing and interdisciplinary field, we are considering and publishing the most important discoveries on any and all materials from materials scientists, chemists, physicists, engineers as well as health and life scientists and bringing you the latest results and trends in modern materials-related research every week.