{"title":"极简集成,超薄,可扩展的热光学接口设计,用于环境上方冷却","authors":"Renhao Ding, Shuangjiang Feng, Zezhou Wu, Fan Fan, Huajie Tang, Chengyue Guo, Qixiang Chen, Decheng Kong, Dongliang Zhao","doi":"10.1016/j.nanoen.2025.111524","DOIUrl":null,"url":null,"abstract":"Radiative cooling (RC) exhibits substantial potential for energy conservation and sustainable development, leveraging its dual mechanism of sunlight reflection and passive thermal emission to deep space without consuming any energy. However, RC remains a fundamental challenge for objects with substantial self-generated heat and operating above ambient temperature in both indoor and outdoor environments (e.g., electronic devices and communication base stations). To address this limitation, this work proposes an integrated and ultrathin thermal photonic interface (TPI) through thermo-optical design, which incorporates 2D hexagonal boron nitride (<em>h</em>-BN) nanoplates with high backward scattering efficiency into a polymer/metal oxide RC framework. The optimized TPI demonstrates exceptional solar reflectivity (>93%) and mid-infrared emissivity (96%). Indoors under high thermal loading, the object coated with the TPI demonstrates temperatures 11.5 °C and 13.2 °C lower than the commercial paint and polymer matrix systems, respectively. Additionally, under daytime with high thermal loading in summer, the TPI system maintains temperatures 5-8 °C below the other two. Notably, the TPI demonstrates excellent cooling performance above the ambient temperature. This work establishes a scalable design strategy for above-ambient radiative coolers, offering an innovative paradigm for implementing 2D planar materials to RC applications.","PeriodicalId":394,"journal":{"name":"Nano Energy","volume":"25 1","pages":""},"PeriodicalIF":17.1000,"publicationDate":"2025-10-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Minimalist integrated, ultrathin, scalable design of thermo-optical interfaces for above-ambient cooling\",\"authors\":\"Renhao Ding, Shuangjiang Feng, Zezhou Wu, Fan Fan, Huajie Tang, Chengyue Guo, Qixiang Chen, Decheng Kong, Dongliang Zhao\",\"doi\":\"10.1016/j.nanoen.2025.111524\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"Radiative cooling (RC) exhibits substantial potential for energy conservation and sustainable development, leveraging its dual mechanism of sunlight reflection and passive thermal emission to deep space without consuming any energy. However, RC remains a fundamental challenge for objects with substantial self-generated heat and operating above ambient temperature in both indoor and outdoor environments (e.g., electronic devices and communication base stations). To address this limitation, this work proposes an integrated and ultrathin thermal photonic interface (TPI) through thermo-optical design, which incorporates 2D hexagonal boron nitride (<em>h</em>-BN) nanoplates with high backward scattering efficiency into a polymer/metal oxide RC framework. The optimized TPI demonstrates exceptional solar reflectivity (>93%) and mid-infrared emissivity (96%). Indoors under high thermal loading, the object coated with the TPI demonstrates temperatures 11.5 °C and 13.2 °C lower than the commercial paint and polymer matrix systems, respectively. Additionally, under daytime with high thermal loading in summer, the TPI system maintains temperatures 5-8 °C below the other two. Notably, the TPI demonstrates excellent cooling performance above the ambient temperature. This work establishes a scalable design strategy for above-ambient radiative coolers, offering an innovative paradigm for implementing 2D planar materials to RC applications.\",\"PeriodicalId\":394,\"journal\":{\"name\":\"Nano Energy\",\"volume\":\"25 1\",\"pages\":\"\"},\"PeriodicalIF\":17.1000,\"publicationDate\":\"2025-10-13\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Nano Energy\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://doi.org/10.1016/j.nanoen.2025.111524\",\"RegionNum\":1,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"CHEMISTRY, PHYSICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Nano Energy","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1016/j.nanoen.2025.111524","RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
Minimalist integrated, ultrathin, scalable design of thermo-optical interfaces for above-ambient cooling
Radiative cooling (RC) exhibits substantial potential for energy conservation and sustainable development, leveraging its dual mechanism of sunlight reflection and passive thermal emission to deep space without consuming any energy. However, RC remains a fundamental challenge for objects with substantial self-generated heat and operating above ambient temperature in both indoor and outdoor environments (e.g., electronic devices and communication base stations). To address this limitation, this work proposes an integrated and ultrathin thermal photonic interface (TPI) through thermo-optical design, which incorporates 2D hexagonal boron nitride (h-BN) nanoplates with high backward scattering efficiency into a polymer/metal oxide RC framework. The optimized TPI demonstrates exceptional solar reflectivity (>93%) and mid-infrared emissivity (96%). Indoors under high thermal loading, the object coated with the TPI demonstrates temperatures 11.5 °C and 13.2 °C lower than the commercial paint and polymer matrix systems, respectively. Additionally, under daytime with high thermal loading in summer, the TPI system maintains temperatures 5-8 °C below the other two. Notably, the TPI demonstrates excellent cooling performance above the ambient temperature. This work establishes a scalable design strategy for above-ambient radiative coolers, offering an innovative paradigm for implementing 2D planar materials to RC applications.
期刊介绍:
Nano Energy is a multidisciplinary, rapid-publication forum of original peer-reviewed contributions on the science and engineering of nanomaterials and nanodevices used in all forms of energy harvesting, conversion, storage, utilization and policy. Through its mixture of articles, reviews, communications, research news, and information on key developments, Nano Energy provides a comprehensive coverage of this exciting and dynamic field which joins nanoscience and nanotechnology with energy science. The journal is relevant to all those who are interested in nanomaterials solutions to the energy problem.
Nano Energy publishes original experimental and theoretical research on all aspects of energy-related research which utilizes nanomaterials and nanotechnology. Manuscripts of four types are considered: review articles which inform readers of the latest research and advances in energy science; rapid communications which feature exciting research breakthroughs in the field; full-length articles which report comprehensive research developments; and news and opinions which comment on topical issues or express views on the developments in related fields.