高效吸附剂对柴油机尾气CO2吸附性能的评价——实验研究

IF 3 4区 环境科学与生态学 Q2 ENVIRONMENTAL SCIENCES
Maniarasu Ravi
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引用次数: 0

摘要

二氧化碳(CO2)是一种重要的人工温室气体(ghg),它给当今的地球带来了复杂的麻烦。由于化石燃料的消耗,排放到环境中的二氧化碳量增加,地球表面平均温度上升和灾难性气候变化的可能性极大。就研究而言,试图抑制主要单点贡献者的二氧化碳,例如(a)内燃机(IC)发动机,(b)移动发电机系统和(c)分散的发电装置。通过捕获燃烧后的二氧化碳,已经开展了一些研究,以尽量减少内燃机和乘用车的二氧化碳排放。农业基捕获材料已被探索作为一种吸附剂,用于从测试发动机的排气单元隔离二氧化碳污染物。三种潜在的农业基二氧化碳捕获材料,包括(i)棕榈壳,(ii)大麦秸秆和(iii)玉米芯,用于本实验研究的捕获系统中,以捕获来自测试发动机的污染物。通过将一个充满吸附剂的捕集装置连接到测试发动机上,探索了三种吸附剂的吸附效率。捕集装置采用变温吸附(TSA)再生技术对使用过的吸附剂进行再生。多次利用循环吸附和解吸效率来测试再生吸附剂的吸附能力。吸附剂样品的吸附能力是通过多次实验确定的。在TSA操作过程中,被吸附的气体组分从吸附剂表面释放出来,再次获得并收集在一个圆筒中。对收集到的吸附气进一步进行气相色谱-质谱(GC-MS)表征,以估计和确定吸附剂样品的气体吸收峰。实验工作的结果被处理并在当前的研究中提出。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Assessment of CO2 Adsorption by Using Efficient Adsorbents in a CI Engine Exhaust-An Experimental Study

Assessment of CO2 Adsorption by Using Efficient Adsorbents in a CI Engine Exhaust-An Experimental Study

Carbon dioxide (CO2) is one of the significant artificial greenhouse gases (GHGs) that produces complex trouble facing the Earth’s planet today. The volume of CO2 discharged into the environment as a consequence of the consumption of fossil fuels rises, and there is a tremendous potential for increasing the average Earth’s surface temperature and catastrophic climate change. Regarding the research, attempts are made to curb CO2 from primary single-point contributors, such as (a) internal combustion (IC) engines, (b) mobile generator systems, and (c) dispersed power production units. By capturing CO2 after combustion, some research has been carried out on minimizing CO2 emissions in IC engines and passenger vehicles. Agro-based capture material has been explored as an adsorbent for sequestrating CO2 pollutants from a test engine’s exhaust unit. Three potential agro-based CO2 capture materials, including (i) palm shell, (ii) barley straw, and (iii) corn cob, are used in the capture system of this experimental investigation to trap the pollutants from the test engine. The adsorption efficiency of the three adsorbents is explored by linking a capture unit filled with adsorbents to the test engine. Temperature Swing Adsorption (TSA) regeneration technique is employed in the capture unit to renew the used adsorbents. They are utilized several times to assess cyclic adsorption and desorption efficiency to test the adsorption capacity of the regenerated adsorbents. The adsorption capability of the adsorbent samples is determined over multiple experiments. The adsorbed gas components get liberated from the adsorbent’s surface during TSA operation, which is once more acquired and collected in a cylinder. The collected adsorbed gas is further analyzed in Gas Chromatography-Mass Spectroscopy (GC–MS) characterization to estimate and ascertain the gas uptake peaks of the adsorbent samples. The findings of the experimental work are addressed and presented in the current study.

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来源期刊
Water, Air, & Soil Pollution
Water, Air, & Soil Pollution 环境科学-环境科学
CiteScore
4.50
自引率
6.90%
发文量
448
审稿时长
2.6 months
期刊介绍: Water, Air, & Soil Pollution is an international, interdisciplinary journal on all aspects of pollution and solutions to pollution in the biosphere. This includes chemical, physical and biological processes affecting flora, fauna, water, air and soil in relation to environmental pollution. Because of its scope, the subject areas are diverse and include all aspects of pollution sources, transport, deposition, accumulation, acid precipitation, atmospheric pollution, metals, aquatic pollution including marine pollution and ground water, waste water, pesticides, soil pollution, sewage, sediment pollution, forestry pollution, effects of pollutants on humans, vegetation, fish, aquatic species, micro-organisms, and animals, environmental and molecular toxicology applied to pollution research, biosensors, global and climate change, ecological implications of pollution and pollution models. Water, Air, & Soil Pollution also publishes manuscripts on novel methods used in the study of environmental pollutants, environmental toxicology, environmental biology, novel environmental engineering related to pollution, biodiversity as influenced by pollution, novel environmental biotechnology as applied to pollution (e.g. bioremediation), environmental modelling and biorestoration of polluted environments. Articles should not be submitted that are of local interest only and do not advance international knowledge in environmental pollution and solutions to pollution. Articles that simply replicate known knowledge or techniques while researching a local pollution problem will normally be rejected without review. Submitted articles must have up-to-date references, employ the correct experimental replication and statistical analysis, where needed and contain a significant contribution to new knowledge. The publishing and editorial team sincerely appreciate your cooperation. Water, Air, & Soil Pollution publishes research papers; review articles; mini-reviews; and book reviews.
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