{"title":"流化床的非线性动力学:来自耦合CFD-DEM模拟的见解","authors":"Subi Nath, Shantanu Roy","doi":"10.1016/j.cej.2025.169452","DOIUrl":null,"url":null,"abstract":"Accurately capturing the highly nonlinear gas-solid interactions within fluidized beds remains a formidable challenge, critically hindering their robust design and optimization for industrial applications. Conventional numerical characterization methods often focus only on time-averaged data, failing to resolve the inherent dynamic complexities governing these systems. This study proposes an integrated approach, combining Computational Fluid Dynamics - Discrete Element Method (CFD-DEM) simulations with advanced nonlinear dynamics analysis, to comprehensively elucidate the true dynamic characteristics of both monodisperse and polydisperse gas-solid fluidized beds.We systematically investigated dynamic pressure and solids distribution fluctuations extracted from high-fidelity CFD-DEM simulations across varying superficial gas velocities, compositional variations, probe positions, and aspect ratios. Employing tools from nonlinear dynamics theory, this analysis rigorously unveiled the intrinsic nonlinearity of fluidized beds, confirming their profound sensitivity to initial conditions and complex, unpredictable behavior. Specifically, Kolmogorov Entropy, quantifying information loss and system unpredictability, and Correlation Dimension, measuring system complexity and degrees of freedom, were precisely quantified. These robust metrics provided unprecedented, nuanced insights into fluidization regime transitions, the critical influence of polydispersity on dynamic behavior, the intricate dynamics of bubble formation and interaction, and the precise identification of highly chaotic regions within the bed.This study significantly advances the understanding of fluidized bed dynamic characteristics by introducing a robust methodology that transcends conventional reliance on averaged properties. The integration of CFD–DEM with nonlinear dynamics analysis demonstrates high efficacy, yielding robust, data-driven insights crucial for optimizing reactor design and enhancing operational control. Furthermore, by successfully capturing dynamic profiles, this combined approach establishes a strong foundation for rigorous investigations into the scale-up of fluidized bed reactors, delineating a clear trajectory for future research.","PeriodicalId":270,"journal":{"name":"Chemical Engineering Journal","volume":"114 1","pages":""},"PeriodicalIF":13.2000,"publicationDate":"2025-10-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Non-linear dynamics of fluidized beds: Insights from coupled CFD-DEM simulations\",\"authors\":\"Subi Nath, Shantanu Roy\",\"doi\":\"10.1016/j.cej.2025.169452\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"Accurately capturing the highly nonlinear gas-solid interactions within fluidized beds remains a formidable challenge, critically hindering their robust design and optimization for industrial applications. Conventional numerical characterization methods often focus only on time-averaged data, failing to resolve the inherent dynamic complexities governing these systems. This study proposes an integrated approach, combining Computational Fluid Dynamics - Discrete Element Method (CFD-DEM) simulations with advanced nonlinear dynamics analysis, to comprehensively elucidate the true dynamic characteristics of both monodisperse and polydisperse gas-solid fluidized beds.We systematically investigated dynamic pressure and solids distribution fluctuations extracted from high-fidelity CFD-DEM simulations across varying superficial gas velocities, compositional variations, probe positions, and aspect ratios. Employing tools from nonlinear dynamics theory, this analysis rigorously unveiled the intrinsic nonlinearity of fluidized beds, confirming their profound sensitivity to initial conditions and complex, unpredictable behavior. Specifically, Kolmogorov Entropy, quantifying information loss and system unpredictability, and Correlation Dimension, measuring system complexity and degrees of freedom, were precisely quantified. These robust metrics provided unprecedented, nuanced insights into fluidization regime transitions, the critical influence of polydispersity on dynamic behavior, the intricate dynamics of bubble formation and interaction, and the precise identification of highly chaotic regions within the bed.This study significantly advances the understanding of fluidized bed dynamic characteristics by introducing a robust methodology that transcends conventional reliance on averaged properties. The integration of CFD–DEM with nonlinear dynamics analysis demonstrates high efficacy, yielding robust, data-driven insights crucial for optimizing reactor design and enhancing operational control. Furthermore, by successfully capturing dynamic profiles, this combined approach establishes a strong foundation for rigorous investigations into the scale-up of fluidized bed reactors, delineating a clear trajectory for future research.\",\"PeriodicalId\":270,\"journal\":{\"name\":\"Chemical Engineering Journal\",\"volume\":\"114 1\",\"pages\":\"\"},\"PeriodicalIF\":13.2000,\"publicationDate\":\"2025-10-10\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Chemical Engineering Journal\",\"FirstCategoryId\":\"5\",\"ListUrlMain\":\"https://doi.org/10.1016/j.cej.2025.169452\",\"RegionNum\":1,\"RegionCategory\":\"工程技术\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"ENGINEERING, CHEMICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Chemical Engineering Journal","FirstCategoryId":"5","ListUrlMain":"https://doi.org/10.1016/j.cej.2025.169452","RegionNum":1,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"ENGINEERING, CHEMICAL","Score":null,"Total":0}
Non-linear dynamics of fluidized beds: Insights from coupled CFD-DEM simulations
Accurately capturing the highly nonlinear gas-solid interactions within fluidized beds remains a formidable challenge, critically hindering their robust design and optimization for industrial applications. Conventional numerical characterization methods often focus only on time-averaged data, failing to resolve the inherent dynamic complexities governing these systems. This study proposes an integrated approach, combining Computational Fluid Dynamics - Discrete Element Method (CFD-DEM) simulations with advanced nonlinear dynamics analysis, to comprehensively elucidate the true dynamic characteristics of both monodisperse and polydisperse gas-solid fluidized beds.We systematically investigated dynamic pressure and solids distribution fluctuations extracted from high-fidelity CFD-DEM simulations across varying superficial gas velocities, compositional variations, probe positions, and aspect ratios. Employing tools from nonlinear dynamics theory, this analysis rigorously unveiled the intrinsic nonlinearity of fluidized beds, confirming their profound sensitivity to initial conditions and complex, unpredictable behavior. Specifically, Kolmogorov Entropy, quantifying information loss and system unpredictability, and Correlation Dimension, measuring system complexity and degrees of freedom, were precisely quantified. These robust metrics provided unprecedented, nuanced insights into fluidization regime transitions, the critical influence of polydispersity on dynamic behavior, the intricate dynamics of bubble formation and interaction, and the precise identification of highly chaotic regions within the bed.This study significantly advances the understanding of fluidized bed dynamic characteristics by introducing a robust methodology that transcends conventional reliance on averaged properties. The integration of CFD–DEM with nonlinear dynamics analysis demonstrates high efficacy, yielding robust, data-driven insights crucial for optimizing reactor design and enhancing operational control. Furthermore, by successfully capturing dynamic profiles, this combined approach establishes a strong foundation for rigorous investigations into the scale-up of fluidized bed reactors, delineating a clear trajectory for future research.
期刊介绍:
The Chemical Engineering Journal is an international research journal that invites contributions of original and novel fundamental research. It aims to provide an international platform for presenting original fundamental research, interpretative reviews, and discussions on new developments in chemical engineering. The journal welcomes papers that describe novel theory and its practical application, as well as those that demonstrate the transfer of techniques from other disciplines. It also welcomes reports on carefully conducted experimental work that is soundly interpreted. The main focus of the journal is on original and rigorous research results that have broad significance. The Catalysis section within the Chemical Engineering Journal focuses specifically on Experimental and Theoretical studies in the fields of heterogeneous catalysis, molecular catalysis, and biocatalysis. These studies have industrial impact on various sectors such as chemicals, energy, materials, foods, healthcare, and environmental protection.