固废基硫铝酸钙水泥强度影响因素的数据驱动分析

IF 7.3 1区 化学 Q1 CHEMISTRY, MULTIDISCIPLINARY
Jiahao Li, , , Xujiang Wang*, , , Xiang Lin, , , Xinshun Xu, , , Deqiang Sun, , , Yonggang Yao, , , Jingwei Li, , , Yanpeng Mao, , and , Wenlong Wang, 
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引用次数: 0

摘要

硫铝酸钙水泥(CSA)可以利用高比例的工业固体废物生产,为建材行业向低碳成分转型提供了一条很有前景的途径。然而,这类废料组成复杂多变,严重影响了CSA的性能,从而限制了其广泛应用。为了解决这一限制,本研究采用机器学习(ML)技术对影响固体废物基CSA强度的因素进行数据驱动分析。研究了从原料制备到膏体形成的关键参数。采用人工神经网络(ANN)、支持向量机(SVM)、随机森林(RF)、自适应增强(AdaBoost)、梯度增强决策树(GBDT)和极限梯度增强(XGBoost)等多种ML模型预测CSA的抗压强度。应用SHapley加性解释(SHAP)分析来解释各特征的贡献。结果表明,集成模型总体上优于传统模型,其中XGBoost模型表现出更好的性能(训练R2 = 0.99,测试R2 = 0.96),预测误差主要在±5 MPa以内。特征重要性分析发现,影响铝硅比(N)、铝铁比(Al/Fe)、焙烧温度、石膏含量、铝硫比(P)、碱度系数(Cm)是影响铝硅比(Al/Fe)的主要因素。延长养护龄期、增加N和添加石膏均可提高抗压强度,而增加P、Cm、煅烧时间和水灰比(W/C)对抗压强度有不利影响。此外,样本聚类可以识别特定特征的最佳范围。本研究采用的数据驱动和可解释的方法有望促进基于固体废物的CSA抗压强度的快速评估,并支持性能优化策略。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Data-Driven Analysis of Strength-Influencing Factors in Solid-Waste-Based Calcium Sulfoaluminate Cement

Data-Driven Analysis of Strength-Influencing Factors in Solid-Waste-Based Calcium Sulfoaluminate Cement

Data-Driven Analysis of Strength-Influencing Factors in Solid-Waste-Based Calcium Sulfoaluminate Cement

Calcium sulfoaluminate cement (CSA), which can be produced with a high proportion of industrial solid waste, presents a promising pathway for the transition of the building materials industry to low-carbon components. However, the complex and variable composition of such waste materials significantly influences the performance of CSA, thereby limiting its widespread application. To address this limitation, this study employed machine-learning (ML) techniques to perform a data-driven analysis of the factors affecting the strength of solid-waste-based CSA. Key parameters from raw material preparation to paste formation were investigated. Multiple ML models, including Artificial Neural Network (ANN), Support Vector Machine (SVM), Random Forest (RF), Adaptive Boosting (AdaBoost), Gradient Boosting Decision Tree (GBDT), and eXtreme Gradient Boosting (XGBoost), were employed to predict the compressive strength of CSA. SHapley Additive exPlanations (SHAP) analysis was applied to interpret the contribution of each feature. The results show that ensemble models generally outperform traditional ones, with the XGBoost model demonstrating superior performance (R2 = 0.99 for training and 0.96 for testing) and prediction errors predominantly falling within ±5 MPa. Feature importance analysis identified curing age, Al/Fe ratio, and aluminum–silicon ratio (N) as the most influential factors, followed by calcination temperature, gypsum content, aluminum–sulfur ratio (P), and alkalinity coefficient (Cm). Extending the curing age, increasing N, and adding gypsum were found to enhance compressive strength, whereas increasing P, Cm, calcination time, and the water-to-cement ratio (W/C) negatively affected strength. Furthermore, sample clustering enabled the identification of optimal ranges for specific features. The data-driven and interpretable approach adopted in this study is expected to facilitate rapid evaluation of the compressive strength of solid-waste-based CSA and to support performance optimization strategies.

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来源期刊
ACS Sustainable Chemistry & Engineering
ACS Sustainable Chemistry & Engineering CHEMISTRY, MULTIDISCIPLINARY-ENGINEERING, CHEMICAL
CiteScore
13.80
自引率
4.80%
发文量
1470
审稿时长
1.7 months
期刊介绍: ACS Sustainable Chemistry & Engineering is a prestigious weekly peer-reviewed scientific journal published by the American Chemical Society. Dedicated to advancing the principles of green chemistry and green engineering, it covers a wide array of research topics including green chemistry, green engineering, biomass, alternative energy, and life cycle assessment. The journal welcomes submissions in various formats, including Letters, Articles, Features, and Perspectives (Reviews), that address the challenges of sustainability in the chemical enterprise and contribute to the advancement of sustainable practices. Join us in shaping the future of sustainable chemistry and engineering.
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