Friday Junior Owuna, , , Antonin Chapoy*, , , Pezhman Ahmadi, , and , Rod Burgass,
{"title":"富氢天然气混合物(xH2 = 0,5,20,50和80%)的粘度从223到323 K,高达30 MPa","authors":"Friday Junior Owuna, , , Antonin Chapoy*, , , Pezhman Ahmadi, , and , Rod Burgass, ","doi":"10.1021/acs.jced.5c00401","DOIUrl":null,"url":null,"abstract":"<p >Natural gas (NG) transmission networks have been recognized as a cost-effective strategy for the distribution of hydrogen (H<sub>2</sub>). Thermophysical properties of H<sub>2</sub>-enriched NG are critical to the design and operations of these mixtures. Viscosities of H<sub>2</sub>-enriched NG mixtures (with H<sub>2</sub> mol % values of 0, 5, 20, 50, and 80) were measured at temperatures from 223 to 323 K and pressures up to 30 MPa using a capillary tube viscometer. The measured viscosity data were evaluated against the predictions of a residual entropy scaling (SRES) method, the corresponding states using molecular dynamic simulations of Lennard-Jones fluids, a one-fluid reference corresponding states model (Pedersen), and an extended corresponding state SUPERTRAPP model. All the models were adequate for predicting the measured viscosities. This work contributes accurate viscosity data for H<sub>2</sub>-enriched NG blends and enhances the understanding of the blends’ properties, which enable modification to the NG distribution facilities to accommodate H<sub>2</sub> transportation.</p>","PeriodicalId":42,"journal":{"name":"Journal of Chemical & Engineering Data","volume":"70 10","pages":"3990–4005"},"PeriodicalIF":2.1000,"publicationDate":"2025-09-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/pdf/10.1021/acs.jced.5c00401","citationCount":"0","resultStr":"{\"title\":\"Viscosity of Hydrogen-Enriched Natural Gas Blends (xH2 = 0, 5, 20, 50, and 80%) from 223 to 323 K and up to 30 MPa\",\"authors\":\"Friday Junior Owuna, , , Antonin Chapoy*, , , Pezhman Ahmadi, , and , Rod Burgass, \",\"doi\":\"10.1021/acs.jced.5c00401\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p >Natural gas (NG) transmission networks have been recognized as a cost-effective strategy for the distribution of hydrogen (H<sub>2</sub>). Thermophysical properties of H<sub>2</sub>-enriched NG are critical to the design and operations of these mixtures. Viscosities of H<sub>2</sub>-enriched NG mixtures (with H<sub>2</sub> mol % values of 0, 5, 20, 50, and 80) were measured at temperatures from 223 to 323 K and pressures up to 30 MPa using a capillary tube viscometer. The measured viscosity data were evaluated against the predictions of a residual entropy scaling (SRES) method, the corresponding states using molecular dynamic simulations of Lennard-Jones fluids, a one-fluid reference corresponding states model (Pedersen), and an extended corresponding state SUPERTRAPP model. All the models were adequate for predicting the measured viscosities. This work contributes accurate viscosity data for H<sub>2</sub>-enriched NG blends and enhances the understanding of the blends’ properties, which enable modification to the NG distribution facilities to accommodate H<sub>2</sub> transportation.</p>\",\"PeriodicalId\":42,\"journal\":{\"name\":\"Journal of Chemical & Engineering Data\",\"volume\":\"70 10\",\"pages\":\"3990–4005\"},\"PeriodicalIF\":2.1000,\"publicationDate\":\"2025-09-05\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"https://pubs.acs.org/doi/pdf/10.1021/acs.jced.5c00401\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Journal of Chemical & Engineering Data\",\"FirstCategoryId\":\"1\",\"ListUrlMain\":\"https://pubs.acs.org/doi/10.1021/acs.jced.5c00401\",\"RegionNum\":3,\"RegionCategory\":\"工程技术\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q3\",\"JCRName\":\"CHEMISTRY, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Journal of Chemical & Engineering Data","FirstCategoryId":"1","ListUrlMain":"https://pubs.acs.org/doi/10.1021/acs.jced.5c00401","RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
Viscosity of Hydrogen-Enriched Natural Gas Blends (xH2 = 0, 5, 20, 50, and 80%) from 223 to 323 K and up to 30 MPa
Natural gas (NG) transmission networks have been recognized as a cost-effective strategy for the distribution of hydrogen (H2). Thermophysical properties of H2-enriched NG are critical to the design and operations of these mixtures. Viscosities of H2-enriched NG mixtures (with H2 mol % values of 0, 5, 20, 50, and 80) were measured at temperatures from 223 to 323 K and pressures up to 30 MPa using a capillary tube viscometer. The measured viscosity data were evaluated against the predictions of a residual entropy scaling (SRES) method, the corresponding states using molecular dynamic simulations of Lennard-Jones fluids, a one-fluid reference corresponding states model (Pedersen), and an extended corresponding state SUPERTRAPP model. All the models were adequate for predicting the measured viscosities. This work contributes accurate viscosity data for H2-enriched NG blends and enhances the understanding of the blends’ properties, which enable modification to the NG distribution facilities to accommodate H2 transportation.
期刊介绍:
The Journal of Chemical & Engineering Data is a monthly journal devoted to the publication of data obtained from both experiment and computation, which are viewed as complementary. It is the only American Chemical Society journal primarily concerned with articles containing data on the phase behavior and the physical, thermodynamic, and transport properties of well-defined materials, including complex mixtures of known compositions. While environmental and biological samples are of interest, their compositions must be known and reproducible. As a result, adsorption on natural product materials does not generally fit within the scope of Journal of Chemical & Engineering Data.