Xiaoyu Chen, Biruk Teka Gidreta, Tanner Gaw, Michal Remer, Dan Daniel, Xiaoguang Wang, Solomon Adera
{"title":"滴摩擦的纹理润滑剂涂层表面","authors":"Xiaoyu Chen, Biruk Teka Gidreta, Tanner Gaw, Michal Remer, Dan Daniel, Xiaoguang Wang, Solomon Adera","doi":"10.1021/acsami.5c08905","DOIUrl":null,"url":null,"abstract":"Understanding drop friction on textured surfaces has implications in microfluidics and lab-on-a-chip devices. In this work, we investigated the drop friction on lubricant-coated pillars by systematically varying pillar height and density. First, we measured the friction force on a moving drop using a cantilever force sensor that has ±0.1 μN sensitivity. This measurement shows that drop friction on tall dense pillars is comparable to drop friction on short pillars, a significant result that suggests the presence of a Landau–Levich–Derjaguin (LLD) film underneath the moving drop. Second, we validated the force measurement by estimating the lubricant layer thickness by using white-light interferometry. Third, we visualized the lubricant film underneath the moving drop using reflection interference contrast microscopy. The three independent diagnostic tools and measurement techniques complement each other and reaffirm that drops oleoplane on tall dense pillars, while they graze over the pillar tops in tall sparse pillars. The critical density that forces this transition to drop friction is ≈50%. Furthermore, the experimental results show that friction on microholes and micropillars is comparable when the solid fraction is the same. The results reported in this study contradict past studies that reported the absence of an oil layer on tall pillars. Besides improving current understanding, the insights gained from this work provide design guidelines for turning drop friction on–off on demand for microfluidics applications.","PeriodicalId":5,"journal":{"name":"ACS Applied Materials & Interfaces","volume":"84 1","pages":""},"PeriodicalIF":8.2000,"publicationDate":"2025-10-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Drop Friction on Textured Lubricant-Coated Surfaces\",\"authors\":\"Xiaoyu Chen, Biruk Teka Gidreta, Tanner Gaw, Michal Remer, Dan Daniel, Xiaoguang Wang, Solomon Adera\",\"doi\":\"10.1021/acsami.5c08905\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"Understanding drop friction on textured surfaces has implications in microfluidics and lab-on-a-chip devices. In this work, we investigated the drop friction on lubricant-coated pillars by systematically varying pillar height and density. First, we measured the friction force on a moving drop using a cantilever force sensor that has ±0.1 μN sensitivity. This measurement shows that drop friction on tall dense pillars is comparable to drop friction on short pillars, a significant result that suggests the presence of a Landau–Levich–Derjaguin (LLD) film underneath the moving drop. Second, we validated the force measurement by estimating the lubricant layer thickness by using white-light interferometry. Third, we visualized the lubricant film underneath the moving drop using reflection interference contrast microscopy. The three independent diagnostic tools and measurement techniques complement each other and reaffirm that drops oleoplane on tall dense pillars, while they graze over the pillar tops in tall sparse pillars. The critical density that forces this transition to drop friction is ≈50%. Furthermore, the experimental results show that friction on microholes and micropillars is comparable when the solid fraction is the same. The results reported in this study contradict past studies that reported the absence of an oil layer on tall pillars. Besides improving current understanding, the insights gained from this work provide design guidelines for turning drop friction on–off on demand for microfluidics applications.\",\"PeriodicalId\":5,\"journal\":{\"name\":\"ACS Applied Materials & Interfaces\",\"volume\":\"84 1\",\"pages\":\"\"},\"PeriodicalIF\":8.2000,\"publicationDate\":\"2025-10-08\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"ACS Applied Materials & Interfaces\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://doi.org/10.1021/acsami.5c08905\",\"RegionNum\":2,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"MATERIALS SCIENCE, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"ACS Applied Materials & Interfaces","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1021/acsami.5c08905","RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"MATERIALS SCIENCE, MULTIDISCIPLINARY","Score":null,"Total":0}
Drop Friction on Textured Lubricant-Coated Surfaces
Understanding drop friction on textured surfaces has implications in microfluidics and lab-on-a-chip devices. In this work, we investigated the drop friction on lubricant-coated pillars by systematically varying pillar height and density. First, we measured the friction force on a moving drop using a cantilever force sensor that has ±0.1 μN sensitivity. This measurement shows that drop friction on tall dense pillars is comparable to drop friction on short pillars, a significant result that suggests the presence of a Landau–Levich–Derjaguin (LLD) film underneath the moving drop. Second, we validated the force measurement by estimating the lubricant layer thickness by using white-light interferometry. Third, we visualized the lubricant film underneath the moving drop using reflection interference contrast microscopy. The three independent diagnostic tools and measurement techniques complement each other and reaffirm that drops oleoplane on tall dense pillars, while they graze over the pillar tops in tall sparse pillars. The critical density that forces this transition to drop friction is ≈50%. Furthermore, the experimental results show that friction on microholes and micropillars is comparable when the solid fraction is the same. The results reported in this study contradict past studies that reported the absence of an oil layer on tall pillars. Besides improving current understanding, the insights gained from this work provide design guidelines for turning drop friction on–off on demand for microfluidics applications.
期刊介绍:
ACS Applied Materials & Interfaces is a leading interdisciplinary journal that brings together chemists, engineers, physicists, and biologists to explore the development and utilization of newly-discovered materials and interfacial processes for specific applications. Our journal has experienced remarkable growth since its establishment in 2009, both in terms of the number of articles published and the impact of the research showcased. We are proud to foster a truly global community, with the majority of published articles originating from outside the United States, reflecting the rapid growth of applied research worldwide.