Prasad P. Iyer*, , , Mihir Pendharkar, , , Anchal Agarwal, , , Humberto Foronda, , , Micheal Iza, , , Umesh K. Mishra, , , Shuji Nakamura, , , Steven DenBaars, , , Stacia Keller, , , Chris Palmstrøm, , and , Jon A. Schuller*,
{"title":"嵌入在零折射率腔中的高q、尺寸无关和可重构光学天线。","authors":"Prasad P. Iyer*, , , Mihir Pendharkar, , , Anchal Agarwal, , , Humberto Foronda, , , Micheal Iza, , , Umesh K. Mishra, , , Shuji Nakamura, , , Steven DenBaars, , , Stacia Keller, , , Chris Palmstrøm, , and , Jon A. Schuller*, ","doi":"10.1021/acsnano.5c04424","DOIUrl":null,"url":null,"abstract":"<p >Enhancing light–matter interactions at the nanoscale is foundational to nanophotonics, with epsilon-near-zero (ENZ) materials demonstrating significant potential. High-quality factor (<i>Q</i>) resonances that maximize these interactions are typically realized in photonic crystals requiring sub-50 nm precision nanofabrication over large areas, limiting scalability and increasing complexity. Mie resonances offer an alternative but are constrained by low <i>Q</i>-factors due to the scarcity of high-refractive index materials, necessitating large refractive index changes for effective resonance switching and limiting dynamic reconfigurability. We overcome these limitations by embedding Mie resonators within ENZ media, thereby enhancing <i>Q</i>-factors, mitigating geometric dispersion and fabrication challenges, and maximizing optical reconfigurability. We introduce three resonator-ENZ configurations: voids in AlN, Ge in SiO<sub>2</sub>, and intrinsic InSb in doped InSb─spanning from low-loss phononic to lossy plasmonic ENZ modes. Using novel epitaxial regrowth techniques, we achieve significant <i>Q</i>-factor improvements over nonembedded resonators. An air-based Mie resonator embedded in AlN supports resonant <i>Q</i>-factors exceeding 100, with negligible geometric dispersion across sizes from 800 to 2800 nm. Additionally, we demonstrate dynamic reconfigurability of intrinsic InSb resonators by thermally tuning the ENZ wavelength over a 2 μm range in the mid-infrared (11–16 μm) wavelength regime. These results showcase the potential of Mie reonators embedded in ENZ media for high-fidelity sensors, thermal emitters, and reconfigurable metasurfaces, bridging theoretical predictions with practical applications and advancing the development of dynamic, high-<i>Q</i> optical devices.</p>","PeriodicalId":21,"journal":{"name":"ACS Nano","volume":"19 41","pages":"36148–36157"},"PeriodicalIF":16.0000,"publicationDate":"2025-10-07","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"High-Q, Size-Independent, and Reconfigurable Optical Antennas Embedded in Zero-Index Cavities\",\"authors\":\"Prasad P. Iyer*, , , Mihir Pendharkar, , , Anchal Agarwal, , , Humberto Foronda, , , Micheal Iza, , , Umesh K. Mishra, , , Shuji Nakamura, , , Steven DenBaars, , , Stacia Keller, , , Chris Palmstrøm, , and , Jon A. Schuller*, \",\"doi\":\"10.1021/acsnano.5c04424\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p >Enhancing light–matter interactions at the nanoscale is foundational to nanophotonics, with epsilon-near-zero (ENZ) materials demonstrating significant potential. High-quality factor (<i>Q</i>) resonances that maximize these interactions are typically realized in photonic crystals requiring sub-50 nm precision nanofabrication over large areas, limiting scalability and increasing complexity. Mie resonances offer an alternative but are constrained by low <i>Q</i>-factors due to the scarcity of high-refractive index materials, necessitating large refractive index changes for effective resonance switching and limiting dynamic reconfigurability. We overcome these limitations by embedding Mie resonators within ENZ media, thereby enhancing <i>Q</i>-factors, mitigating geometric dispersion and fabrication challenges, and maximizing optical reconfigurability. We introduce three resonator-ENZ configurations: voids in AlN, Ge in SiO<sub>2</sub>, and intrinsic InSb in doped InSb─spanning from low-loss phononic to lossy plasmonic ENZ modes. Using novel epitaxial regrowth techniques, we achieve significant <i>Q</i>-factor improvements over nonembedded resonators. An air-based Mie resonator embedded in AlN supports resonant <i>Q</i>-factors exceeding 100, with negligible geometric dispersion across sizes from 800 to 2800 nm. Additionally, we demonstrate dynamic reconfigurability of intrinsic InSb resonators by thermally tuning the ENZ wavelength over a 2 μm range in the mid-infrared (11–16 μm) wavelength regime. 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High-Q, Size-Independent, and Reconfigurable Optical Antennas Embedded in Zero-Index Cavities
Enhancing light–matter interactions at the nanoscale is foundational to nanophotonics, with epsilon-near-zero (ENZ) materials demonstrating significant potential. High-quality factor (Q) resonances that maximize these interactions are typically realized in photonic crystals requiring sub-50 nm precision nanofabrication over large areas, limiting scalability and increasing complexity. Mie resonances offer an alternative but are constrained by low Q-factors due to the scarcity of high-refractive index materials, necessitating large refractive index changes for effective resonance switching and limiting dynamic reconfigurability. We overcome these limitations by embedding Mie resonators within ENZ media, thereby enhancing Q-factors, mitigating geometric dispersion and fabrication challenges, and maximizing optical reconfigurability. We introduce three resonator-ENZ configurations: voids in AlN, Ge in SiO2, and intrinsic InSb in doped InSb─spanning from low-loss phononic to lossy plasmonic ENZ modes. Using novel epitaxial regrowth techniques, we achieve significant Q-factor improvements over nonembedded resonators. An air-based Mie resonator embedded in AlN supports resonant Q-factors exceeding 100, with negligible geometric dispersion across sizes from 800 to 2800 nm. Additionally, we demonstrate dynamic reconfigurability of intrinsic InSb resonators by thermally tuning the ENZ wavelength over a 2 μm range in the mid-infrared (11–16 μm) wavelength regime. These results showcase the potential of Mie reonators embedded in ENZ media for high-fidelity sensors, thermal emitters, and reconfigurable metasurfaces, bridging theoretical predictions with practical applications and advancing the development of dynamic, high-Q optical devices.
期刊介绍:
ACS Nano, published monthly, serves as an international forum for comprehensive articles on nanoscience and nanotechnology research at the intersections of chemistry, biology, materials science, physics, and engineering. The journal fosters communication among scientists in these communities, facilitating collaboration, new research opportunities, and advancements through discoveries. ACS Nano covers synthesis, assembly, characterization, theory, and simulation of nanostructures, nanobiotechnology, nanofabrication, methods and tools for nanoscience and nanotechnology, and self- and directed-assembly. Alongside original research articles, it offers thorough reviews, perspectives on cutting-edge research, and discussions envisioning the future of nanoscience and nanotechnology.