Baosheng Chen, , , Yupei Zeng, , , Nan Peng*, , and , Ercang Luo*,
{"title":"超声速分离技术去除N2/He混合物中N2的数值研究","authors":"Baosheng Chen, , , Yupei Zeng, , , Nan Peng*, , and , Ercang Luo*, ","doi":"10.1021/acs.iecr.5c02209","DOIUrl":null,"url":null,"abstract":"<p >The application of supersonic separation technology in extracting helium from the N<sub>2</sub>/He mixture is the primary innovation of this work, holding noteworthy promise. To begin with, a numerical model is constructed, incorporating governing equations for gas–liquid phase and the condensation model. The study reveals that nitrogen nonequilibrium condensation can be accomplished using the Laval nozzle, demonstrating the potential for N<sub>2</sub>/He separation in the supersonic separator. Enhancing nitrogen nonequilibrium condensation within the Laval nozzle can be achieved by lowering the inlet temperature and raising the inlet pressure. Results show that nitrogen experiences intensive homogeneous nucleation over a short duration in the divergent section, leading to an ongoing rise in the nitrogen liquid mass fraction from 0% at the inlet to 10.5% at the outlet. This research verifies the viability of employing the Laval nozzle for nitrogen removal, carrying significant strategic implications for advancing nitrogen removal technologies in the recovery of helium from natural gas.</p>","PeriodicalId":39,"journal":{"name":"Industrial & Engineering Chemistry Research","volume":"64 41","pages":"20014–20029"},"PeriodicalIF":3.9000,"publicationDate":"2025-10-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Numerical Study on N2 Removal from the N2/He Mixture by Supersonic Separation Technology\",\"authors\":\"Baosheng Chen, , , Yupei Zeng, , , Nan Peng*, , and , Ercang Luo*, \",\"doi\":\"10.1021/acs.iecr.5c02209\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p >The application of supersonic separation technology in extracting helium from the N<sub>2</sub>/He mixture is the primary innovation of this work, holding noteworthy promise. To begin with, a numerical model is constructed, incorporating governing equations for gas–liquid phase and the condensation model. The study reveals that nitrogen nonequilibrium condensation can be accomplished using the Laval nozzle, demonstrating the potential for N<sub>2</sub>/He separation in the supersonic separator. Enhancing nitrogen nonequilibrium condensation within the Laval nozzle can be achieved by lowering the inlet temperature and raising the inlet pressure. Results show that nitrogen experiences intensive homogeneous nucleation over a short duration in the divergent section, leading to an ongoing rise in the nitrogen liquid mass fraction from 0% at the inlet to 10.5% at the outlet. This research verifies the viability of employing the Laval nozzle for nitrogen removal, carrying significant strategic implications for advancing nitrogen removal technologies in the recovery of helium from natural gas.</p>\",\"PeriodicalId\":39,\"journal\":{\"name\":\"Industrial & Engineering Chemistry Research\",\"volume\":\"64 41\",\"pages\":\"20014–20029\"},\"PeriodicalIF\":3.9000,\"publicationDate\":\"2025-10-06\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Industrial & Engineering Chemistry Research\",\"FirstCategoryId\":\"5\",\"ListUrlMain\":\"https://pubs.acs.org/doi/10.1021/acs.iecr.5c02209\",\"RegionNum\":3,\"RegionCategory\":\"工程技术\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"ENGINEERING, CHEMICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Industrial & Engineering Chemistry Research","FirstCategoryId":"5","ListUrlMain":"https://pubs.acs.org/doi/10.1021/acs.iecr.5c02209","RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"ENGINEERING, CHEMICAL","Score":null,"Total":0}
Numerical Study on N2 Removal from the N2/He Mixture by Supersonic Separation Technology
The application of supersonic separation technology in extracting helium from the N2/He mixture is the primary innovation of this work, holding noteworthy promise. To begin with, a numerical model is constructed, incorporating governing equations for gas–liquid phase and the condensation model. The study reveals that nitrogen nonequilibrium condensation can be accomplished using the Laval nozzle, demonstrating the potential for N2/He separation in the supersonic separator. Enhancing nitrogen nonequilibrium condensation within the Laval nozzle can be achieved by lowering the inlet temperature and raising the inlet pressure. Results show that nitrogen experiences intensive homogeneous nucleation over a short duration in the divergent section, leading to an ongoing rise in the nitrogen liquid mass fraction from 0% at the inlet to 10.5% at the outlet. This research verifies the viability of employing the Laval nozzle for nitrogen removal, carrying significant strategic implications for advancing nitrogen removal technologies in the recovery of helium from natural gas.
期刊介绍:
ndustrial & Engineering Chemistry, with variations in title and format, has been published since 1909 by the American Chemical Society. Industrial & Engineering Chemistry Research is a weekly publication that reports industrial and academic research in the broad fields of applied chemistry and chemical engineering with special focus on fundamentals, processes, and products.