土壤侵蚀过程中粒间力和流速对粘粒运动的影响

IF 5.7 1区 农林科学 Q1 GEOSCIENCES, MULTIDISCIPLINARY
Mao Qiu , Xiaochao Zhang , Xiangjun Pei , Xi Yang , Xiaoyi Zhao , Hongchao Xi , Jining Zhang , Renji Zhang , Renjie Wei , Yu Zhou
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引用次数: 0

摘要

土壤侵蚀过程中粘土颗粒的运动受宏观水动力和微观颗粒间力(静电斥力、范德华力和水化斥力)共同控制;然而,微观力学机制尚不清楚。本研究建立了可视化微流控实验平台,通过控制电解质浓度来调节颗粒间力,并结合高速摄影系统,研究流体速度和颗粒间力对粘土颗粒分离、迁移和碰撞粘附行为的影响。结果表明:颗粒间净斥力增大,土壤抗侵蚀能力显著减弱;在粒子间距为2 nm时,净斥力的临界阈值为5.72 atm。超过这个阈值,黏土团聚体破碎释放的粒径小于20 μm颗粒的比例超过70%。此外,侵蚀速率增加了7倍以上,单个输运颗粒的比例急剧增加。低于这个阈值,吸引力起主导作用,颗粒倾向于聚集,侵蚀主要通过块体分离发生,导致侵蚀速率较低。增大流速可显著增大侵蚀速率;流速增加10倍会导致侵蚀速率增加7.5 - 13倍。此外,流速决定了粒子碰撞频率。总体而言,流速和颗粒-颗粒斥力协同驱动侵蚀;然而,流速的贡献是主要的。定量揭示了流速优势和粒间力协同驱动的侵蚀机理,为研究粘土侵蚀的微观力学提供了新的思路。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Influence of inter particle force and flow velocity on the motion of clay particles during soil erosion
Clay particle movement during soil erosion is jointly controlled by macroscopic hydrodynamic and microscopic interparticle forces (electrostatic repulsion, van der Waals forces, and hydration repulsion); however, the microscopic mechanical mechanisms remain unclear. This study established a visual microfluidic experimental platform, adjusting interparticle forces by controlling the electrolyte concentration, and combined it with a high-speed photography system to investigate the effects of fluid velocity and interparticle forces on clay particle separation, migration, and collision-adhesion behavior. The results indicated that an increase in the net repulsive force between the particles significantly weakens soil erosion resistance. The critical threshold for the net repulsive force at a particle spacing of 2 nm was 5.72 atm. Beyond this threshold, the proportion of particles with a diameter of less than 20 μm released from the breakdown of clay aggregates exceeds 70 %. Moreover, the erosion rates increase by more than sevenfold, and the proportion of individual transported particles sharply increases. Below this threshold, attractive forces dominate, particles tend to aggregate, and erosion occurs primarily through block detachment, resulting in lower erosion rates. Increasing the flow velocity significantly amplifies erosion rates; a 10-fold increase in flow velocity results in a 7.5–13-fold increase in erosion rates. Additionally, the flow velocity governs the particle collision frequency. Overall, the flow velocity and particle–particle repulsive forces synergistically drive erosion; however, flow velocity’s contribution is dominant. This study quantitatively revealed the erosion mechanism driven by flow velocity dominance and interparticle force synergy, providing new insights into the microscopic mechanics of clay erosion.
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来源期刊
Catena
Catena 环境科学-地球科学综合
CiteScore
10.50
自引率
9.70%
发文量
816
审稿时长
54 days
期刊介绍: Catena publishes papers describing original field and laboratory investigations and reviews on geoecology and landscape evolution with emphasis on interdisciplinary aspects of soil science, hydrology and geomorphology. It aims to disseminate new knowledge and foster better understanding of the physical environment, of evolutionary sequences that have resulted in past and current landscapes, and of the natural processes that are likely to determine the fate of our terrestrial environment. Papers within any one of the above topics are welcome provided they are of sufficiently wide interest and relevance.
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