{"title":"煤层气渗流渗透率-黏度双重控制:优化固存的碳安全监管评价","authors":"Dahan Yang, , , Xinlei Xu, , , Zhengdong Liu, , , Wenxu Xu, , , Dingbo Zhou, , , Wang Tong, , and , Naishun Bu*, ","doi":"10.1021/acsomega.5c05268","DOIUrl":null,"url":null,"abstract":"<p >Geological sequestration of CO<sub>2</sub> in coal seams is one of the effective methods to reduce carbon emissions. However, the combined effects of evolving CO<sub>2</sub> viscosity and the inherently low permeability of coal reservoirs can significantly inhibit CO<sub>2</sub> flow capacity, thereby affecting the overall storage efficiency. The dynamic dual-control mechanisms governing CO<sub>2</sub> migration in coal seams remain insufficiently understood. The analysis of dynamic dual-control weights influencing CO<sub>2</sub> flow behavior is focused on in this study. On this basis, a mathematical model is developed and numerical simulations are conducted. The model captures the transient evolution of CO<sub>2</sub> viscosity and the permeability of coal seams during the sequestration process and investigates the coupling relationship between CO<sub>2</sub> properties and coal seam permeability. Two mathematical decomposition methods─the logarithmic decomposition method and the finite difference decomposition method─are employed to perform parameter decoupling analysis of CO<sub>2</sub> migration in coal seams. The dynamic coupling characteristics between permeability and viscosity are elucidated, and the dominant influence weights of their evolution on the CO<sub>2</sub> flow field are quantitatively evaluated. The study clarifies the stage-dependent control of fluid migration: permeability dominates initially, viscosity gains influence midstage, and both reach dynamic equilibrium over time. A dynamic dual-control weighting approach is proposed to optimize injection strategies, aiming to enhance CO<sub>2</sub> mobility and storage efficiency in an economically viable manner. The findings provide a theoretical basis for the accurate performance assessment of CO<sub>2</sub> sequestration in coal seams.</p>","PeriodicalId":22,"journal":{"name":"ACS Omega","volume":"10 38","pages":"44087–44097"},"PeriodicalIF":4.3000,"publicationDate":"2025-09-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/pdf/10.1021/acsomega.5c05268","citationCount":"0","resultStr":"{\"title\":\"Dual Control of Permeability-Viscosity in Coalbed CO2 Flow: Carbon Safety Supervision Assessment for Optimized Sequestration\",\"authors\":\"Dahan Yang, , , Xinlei Xu, , , Zhengdong Liu, , , Wenxu Xu, , , Dingbo Zhou, , , Wang Tong, , and , Naishun Bu*, \",\"doi\":\"10.1021/acsomega.5c05268\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p >Geological sequestration of CO<sub>2</sub> in coal seams is one of the effective methods to reduce carbon emissions. However, the combined effects of evolving CO<sub>2</sub> viscosity and the inherently low permeability of coal reservoirs can significantly inhibit CO<sub>2</sub> flow capacity, thereby affecting the overall storage efficiency. The dynamic dual-control mechanisms governing CO<sub>2</sub> migration in coal seams remain insufficiently understood. The analysis of dynamic dual-control weights influencing CO<sub>2</sub> flow behavior is focused on in this study. On this basis, a mathematical model is developed and numerical simulations are conducted. The model captures the transient evolution of CO<sub>2</sub> viscosity and the permeability of coal seams during the sequestration process and investigates the coupling relationship between CO<sub>2</sub> properties and coal seam permeability. Two mathematical decomposition methods─the logarithmic decomposition method and the finite difference decomposition method─are employed to perform parameter decoupling analysis of CO<sub>2</sub> migration in coal seams. The dynamic coupling characteristics between permeability and viscosity are elucidated, and the dominant influence weights of their evolution on the CO<sub>2</sub> flow field are quantitatively evaluated. The study clarifies the stage-dependent control of fluid migration: permeability dominates initially, viscosity gains influence midstage, and both reach dynamic equilibrium over time. A dynamic dual-control weighting approach is proposed to optimize injection strategies, aiming to enhance CO<sub>2</sub> mobility and storage efficiency in an economically viable manner. The findings provide a theoretical basis for the accurate performance assessment of CO<sub>2</sub> sequestration in coal seams.</p>\",\"PeriodicalId\":22,\"journal\":{\"name\":\"ACS Omega\",\"volume\":\"10 38\",\"pages\":\"44087–44097\"},\"PeriodicalIF\":4.3000,\"publicationDate\":\"2025-09-16\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"https://pubs.acs.org/doi/pdf/10.1021/acsomega.5c05268\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"ACS Omega\",\"FirstCategoryId\":\"92\",\"ListUrlMain\":\"https://pubs.acs.org/doi/10.1021/acsomega.5c05268\",\"RegionNum\":3,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"CHEMISTRY, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"ACS Omega","FirstCategoryId":"92","ListUrlMain":"https://pubs.acs.org/doi/10.1021/acsomega.5c05268","RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
Dual Control of Permeability-Viscosity in Coalbed CO2 Flow: Carbon Safety Supervision Assessment for Optimized Sequestration
Geological sequestration of CO2 in coal seams is one of the effective methods to reduce carbon emissions. However, the combined effects of evolving CO2 viscosity and the inherently low permeability of coal reservoirs can significantly inhibit CO2 flow capacity, thereby affecting the overall storage efficiency. The dynamic dual-control mechanisms governing CO2 migration in coal seams remain insufficiently understood. The analysis of dynamic dual-control weights influencing CO2 flow behavior is focused on in this study. On this basis, a mathematical model is developed and numerical simulations are conducted. The model captures the transient evolution of CO2 viscosity and the permeability of coal seams during the sequestration process and investigates the coupling relationship between CO2 properties and coal seam permeability. Two mathematical decomposition methods─the logarithmic decomposition method and the finite difference decomposition method─are employed to perform parameter decoupling analysis of CO2 migration in coal seams. The dynamic coupling characteristics between permeability and viscosity are elucidated, and the dominant influence weights of their evolution on the CO2 flow field are quantitatively evaluated. The study clarifies the stage-dependent control of fluid migration: permeability dominates initially, viscosity gains influence midstage, and both reach dynamic equilibrium over time. A dynamic dual-control weighting approach is proposed to optimize injection strategies, aiming to enhance CO2 mobility and storage efficiency in an economically viable manner. The findings provide a theoretical basis for the accurate performance assessment of CO2 sequestration in coal seams.
ACS OmegaChemical Engineering-General Chemical Engineering
CiteScore
6.60
自引率
4.90%
发文量
3945
审稿时长
2.4 months
期刊介绍:
ACS Omega is an open-access global publication for scientific articles that describe new findings in chemistry and interfacing areas of science, without any perceived evaluation of immediate impact.