煤层气渗流渗透率-黏度双重控制:优化固存的碳安全监管评价

IF 4.3 3区 化学 Q2 CHEMISTRY, MULTIDISCIPLINARY
ACS Omega Pub Date : 2025-09-16 DOI:10.1021/acsomega.5c05268
Dahan Yang, , , Xinlei Xu, , , Zhengdong Liu, , , Wenxu Xu, , , Dingbo Zhou, , , Wang Tong, , and , Naishun Bu*, 
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引用次数: 0

摘要

煤层地质封存是减少煤层碳排放的有效方法之一。然而,不断变化的CO2粘度和煤储层固有的低渗透性共同作用会显著抑制CO2的流动能力,从而影响整体储层效率。控制煤层中CO2运移的动态双控机制尚不清楚。本文着重分析了影响CO2流动特性的动态双控权值。在此基础上,建立了数学模型并进行了数值模拟。该模型捕捉了封存过程中CO2黏度与煤层渗透率的瞬态演化,研究了CO2性质与煤层渗透率的耦合关系。采用对数分解法和有限差分分解法两种数学分解方法对煤层中CO2运移进行参数解耦分析。阐明了渗透率和粘度的动态耦合特性,定量评价了它们的演化对CO2流场的主导影响权重。该研究阐明了流体运移的阶段依赖控制:渗透率在初期起主导作用,粘度增加影响中期,两者随着时间的推移达到动态平衡。提出了一种动态双控制加权方法来优化注入策略,旨在以经济可行的方式提高二氧化碳的流动性和储存效率。研究结果为准确评价煤层CO2固存性能提供了理论依据。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Dual Control of Permeability-Viscosity in Coalbed CO2 Flow: Carbon Safety Supervision Assessment for Optimized Sequestration

Geological sequestration of CO2 in coal seams is one of the effective methods to reduce carbon emissions. However, the combined effects of evolving CO2 viscosity and the inherently low permeability of coal reservoirs can significantly inhibit CO2 flow capacity, thereby affecting the overall storage efficiency. The dynamic dual-control mechanisms governing CO2 migration in coal seams remain insufficiently understood. The analysis of dynamic dual-control weights influencing CO2 flow behavior is focused on in this study. On this basis, a mathematical model is developed and numerical simulations are conducted. The model captures the transient evolution of CO2 viscosity and the permeability of coal seams during the sequestration process and investigates the coupling relationship between CO2 properties and coal seam permeability. Two mathematical decomposition methods─the logarithmic decomposition method and the finite difference decomposition method─are employed to perform parameter decoupling analysis of CO2 migration in coal seams. The dynamic coupling characteristics between permeability and viscosity are elucidated, and the dominant influence weights of their evolution on the CO2 flow field are quantitatively evaluated. The study clarifies the stage-dependent control of fluid migration: permeability dominates initially, viscosity gains influence midstage, and both reach dynamic equilibrium over time. A dynamic dual-control weighting approach is proposed to optimize injection strategies, aiming to enhance CO2 mobility and storage efficiency in an economically viable manner. The findings provide a theoretical basis for the accurate performance assessment of CO2 sequestration in coal seams.

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来源期刊
ACS Omega
ACS Omega Chemical Engineering-General Chemical Engineering
CiteScore
6.60
自引率
4.90%
发文量
3945
审稿时长
2.4 months
期刊介绍: ACS Omega is an open-access global publication for scientific articles that describe new findings in chemistry and interfacing areas of science, without any perceived evaluation of immediate impact.
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