基于双曲率herriott型多通道气体电池的高灵敏度TDLAS气体传感器

IF 3.7 1区 化学 Q1 CHEMISTRY, ANALYTICAL
Haiyong Chen, Xiaolu Ma, Mengchao Yan, Hongjun Ren, Hua-Yao Li, Yuheng Wu, Zishuo Xiao, Xinjie Zheng, Qingyong Yang, Fukang Ding, Huan Liu
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引用次数: 0

摘要

可调谐二极管激光吸收光谱(TDLAS)气体传感器非常适用于快速、准确的气体检测。TDLAS气体传感器面临的挑战是将光与气体之间的相互作用转换为密闭空间内的敏感传感器信号。解决这一挑战的一个有效方法主要是设计小型化的多通道气体电池(mpgc),以延长有效光程长度(EOPL)。在传统的herriott型MPGC设计中,由于使用单曲率反射镜,限制了镜面的利用率和光斑的完整性。本文提出了一种具有独特的三同心圆光斑图案的herriott型mpgc双曲率反射镜设计策略。光线追踪模拟是基于光学传输模型进行的,该模型定量地联系了反射镜间距、入射光束参数和产生的光斑分布。在155.13 mL的体积内,最佳MPGC原型的EOPL为32.05 m,从而实现了20.66 cm−2的高光路长度与体积之比。通过波长调制光谱的结合,我们开发了一种检测限低至33.78 ppb的甲烷TDLAS气体传感器。双曲率herriott型mpgc为高灵敏度TDLAS气体传感器的小型化提供了新的自由度。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Highly sensitive TDLAS gas sensor based on a dual-curvature Herriott-type multi-pass gas cell

Highly sensitive TDLAS gas sensor based on a dual-curvature Herriott-type multi-pass gas cell
Tunable diode laser absorption spectroscopy (TDLAS) gas sensors are highly suitable for rapid and accurate gas detection. The challenge for the TDLAS gas sensors is to convert the interaction between light and gas into a sensitive sensor signal within a confined space. One effective method to address this challenge has come primarily from the design of miniaturized multi-pass gas cells (MPGCs) to extend effective optical path length (EOPL). In the conventional Herriott-type MPGC design, the utilization rate of the mirror surface and the integrity of the light spot are both limited due to the use of a single-curvature mirror. Here, we propose a dual-curvature mirror design strategy for the Herriott-type MPGCs, featuring a unique three-concentric-circle spot pattern. The ray-tracing simulations were conducted based on an optical transmission model that quantitatively relates mirror spacing, incident beam parameters, and the resulting spot distribution. The optimal MPGC prototype exhibited an EOPL of 32.05 m within a volume of 155.13 mL, thereby achieving a high ratio of optical path length to volume of 20.66 cm−2. Through a combination of wavelength modulation spectroscopy, we have developed a methane TDLAS gas sensor with a detection limit as low as 33.78 ppb. The dual-curvature Herriott-type MPGCs offer a new degree of freedom for the miniaturization of highly sensitive TDLAS gas sensors.
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来源期刊
Sensors and Actuators B: Chemical
Sensors and Actuators B: Chemical 工程技术-电化学
CiteScore
14.60
自引率
11.90%
发文量
1776
审稿时长
3.2 months
期刊介绍: Sensors & Actuators, B: Chemical is an international journal focused on the research and development of chemical transducers. It covers chemical sensors and biosensors, chemical actuators, and analytical microsystems. The journal is interdisciplinary, aiming to publish original works showcasing substantial advancements beyond the current state of the art in these fields, with practical applicability to solving meaningful analytical problems. Review articles are accepted by invitation from an Editor of the journal.
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